In the safety assessment of a potential site for high-level radioactive wastes (HLW) disposal, the investigation on the geochemical behaviors of key radionuclides with the possibility for releasing from the potential ...In the safety assessment of a potential site for high-level radioactive wastes (HLW) disposal, the investigation on the geochemical behaviors of key radionuclides with the possibility for releasing from the potential repository is an important aspect. Due to the high mobility of technetium under most repository conditions, lots of research works were performed to investigate the diffusion of technetium in different potential rocks. In spite of these studies, there remains a lack of data addressing temperature effects. In this paper, the diffusion of 99Tc in Beishan granite at temperatures from 25℃ to 55℃ was studied with laboratory small scale diffusion devices. The experimental data were fitted with a finite difference scheme to get the effective diffusion coefficient (De) of . The results indicated that the relationship of De with temperatures could be described as the modified Stokes-Einstein equation, and the formation factor of Beishan granite was constant in the temperature range of 25℃ - 55℃ with the value of (3.91 ± 1.77) × 10-4.展开更多
The number of J/ψ events collected with the BES detector at the BEPC from June 12 to July 28, 2009 is determined to be (225.3 ± 2.8) × 10^ 6 using J/ψ→inclusive events, where the uncertainty is the syst...The number of J/ψ events collected with the BES detector at the BEPC from June 12 to July 28, 2009 is determined to be (225.3 ± 2.8) × 10^ 6 using J/ψ→inclusive events, where the uncertainty is the systematic error and the statistical one is negligible.展开更多
文摘In the safety assessment of a potential site for high-level radioactive wastes (HLW) disposal, the investigation on the geochemical behaviors of key radionuclides with the possibility for releasing from the potential repository is an important aspect. Due to the high mobility of technetium under most repository conditions, lots of research works were performed to investigate the diffusion of technetium in different potential rocks. In spite of these studies, there remains a lack of data addressing temperature effects. In this paper, the diffusion of 99Tc in Beishan granite at temperatures from 25℃ to 55℃ was studied with laboratory small scale diffusion devices. The experimental data were fitted with a finite difference scheme to get the effective diffusion coefficient (De) of . The results indicated that the relationship of De with temperatures could be described as the modified Stokes-Einstein equation, and the formation factor of Beishan granite was constant in the temperature range of 25℃ - 55℃ with the value of (3.91 ± 1.77) × 10-4.
基金Supported by Ministry of Science and Technology of China (2009CB825200)National Natural Science Foundation of China (NSFC) (10625524, 10821063, 10825524, 10835001, 10935007, 11125525)+3 种基金Joint Funds of National Natural Science Foundation of China (11079008, 11179007)Chinese Academy of Sciences (CAS) Large-Scale Scientific Facility Program (KJCX2-YW-N29, KJCX2-YW-N45)100 Talents Program of CAS, Istituto Nazionale di Fisica Nucleare, Italy, U. S. Department of Energy (DE-FG02-04ER41291, DE-FG02-91ER40682, DE-FG02-94ER40823)U.S. National Science Foundation, University of Groningen (RuG) and the Helmholtzzentrum fuer Schwerionenforschung GmbH (GSI), Darmstadt, WCU Program of National Research Foundation of Korea (R32-2008-000-10155-0)
文摘The number of J/ψ events collected with the BES detector at the BEPC from June 12 to July 28, 2009 is determined to be (225.3 ± 2.8) × 10^ 6 using J/ψ→inclusive events, where the uncertainty is the systematic error and the statistical one is negligible.