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An observed nocturnal ozone transport event in the Sichuan Basin,Southwestern China
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作者 Ruyue Guo Guangming Shi +4 位作者 Dan Zhang Yang Chen Chao Peng chongzhi zhai Fumo Yang 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2024年第4期10-18,共9页
The ozone(O_(3))pollution in China drew lots of attention in recent years,and the Sichuan Basin(SCB)was one of the regions confronting worsening O_(3)pollution problem.Many previous studies have shown that regional tr... The ozone(O_(3))pollution in China drew lots of attention in recent years,and the Sichuan Basin(SCB)was one of the regions confronting worsening O_(3)pollution problem.Many previous studies have shown that regional transport is an important contributor to O_(3)pollution.However,very few features of the O_(3)profile during transport have been reported,especially in the border regions between different administrative divisions.In this study,we conducted tethered balloon soundings in SCB during the summer of 2020 and captured a nocturnal O_(3)transport event during the campaign.Vertically,the O_(3)transport occurred in the bottom of the residual layer,between 200 and 500 m above ground level.Horizontally,the transport pathway was directed from southeast to northwest based on the analysis of the wind field and air mass trajectories.The effect of transport in the residual layer on the surface O_(3)concentration was related to the spatial distribution of O_(3).For cities with high O_(3)concentrations in the upwind region,the transport process would bring clean air masses and abate pollution.For downwind lightly polluted cities,the transport process would slow down the decreasing or even increase the surface O_(3)concentration during the night.We provided observational facts on the profile features of a transboundary O_(3)transport event between two provincial administrative divisions,which implicated the importance of joint prevention and control measures.However,the sounding parameters were limited and the quantitative analysis was preliminary,more integrated,and thorough studies of this topic were called for in the future. 展开更多
关键词 OZONE Sichuan basin Transport event Vertical profile
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我国典型城市群O_3污染成因和关键VOCs活性解析 被引量:109
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作者 蒋美青 陆克定 +12 位作者 苏榕 谭照峰 王红丽 李莉 伏晴艳 翟崇治 谭钦文 岳玎利 陈多宏 王占山 谢绍东 曾立民 张远航 《科学通报》 EI CAS CSCD 北大核心 2018年第12期1130-1141,共12页
京津冀、长三角、珠三角和成渝地区四大城市群在夏秋季大气臭氧(O_3)污染问题严重.为了深入认识O_3的区域污染特征及其成因,在上述4个城市群于2014~2016年夏秋季节,开展了大气O_3及其前体物(氮氧化物(NOx)、挥发性有机物(VOCs))等的综... 京津冀、长三角、珠三角和成渝地区四大城市群在夏秋季大气臭氧(O_3)污染问题严重.为了深入认识O_3的区域污染特征及其成因,在上述4个城市群于2014~2016年夏秋季节,开展了大气O_3及其前体物(氮氧化物(NOx)、挥发性有机物(VOCs))等的综合观测研究.观测发现,臭氧污染区域性明显,臭氧最大8h值在59~146(10^(-9)V/V),整体上城市站点臭氧浓度水平较郊区站点低,臭氧前体物NO2平均浓度水平在4~22(10^(-9)V/V),VOCs浓度为11~53(10^(-9)V/V),VOCs活性水平在1.6~10.5s^(-1).使用基于观测的盒子模型(OBM)分析臭氧生成控制区,发现四大城市群的O_3生成多数处于人为源VOCs控制区或者过渡区,且对烯烃和芳香烃的敏感性最强.运用PMF受体模型对城市站点VOCs来源进行解析,结果表明机动车尾气排放和汽油挥发是城市VOCs主要来源,占比30%~50%;溶剂涂料使用其次,占比为10%~20%.综合而言,我国现阶段臭氧污染防控应以VOCs控制为主,其中应着重控制机动车尾气排放和溶剂涂料使用. 展开更多
关键词 臭氧 VOCS 敏感性分析 源解析 经验动力学模拟法
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Impacts of reducing air pollutants and CO_(2) emissions in urban road transport through 2035 in Chongqing, China 被引量:3
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作者 Linfeng Duan Wei Hu +5 位作者 Di Deng Weikai Fang Min Xiong Peili Lu Zhenliang Li chongzhi zhai 《Environmental Science and Ecotechnology》 2021年第4期55-66,共12页
The road transport sector in megacities is confronted with pressing local air pollution and carbon dioxide(CO_(2))control issues.To determine effective policy instruments for saving energy and the co-control of air po... The road transport sector in megacities is confronted with pressing local air pollution and carbon dioxide(CO_(2))control issues.To determine effective policy instruments for saving energy and the co-control of air pollutants and CO_(2),several mainstream measures were examined and compared in Chongqing's road transport sector from 2017 to 2035.An integration assessment framework was developed by combining the Long-range Energy Alternatives Planning(LEAP)system and a set of quantitative methods for evaluating the co-benefits of emission reductions(including the air pollutant equivalent(APeq),cocontrol coordinate system,and pollutant reduction cross-elasticity(Elsa/b)).Results showed that the shifting transportation modes scenario presented the most significant potential for energy-saving and emission reductions,reducing energy use by 30.9%and air pollutants and CO_(2) emissions by approximately 27e32%compared with the business as usual(BAU)scenario in 2035.The improving energy efficiency scenario also provided significant co-benefits for reducing air pollutants and CO_(2) emissions.Nevertheless,the promoting alternative fuel scenario may increase fine particulate matter(PM2.5)emissions by 2.2%compared to BAU in 2035 under the cleanness of regional electricity in 2017.Our findings suggest that the shifting transportation modes were effective measures to reduce air pollutants and CO_(2) in the short term synergistically,and highlighted the importance of cleaner electricity generation to develop electric vehicles in the medium and long term. 展开更多
关键词 CO-BENEFITS Air pollutants Carbon dioxide Energy consumption Road transport
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