Naturally Crosslinked Biocompatible Carbonaceous Liquid Metal Aqueous Ink Printing Wearable Electronics for Multi-Sensing and Energy Harvesting

Achieving flexible electronics with comfort and durability comparable to traditional textiles is one of the ultimate pursuits of smart wearables.Ink printing is desirable for e-textile development using a simple and inexpensive process.However,fabricating high-performance atop textiles with good dispersity,stability,biocompatibility,and wearability for high-resolution,large-scale manufacturing,and practical applications has remained challenging.Here,waterbased multi-walled carbon nanotubes(MWCNTs)-decorated liquid metal(LM)inks are proposed with carbonaceous gallium–indium micro-nanostructure.With the assistance of biopolymers,the sodium alginate-encapsulated LM droplets contain high carboxyl groups which non-covalently crosslink with silk sericin-mediated MWCNTs.E-textile can be prepared subsequently via printing technique and natural waterproof triboelectric coating,enabling good flexibility,hydrophilicity,breathability,wearability,biocompatibility,conductivity,stability,and excellent versatility,without any artificial chemicals.The obtained e-textile can be used in various applications with designable patterns and circuits.Multi-sensing applications of recognizing complex human motions,breathing,phonation,and pressure distribution are demonstrated with repeatable and reliable signals.Self-powered and energy-harvesting capabilities are also presented by driving electronic devices and lighting LEDs.As proof of concept,this work provides new opportunities in a scalable and sustainable way to develop novel wearable electronics and smart clothing for future commercial applications.

Advanced Design of Soft Robots with Artificial Intelligence

In recent years,breakthrough has been made in the field of artificial intelligence(AI),which has also revolutionized the industry of robotics.Soft robots featured with high-level safety,less weight,lower power consumption have always been one of the research hotspots.Recently,multifunctional sensors for perception of soft robotics have been rapidly developed,while more algorithms and models of machine learning with high accuracy have been optimized and proposed.Designs of soft robots with AI have also been advanced ranging from multimodal sensing,human-machine interaction to effective actuation in robotic systems.Nonethe-less,comprehensive reviews concerning the new developments and strategies for the ingenious design of the soft robotic systems equipped with AI are rare.Here,the new development is systematically reviewed in the field of soft robots with AI.First,background and mechanisms of soft robotic systems are briefed,after which development focused on how to endow the soft robots with AI,including the aspects of feeling,thought and reaction,is illustrated.Next,applications of soft robots with AI are systematically summarized and discussed together with advanced strategies proposed for performance enhancement.Design thoughts for future intelligent soft robotics are pointed out.Finally,some perspectives are put forward.

Solution‑Processed Transparent Conducting Electrodes for Flexible Organic Solar Cells with 16.61% Efficiency

Nonfullerene organic solar cells(OSCs)have achieved breakthrough with pushing the efficiency exceeding 17%.While this shed light on OSC commercialization,high-performance flexible OSCs should be pursued through solution manufacturing.Herein,we report a solution-processed flexible OSC based on a transparent conducting PEDOT:PSS anode doped with trifluoromethanesulfonic acid(CF3SO3H).Through a low-concentration and low-temperature CF3SO3H doping,the conducting polymer anodes exhibited a main sheet resistance of 35Ωsq−1(minimum value:32Ωsq−1),a raised work function(≈5.0 eV),a superior wettability,and a high electrical stability.The high work function minimized the energy level mismatch among the anodes,hole-transporting layers and electron-donors of the active layers,thereby leading to an enhanced carrier extraction.The solution-processed flexible OSCs yielded a record-high efficiency of 16.41%(maximum value:16.61%).Besides,the flexible OSCs afforded the 1000 cyclic bending tests at the radius of 1.5 mm and the long-time thermal treatments at 85°C,demonstrating a high flexibility and a good thermal stability.

Toward Flexible and Wearable Embroidered Supercapacitors from Cobalt Phosphides-Decorated Conductive Fibers

Wearable supercapacitors(SCs)are gaining prominence as portable energy storage devices.To develop high-performance wearable SCs,the significant relationship among material,structure,and performance inspired us with a delicate design of the highly wearable embroidered supercapacitors made from the conductive fibers composited.By rendering the conductive interdigitally patterned embroidery as both the current collector and skeleton for the SCs,the novel pseudocapacitive material cobalt phosphides were then successfully electrodeposited,forming the first flexible and wearable in-plane embroidery SCs.The electrochemical measurements manifested that the highest specific capacitance was nearly 156.6 mF cm?2(65.72 F g?1)at the current density of 0.6 mA cm?2(0.25 A g?1),with a high energy density of 0.013 mWh cm?2(5.55 Wh kg?1)at a power density of 0.24 mW cm?2(100 W kg?1).As a demonstration,a monogrammed pattern was ingeniously designed and embroidered on the laboratory gown as the wearable in-plane SCs,which showed both decent electrochemical performance and excellent flexibility.

Revolutionizing digital healthcare networks with wearable strain sensors using sustainable fibers

Wearable strain sensors have attracted research interest owing to their poten-tial within digital healthcare,offering smarter tracking,efficient diagnostics,and lower costs.Unlike rigid sensors,fiber-based ones compete with their flexibility,durability,adaptability to body structures as well as eco-friendliness to envi-ronment.Here,the sustainable fiber-based wearable strain sensors for digital health are reviewed,and material,fabrication,and practical healthcare aspects are explored.Typical strain sensors predicated on various sensing modalities,be it resistive,capacitive,piezoelectric,or triboelectric,are explained and analyzed according to their strengths and weaknesses toward fabrication and applica-tions.The applications in digital healthcare spanning from body area sensing networks,intelligent health management,and medical rehabilitation to mul-tifunctional healthcare systems are also evaluated.Moreover,to create a more complete digital health network,wired and wireless methods of data collec-tion and examples of machine learning are elaborated in detail.Finally,the prevailing challenges and prospective insights into the advancement of novel fibers,enhancement of sensing precision and wearability,and the establishment of seamlessly integrated systems are critically summarized and offered.This endeavor not only encapsulates the present landscape but also lays the founda-tion for future breakthroughs in fiber-based wearable strain sensor technology within the domain of digital health.