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RBER生物降解溴酸盐及微生物群落结构分析 被引量:3
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作者 钟宇 杨麒 +6 位作者 李小明 刘湛 向仁军 文涛 成应向 尤翔宇 罗达通 《中国环境科学》 EI CAS CSSCI CSCD 北大核心 2017年第5期1945-1953,共9页
溴酸盐(BrO_3^-)是由于含溴离子(Br^-)的水体经过臭氧或加氯消毒后产生的消毒副产物,在毒理致癌性分级上被国际癌症研究机构定为II类致癌物.实验设计了一种旋转电极生物膜反应器系统(RBER),可将浓度范围为150~800μg/L的溴酸盐降解,且... 溴酸盐(BrO_3^-)是由于含溴离子(Br^-)的水体经过臭氧或加氯消毒后产生的消毒副产物,在毒理致癌性分级上被国际癌症研究机构定为II类致癌物.实验设计了一种旋转电极生物膜反应器系统(RBER),可将浓度范围为150~800μg/L的溴酸盐降解,且溴酸盐被完全还原为溴离子,没有其他中间产物生成.在反应器运行过程中发现,硝酸盐与溴酸盐对氢电子供体存在明显的竞争关系,且硝酸盐对氢电子供体竞争能力强于溴酸盐.选取反应器运行不同阶段的生物膜样品进行DNA提取和高通量测序分析微生物群落多样性.结果表明,优势菌属主要有Bacillus(枯草杆菌属)、Pseudomonas(假单胞菌属)和Lactococcus(乳球菌属)3类,其在总菌属中相对丰度占比分别为37.0%、16.2%和11.1%,可能是实现溴酸盐生物降解的主要优势菌群. 展开更多
关键词 溴酸盐 硝酸盐 高通量测序 微生物群落
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涉重酸泥硒汞提取分离技术研究 被引量:3
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作者 周霜 钟宇 +5 位作者 向仁军 赵志强 成应向 许友泽 付广义 赵媛媛 《湘潭大学学报(自然科学版)》 CAS 2020年第1期86-94,共9页
该研究采用SEM、EDS、XRD和ICP-MS等手段对涉重酸泥进行了成分分析及物相解析,结果表明,酸泥中主要元素为Pb、Se和Hg等,其主要以ClO4-、CO3-和SO42-等形式存在.该实验采用氯酸钾/盐酸浸出法对涉重酸泥中硒汞进行联合提取,探索了浸出时... 该研究采用SEM、EDS、XRD和ICP-MS等手段对涉重酸泥进行了成分分析及物相解析,结果表明,酸泥中主要元素为Pb、Se和Hg等,其主要以ClO4-、CO3-和SO42-等形式存在.该实验采用氯酸钾/盐酸浸出法对涉重酸泥中硒汞进行联合提取,探索了浸出时间、固液比、浸出温度和氯酸钾/盐酸用量等因素对硒汞浸出率的影响.结果表明,四个因素对汞的浸出率影响均较小,而温度和氯酸钾/盐酸用量对硒浸出率影响较大.该实验采用高效还原法和氧化汞焙烧法分别得到粗硒和粗汞,并在高效还原法中探讨了pH值,温度和时间对粗硒产率的影响.结果表明,粗硒产率可达34.5%以上,杂质含量低于3N标准.实验还研究了温度对氧化汞焙烧法中粗汞产率的影响.结果表明,500℃时粗汞的产率可达72.73%. 展开更多
关键词 涉重酸泥 硒汞 氯酸钾/盐酸浸出法 高效还原法 氧化焙烧法
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Study on the Removal of Ammonia Nitrogen from Wastewater Using Microwave Coupled with Active Carbon 被引量:4
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作者 Zl Pei-jian CHEN Can +2 位作者 DAI You-zhi cheng ying-xiang XIANG Ren-jun 《Meteorological and Environmental Research》 2012年第7期51-54,共4页
[ Objective] The study aimed to discuss the feasibility and optimal conditions of removing ammonia nitrogen by using microwave coupled with active carbon. [ Method ] In the study, a novel process, microwave radiation ... [ Objective] The study aimed to discuss the feasibility and optimal conditions of removing ammonia nitrogen by using microwave coupled with active carbon. [ Method ] In the study, a novel process, microwave radiation coupled with active carbon, was applied to remove ammonia nitro- gen from wastewater, and the influences of solution pH, air conditions, active carbon usage, microwave power and time on the removal effect of ammonia nitrogen were studied. [ Result] Microwave coupled with active carbon can remove ammonia nitrogen efficiently, and pumping air into the wastewater can also increase the removal rate of ammonia nitrogen to a certain extent. Higher pH, intensive microwave power and longer treating time could also increase the removal rate of ammonia nitrogen using microwave radiation coupled with active carbon, whereas the usage of active carbon contributed a small impact. It was proved that microwave coupled with active carbon was an effective method for the removal of ammonia ni- trogen from wastewater. Meanwhile, the orthogonal experiment results showed that the removal rate of ammonia nitrogen reached 92.5% under the optimal conditions, that is, the usage of active carbon was 0.5 g, pH = 11, microwave radiation power was 850 W, and microwave action time was 4 minutes. [ Conclusion] The research provided a new method to remove ammonia nitrogen from wastewater, namely microwave coupled with ac- tive carbon. 展开更多
关键词 MICROWAVE Active carbon Ammonia nitrogen Removal rate Orthogonal experiment China
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