Transparent solar cells(TSCs)are emerging devices that combine the advantages of visible transparency and light-toelectricity conversion.Currently,existing TSCs are based predominantly on organics,dyes,and perovskites...Transparent solar cells(TSCs)are emerging devices that combine the advantages of visible transparency and light-toelectricity conversion.Currently,existing TSCs are based predominantly on organics,dyes,and perovskites;however,the rigidity and color-tinted transparent nature of those devices strongly limit the utility of the resulting TSCs for realworld applications.Here,we demonstrate a flexible,color-neutral,and high-efficiency TSC based on a freestanding form of n-silicon microwires(SiMWs).Flat-tip SiMWs with controllable spacing are fabricated via deep-reactive ion etching and embedded in a freestanding transparent polymer matrix.The light transmittance can be tuned from ~10 to 55% by adjusting the spacing between the microwires.For TSCs,a heterojunction is formed with a p-type polymer in the top portion of the n-type flat-tip SiMWs.Ohmic contact with an indium-doped ZnO film occurs at the bottom,and the side surface has an Al2O3 passivation layer.Furthermore,slanted-tip SiMWs are developed by a novel solventassisted wet etching method to manipulate light absorption.Finite-difference time-domain simulation revealed that the reflected light from slanted-tip SiMWs helps light-matter interactions in adjacent microwires.The TSC based on the slanted-tip SiMWs demonstrates 8%efficiency at a visible transparency of 10% with flexibility.This efficiency is the highest among Si-based TSCs and comparable with that of state-of-the-art neutral-color TSCs based on organic–inorganic hybrid perovskite and organics.Moreover,unlike others,the stretchable and transparent platform in this study is promising for future TSCs.展开更多
A large number of different types of second-order non-Hermitian degeneracies called exceptional points(EPs)were found in various physical systems depending on the mechanism of coupling between eigenstates.We show that...A large number of different types of second-order non-Hermitian degeneracies called exceptional points(EPs)were found in various physical systems depending on the mechanism of coupling between eigenstates.We show that these EPs can be hybridized to form higher-order EPs,which preserve the original properties of the initial EPs before hybridization.For a demonstration,we hybridize chiral and supermode second-order EPs,where the former and the latter are the results of intra-disk and inter-disk mode coupling in an optical system comprised of two Mie-scale microdisks and one Rayleigh-scale scatterer.The high sensitivity of the resulting third-order EP against external perturbations in our feasible system is emphasized.展开更多
Understanding inter-site mutual mode interaction in coupled physical systems is essential to comprehend large compound systems,as this local interaction determines the successive multiple inter-site energy transfer ef...Understanding inter-site mutual mode interaction in coupled physical systems is essential to comprehend large compound systems,as this local interaction determines the successive multiple inter-site energy transfer efficiencies.In the present study,we demonstrate that only the non-Hermitian coupling can correctly account for the light transfer between two coupled optical cavities.We also reveal that the non-Hermitian coupling effect becomes crucial as the system dimension decreases.Our results provide important insight for handling general-coupled devices in the subwavelength regime.展开更多
基金supported by Mid-career Researcher Program through the National Research Foundation of Korea(NRF)grant funded by the Korea government(NRF-2018R1A2B2003720).
文摘Transparent solar cells(TSCs)are emerging devices that combine the advantages of visible transparency and light-toelectricity conversion.Currently,existing TSCs are based predominantly on organics,dyes,and perovskites;however,the rigidity and color-tinted transparent nature of those devices strongly limit the utility of the resulting TSCs for realworld applications.Here,we demonstrate a flexible,color-neutral,and high-efficiency TSC based on a freestanding form of n-silicon microwires(SiMWs).Flat-tip SiMWs with controllable spacing are fabricated via deep-reactive ion etching and embedded in a freestanding transparent polymer matrix.The light transmittance can be tuned from ~10 to 55% by adjusting the spacing between the microwires.For TSCs,a heterojunction is formed with a p-type polymer in the top portion of the n-type flat-tip SiMWs.Ohmic contact with an indium-doped ZnO film occurs at the bottom,and the side surface has an Al2O3 passivation layer.Furthermore,slanted-tip SiMWs are developed by a novel solventassisted wet etching method to manipulate light absorption.Finite-difference time-domain simulation revealed that the reflected light from slanted-tip SiMWs helps light-matter interactions in adjacent microwires.The TSC based on the slanted-tip SiMWs demonstrates 8%efficiency at a visible transparency of 10% with flexibility.This efficiency is the highest among Si-based TSCs and comparable with that of state-of-the-art neutral-color TSCs based on organic–inorganic hybrid perovskite and organics.Moreover,unlike others,the stretchable and transparent platform in this study is promising for future TSCs.
基金supported by Ministry of Health and Welfare, Republic of Korea (Government-wide R&D Fund project for infectious disease research, HG18C0069)
文摘A large number of different types of second-order non-Hermitian degeneracies called exceptional points(EPs)were found in various physical systems depending on the mechanism of coupling between eigenstates.We show that these EPs can be hybridized to form higher-order EPs,which preserve the original properties of the initial EPs before hybridization.For a demonstration,we hybridize chiral and supermode second-order EPs,where the former and the latter are the results of intra-disk and inter-disk mode coupling in an optical system comprised of two Mie-scale microdisks and one Rayleigh-scale scatterer.The high sensitivity of the resulting third-order EP against external perturbations in our feasible system is emphasized.
基金National Research Foundation of Korea(NRF)(2021R1A2C1095623)Institute for Basic Science(IBS-R024-D1).
文摘Understanding inter-site mutual mode interaction in coupled physical systems is essential to comprehend large compound systems,as this local interaction determines the successive multiple inter-site energy transfer efficiencies.In the present study,we demonstrate that only the non-Hermitian coupling can correctly account for the light transfer between two coupled optical cavities.We also reveal that the non-Hermitian coupling effect becomes crucial as the system dimension decreases.Our results provide important insight for handling general-coupled devices in the subwavelength regime.