We proposed a green microwave-assisted hydrothermal way to synthesize highly crystalized N-doped carbon quantum dots(N-CQDs).The N-CQDs obtained by this microwave method have good crystalline degree(ID/IG=0.6)and a hi...We proposed a green microwave-assisted hydrothermal way to synthesize highly crystalized N-doped carbon quantum dots(N-CQDs).The N-CQDs obtained by this microwave method have good crystalline degree(ID/IG=0.6)and a high molar ratio of N/C(11.1%)comparing with those obtained from traditional top-down method.The experimental results show that glycerine plays a key role ill the fonnation of highly crystalized N-CQDs.The as-prepared N-CQDs have good luminescent property and may be utilized as fluorescent probe to detect ions or mark cells.As the majority of N atoms in the N-CQDs were pyridinic type(64.8%),the as-prepared N-CQDs were used as a catalyst for the oxygen reduction reaction(ORR)electrocatalysis in the anode of the fuel cell(the onset potential is-0.121V),which was a 4e-transfer procedure and the catalyst showed good stability after 100 cycles.展开更多
Mesh morphing is a technique which gradually deforms a mesh into another one. Mesh parameterization, a powerful tool adopted to establish the one-to-one correspondence map between different meshes, is of great importa...Mesh morphing is a technique which gradually deforms a mesh into another one. Mesh parameterization, a powerful tool adopted to establish the one-to-one correspondence map between different meshes, is of great importance in 3 D mesh morphing. However, current parameterization methods used in mesh morphing induce large area distortion, resulting in geometric information loss. In this paper, we propose a new morphing approach for topological disk meshes based on area-preserving parameterization. Conformal mapping and M？bius transformation are computed firstly as rough alignment. Then area preserving parameterization is computed via the discrete optimal mass transport map. Features are exactly aligned through radial basis functions. A surface remeshing scheme via Delaunay refinement algorithm is developed to create a new mesh connectivity. Experimental results demonstrate that the proposed method performs well and generates high-quality morphs.展开更多
基金the National Natural Science Foundation of China(Nos.21771084,21771077,21621001)the National Key Research and Development Program of China(No.2016YFB0701100)+1 种基金the"111"Project,China(No.B17020)the Program for Science and Technology Innovative Research Team of Jilin University,China.
文摘We proposed a green microwave-assisted hydrothermal way to synthesize highly crystalized N-doped carbon quantum dots(N-CQDs).The N-CQDs obtained by this microwave method have good crystalline degree(ID/IG=0.6)and a high molar ratio of N/C(11.1%)comparing with those obtained from traditional top-down method.The experimental results show that glycerine plays a key role ill the fonnation of highly crystalized N-CQDs.The as-prepared N-CQDs have good luminescent property and may be utilized as fluorescent probe to detect ions or mark cells.As the majority of N atoms in the N-CQDs were pyridinic type(64.8%),the as-prepared N-CQDs were used as a catalyst for the oxygen reduction reaction(ORR)electrocatalysis in the anode of the fuel cell(the onset potential is-0.121V),which was a 4e-transfer procedure and the catalyst showed good stability after 100 cycles.
基金Supported by the National Natural Science Foundation of China(61772379)the National Key Research and Development Program of China(2016YFB052204)
文摘Mesh morphing is a technique which gradually deforms a mesh into another one. Mesh parameterization, a powerful tool adopted to establish the one-to-one correspondence map between different meshes, is of great importance in 3 D mesh morphing. However, current parameterization methods used in mesh morphing induce large area distortion, resulting in geometric information loss. In this paper, we propose a new morphing approach for topological disk meshes based on area-preserving parameterization. Conformal mapping and M？bius transformation are computed firstly as rough alignment. Then area preserving parameterization is computed via the discrete optimal mass transport map. Features are exactly aligned through radial basis functions. A surface remeshing scheme via Delaunay refinement algorithm is developed to create a new mesh connectivity. Experimental results demonstrate that the proposed method performs well and generates high-quality morphs.
