Synthesis of multi-color laser pulses has been developed as a promising way to improve low conversion efficiency of high-order harmonic generation(HHG). Here we systematically study the effect of laser focus in a two-...Synthesis of multi-color laser pulses has been developed as a promising way to improve low conversion efficiency of high-order harmonic generation(HHG). Here we systematically study the effect of laser focus in a two-color waveform on generation of macroscopic HHG in soft x-rays. We find that the dependence of HHG yields on laser focus at low or high gas pressure is sensitive to the characteristics of single-atom harmonic response, in which “short”-or “long”-trajectory emissions can be selectively controlled by changing the waveform of two-color synthesized laser pulse. We uncover the phase-matching mechanism of HHG in the gas medium by examining the propagation of the two-color waveform and the evolution of time-frequency emissions of high-harmonic field. We further reveal that the nonlinear effects, such as geometric phase, atomic dispersion, and plasma defocusing, are responsible for modification of two-color waveform upon propagation. This work can be used to find better macroscopic conditions for generating soft x-ray HHG by employing two-color optimized waveforms.展开更多
The purpose of this paper is to study the air pollutants in Xiong’an New Area based on MATLAB grey model [1]. From 2011 to 2016, the results of sulfur dioxide (SO2), nitrogen dioxide (NO2) and inhalable particulate m...The purpose of this paper is to study the air pollutants in Xiong’an New Area based on MATLAB grey model [1]. From 2011 to 2016, the results of sulfur dioxide (SO2), nitrogen dioxide (NO2) and inhalable particulate matter (PM1O) detected at monitoring points in the three counties of Xiong’an were analyzed. According to the national environmental air quality standard [2], the air quality in Xiong’an New Area was reasonably evaluated based on grey model in MATLAB. Judging from the weight of pollution factors in the model, sulfur dioxide (SO2) is the controlling factor of air quality in Xiong’an New Area, and the weight of nitrogen dioxide (NO2) gradually increases. The main sources of the three pollutants were obtained by comprehensive data analysis, and a grey model was established according to the mass concentration of the main air pollutants, and the grey forecasting model was tested. The experimental results show that the model can be effectively applied to the forecasting of ambient air quality. On this basis, the present situation of atmospheric environmental quality in Xiong’an New Area and suggestions for improvement are obtained.展开更多
Nonadiabatic phase matching of high-harmonic generation(HHG)driven by few-cycle laser pulses is essential for extending harmonic energy and generating isolated attosecond pulses.However,understanding nonadiabatic HHG ...Nonadiabatic phase matching of high-harmonic generation(HHG)driven by few-cycle laser pulses is essential for extending harmonic energy and generating isolated attosecond pulses.However,understanding nonadiabatic HHG is challenging due to the complex interplay of various optical phases driven by temporally and spatially varying laser fields.Theoretical calculations typically rely on computationally demanding 3-dimensional simulations,which can make it difficult to extract the essential features of nonadiabatic HHG.In this work,we develop a computationally efficient 2-dimensional model that directly considers various phase contributions of HHG.Our model can well explain the experimentally observed pressure-and intensity-dependent behaviors of different harmonic orders.By appropriately parameterizing the single-atom response,our model can also estimate the variation of HHG spectra under different driving conditions.Our model can provide an efficient tool for the design and optimization of HHG-based applications.展开更多
基金Project supported by the National Natural Science Foundation of China (Grant Nos.91950102,12274230,and 11834004)the Funding of Nanjing University of Science and Technology (Grant No.TSXK2022D005)。
文摘Synthesis of multi-color laser pulses has been developed as a promising way to improve low conversion efficiency of high-order harmonic generation(HHG). Here we systematically study the effect of laser focus in a two-color waveform on generation of macroscopic HHG in soft x-rays. We find that the dependence of HHG yields on laser focus at low or high gas pressure is sensitive to the characteristics of single-atom harmonic response, in which “short”-or “long”-trajectory emissions can be selectively controlled by changing the waveform of two-color synthesized laser pulse. We uncover the phase-matching mechanism of HHG in the gas medium by examining the propagation of the two-color waveform and the evolution of time-frequency emissions of high-harmonic field. We further reveal that the nonlinear effects, such as geometric phase, atomic dispersion, and plasma defocusing, are responsible for modification of two-color waveform upon propagation. This work can be used to find better macroscopic conditions for generating soft x-ray HHG by employing two-color optimized waveforms.
文摘The purpose of this paper is to study the air pollutants in Xiong’an New Area based on MATLAB grey model [1]. From 2011 to 2016, the results of sulfur dioxide (SO2), nitrogen dioxide (NO2) and inhalable particulate matter (PM1O) detected at monitoring points in the three counties of Xiong’an were analyzed. According to the national environmental air quality standard [2], the air quality in Xiong’an New Area was reasonably evaluated based on grey model in MATLAB. Judging from the weight of pollution factors in the model, sulfur dioxide (SO2) is the controlling factor of air quality in Xiong’an New Area, and the weight of nitrogen dioxide (NO2) gradually increases. The main sources of the three pollutants were obtained by comprehensive data analysis, and a grey model was established according to the mass concentration of the main air pollutants, and the grey forecasting model was tested. The experimental results show that the model can be effectively applied to the forecasting of ambient air quality. On this basis, the present situation of atmospheric environmental quality in Xiong’an New Area and suggestions for improvement are obtained.
基金Z.T.gratefully acknowledges support from the National Key Research and Development Program of China(Grant Nos.2021YFA1400200 and 2022YFA1404700)National Natural Science Foundation of China(Grant No.12221004)+4 种基金Shanghai Municipal Science and Technology Basic Research Project(Grant No.19JC1410900)B.L.and C.Jj.were supported by the National Natural Science Foundation of China(Grant No.12274230)Funding of NJUST(Grant No.TSXK2022D005)Y.L.acknowledges support from the National Natural Science Foundation of China(Grant No.12034013)G.F.acknowledges support from the National Natural Science Foundation of China(Grant No.12374318).
文摘Nonadiabatic phase matching of high-harmonic generation(HHG)driven by few-cycle laser pulses is essential for extending harmonic energy and generating isolated attosecond pulses.However,understanding nonadiabatic HHG is challenging due to the complex interplay of various optical phases driven by temporally and spatially varying laser fields.Theoretical calculations typically rely on computationally demanding 3-dimensional simulations,which can make it difficult to extract the essential features of nonadiabatic HHG.In this work,we develop a computationally efficient 2-dimensional model that directly considers various phase contributions of HHG.Our model can well explain the experimentally observed pressure-and intensity-dependent behaviors of different harmonic orders.By appropriately parameterizing the single-atom response,our model can also estimate the variation of HHG spectra under different driving conditions.Our model can provide an efficient tool for the design and optimization of HHG-based applications.