Numerical studies on the radiation uniformity of Z-pinch dynamic hohlraum

Radiation uniformity is important for Z-pinch dynamic hohlraum driven fusion. In order to understand the radiation uniformity of Z-pinchdynamic hohlraum, the code MULTI-2D with a new developed magnetic field package is employed to investigate the related physical processeson Julong-I facility with drive current about 7e8 MA. Numerical simulations suggest that Z-pinch dynamic hohlraum with radiation temperaturemore than 100 eV can be created on Julong-I facility. Although some X-rays can escape out of the hohlraum from Z-pinch plasma and electrodes, the radiation field near the foam center is quite uniform after a transition time. For the load parameters used in this paper, the transitiontime for the thermal wave transports from r = 1 mm to r = 0 mm is about 2.0 ns. Implosion of a testing pellet driven by cylindrical dynamichohlraum shows that symmetrical implosion is hard to achieve due to the relatively slow propagation speed of thermal wave and the compressionof cylindrical shock in the foam. With the help of quasi-spherical implosion, the hohlraum radiation uniformity and corresponding pelletimplosion symmetry can be significantly improved thanks to the shape modulation of thermal wave front and shock wave front.

Hydrological assessment of TRMM rainfall data over Yangtze River Basin

High-quality rainfall information is critical for accurate simulation of runoff and water cycle processes on the land surface. In situ monitoring of rainfall has a very limited utility at the regional and global scale because of the high temporal and spatial variability of rainfall. As a step toward overcoming this problem, microwave remote sensing observations can be used to retrieve the temporal and spatial rainfall coverage because of their global availability and frequency of measurement. This paper addresses the question of whether remote sensing rainfall estimates over a catchment can be used for water balance computations in the distributed hydrological model. The TRMM 3B42V6 rainfall product was introduced into the hydrological cycle simulation of the Yangtze River Basin in South China. A tool was developed to interpolate the rain gauge observations at the same temporal and spatial resolution as the TRMM data and then evaluate the precision of TRMM 3B42V6 data from 1998 to 2006. It shows that the TRMM 3B42V6 rainfall product was reliable and had good precision in application to the Yangtze River Basin. The TRMM 3B42V6 data slightly overestimated rainfall during the wet season and underestimated rainfall during the dry season in the Yangtze River Basin. Results suggest that the TRMM 3B42V6 rainfall product can be used as an alternative data source for large-scale distributed hydrological models.

Symmetry dependent activation and reactivity of peroxysulfates on FeS_(2)(001)surface

Heterogeneous peroxysulfates-based advanced oxidation processes(AOPs)have garnered significant attention for purifying organic wastewater since they offer many advantages like low cost,safe storage,facile activation and reactive species participation[1].Nonradical and radical pathways have been proposed to be involved in peroxysulfates activation.

Arsenic retention and transport behavior in the presence of typical anionic and nonionic surfactants

The massive production and wide use of surfactants have resulted in a large amount of surfactant residuals being discharged into the environment,which could have an impact on arsenic behavior.In the present study,the influence of the anionic surfactant sodium dodecyl benzene sulfonate（SDBS） and nonionic surfactant polyethylene glycol octylphenyl ether（Triton X-100） on arsenic behavior was investigated in batch and column tests.The presence of SDBS and Triton X-100 reduced arsenic retention onto ferrihydrite（FH）,enhanced arsenic transport through FH coated sand（FH-sand） columns and promoted arsenic release from the FH surface.With coexisting surfactants in solution,the equilibrium adsorbed amount of arsenic on FH decreased by up to 29.7% and the adsorption rate decreased by up to 52.3%.Pre-coating with surfactants caused a decrease in the adsorbed amount and adsorption rate of arsenic by up to 15.1% and 58.3%,respectively.Because of the adsorption attenuation caused by surfactants,breakthrough of As（Ⅴ） and As（Ⅲ） with SDBS in columns packed with FH-sand was 23.8% and 14.3%faster than that in those without SDBS,respectively.In columns packed with SDBS-coated FH-sand,transport of arsenic was enhanced to a greater extent.Breakthrough of As（Ⅴ） and As（Ⅲ） was 52.4% and 43.8% faster and the cumulative retention amount was 44.5% and 57.3% less than that in pure FH-sand column systems,respectively.Mobilization of arsenic by surfactants increased with the increase of the initial adsorbed amount of arsenic.The cumulative release amount of As（Ⅴ） and As（Ⅲ） from the packed column reached 10.8% and 36.0%,respectively.

Mobilization of arsenic from contaminated sediment by anionic and nonionic surfactants

The increasing manufacture of surfactants and their wide application in industry, agriculture and household detergents have resulted in large amounts of surfactant residuals being discharged into water and distributed into sediment. Surfactants have the potential to enhance arsenic mobility, leading to risks to the environment and even human beings. In this study, batch and column experiments were conducted to investigate arsenic mobilization from contaminated sediment by the commercial anionic surfactants sodium dodecylbenzenesulfonate （SDBS）, sodium dodecyi sulfate （SDS）, sodium laureth sulfate （AES） and nonionic surfactants phenyl-polyethylene glycol （Triton X-100） and polyethylene glycol sorbitan monooleate （Tween-80）. The ability of surfactants to mobilize arsenic followed the order AES 〉 SDBS 〉 SDS = Triton X-100 〉 Tween 80. Arsenic mobilization by AES and Triton X-100 increased greatly with the increase of surfactant concentration and pH, while arsenic release by SDBS, SDS and Tween-80 slightly increased. The divalent ion Ca2＋ caused greater reduction of arsenic mobilization than Na＋. Sequential extraction experiments showed that the main fraction of arsenic mobilized was the specifically adsorbed fraction. Solid phase extraction showed that arsenate （As（V）） was the main species mobilized by surfactants, accounting for 65.05%-77.68% of the total mobilized arsenic. The mobilization of arsenic was positively correlated with the mobilization of iron species. The main fraction of mobilized arsenic was the dissolved fraction, accounting for 70% of total mobilized arsenic.

Aqueous stability and mobility of C_(60) complexed by sodium dodecyl benzene sulfonate surfactant

Surfactant complexation may have significant effects on the environmental behavior of nano-particles.In order to understand the ecological exposure of nano-materials,it is important to determine the stability and mobility of surfactant-complexed nano-materials in aqueous systems.In this study,the aggregation and transport of C（60） complexed by the surfactant sodium dodecyl benzene sulfonate（SDBS）were investigated.It was found that SDBS-complexed C-（60） had aζ-potential of-49.5 m V under near-neutral p H conditions and remained stable during an aging period of 15 days.It had a critical coagulation concentration of 550 mmol/L for Na Cl,which was higher than common natural colloids and many kinds of raw nano-materials,and was comparable to those of many kinds of surface-modified nano-materials.SDBS enhanced the stability of C（60） colloid;however,at the same time,it also enhanced the colloidal particle aggregation rate.Much higher mobility was found for SDBS-complexed C（60） than C（60） colloid.Increase in ionic strength,Ca^2＋ concentration or Al^（3＋） concentration decreased the mobility.In general,SDBS-complexed C（60） had high stability and mobility.