It is of great importance to explore a creative route to improve the degradation e ciency of organic pollutants in wastewater.Herein,we construct a unique hybrid system by combining self-powered triboelectric nanogene...It is of great importance to explore a creative route to improve the degradation e ciency of organic pollutants in wastewater.Herein,we construct a unique hybrid system by combining self-powered triboelectric nanogenerator(TENG)with carbon dots-TiO_(2)sheets doped three-dimensional graphene oxide photocatalyst(3 DGA@CDs-TNs),which can significantly enhance the degradation e ciency of brilliant green(BG)and direct blue 5 B(DB)owing to the powerful interaction of TENG and 3 DGA@CDs-TNs photocatalyst.The power output of TENG can be applied for wastewater purification directly,which exhibits a selfpowered electrocatalytic technology.Furthermore,the results also verify that TENG can replace conventional electric catalyst to remove pollutants e ectively from wastewater without any consumption.Subsequently,the unstable fragments and the plausible removal pathways of the two pollutants are proposed.Our work sheds light on the development of e cient and sustainable TENG/photocatalyst system,opening up new opportunities and possibilities for comprehensive utilization of random energy.展开更多
Textile-based electronic devices have attracted increasing interest in recent years due to their wearability,breathability,comfort.Among them,textile-based triboelectric nanogenerators(T-TENGs)exhibit remarkable advan...Textile-based electronic devices have attracted increasing interest in recent years due to their wearability,breathability,comfort.Among them,textile-based triboelectric nanogenerators(T-TENGs)exhibit remarkable advantages in mechanical energy harvesting and self-powered sensing.However,there are still some key challenges to the development and application of triboelectric fibers(the basic unit of T-TENG).Scalable production and large-scale integration are still significant factors hindering its application.At the same time,there are some difficulties to overcome in the manufacturing process,such as achieving good stretchability and a quick production,overcoming incompatibility between conductive and triboelectric materials.In this study,triboelectric fibers are produced continuously by one-step coaxial wet spinning.They are only 0.18 mm in diameter and consist of liquid metal(LM)core and polyurethane(PU)sheath.Due to the good mechanical properties between them,there is no interface incompatibility of the triboelectric fibers.In addition,triboelectric fibers can be made into large areas of T-TENG by means of digital embroidery and plain weave.The T-TENGs can be used for energy harvesting and self-powered sensing.When they are fixed on the forearm can monitor various strokes in badminton.This work provides a promising strategy for the large-scale fabrication and large-area integration of triboelectric fibers,promotes the development of wearable T-TENGs.展开更多
Wearable electronics are advancing towards miniaturization and flexibility.However,traditional energy supply methods have largely hindered their development.An effective solution to this problem is to convert human me...Wearable electronics are advancing towards miniaturization and flexibility.However,traditional energy supply methods have largely hindered their development.An effective solution to this problem is to convert human mechanical energy into electricity to power wearable electronic devices.Therefore,it is greatly attractive to design flexible,foldable and even stretchable energy harvesting devices.Herein,we use the electrospinning and kirigami approach to develop a type of highly stretchable kirigami-patterned nanofiber-based triboelectric nanogenerator(K-TENG).Due to its innovative structural design,the K-TENG can achieve a tensile strain of 220%,independent of the tensile properties of the material itself.When a person swings their arms,the K-TENG fixed to the clothing can convert mechanical energy from human movement into electrical energy.The produced electricity can directly drive 50 LED lights and a digital watch,or be stored in a lithium battery to charge the smartwatch and smartphone,respectively.This study employs a new method to fabricate a stretchable triboelectric nanogenerator and demonstrates its promising applications in wearable power technology.展开更多
With increasing work pressure in modern society,prolonged sedentary positions with poor sitting postures can cause physical and psychological problems,including obesity,muscular disorders,and myopia.In this paper,we p...With increasing work pressure in modern society,prolonged sedentary positions with poor sitting postures can cause physical and psychological problems,including obesity,muscular disorders,and myopia.In this paper,we present a self-powered sitting position monitoring vest(SPMV)based on triboelectric nanogenerators(TENGs)to achieve accurate real-time posture recognition through an integrated machine learning algorithm.The SPMV achieves high sensitivity(0.16 mV/Pa),favorable stretchability(10%),good stability(12,000 cycles),and machine washability(10 h)by employing knitted double threads interlaced with conductive fiber and nylon yarn.Utilizing a knitted structure and sensor arrays that are stitched into different parts of the clothing,the SPMV offers a non-invasive method of recognizing different sitting postures,providing feedback,and warning users while enhancing long-term wearing comfortability.It achieves a posture recognition accuracy of 96.6%using the random forest classifier,which is higher than the logistic regression(95.5%)and decision tree(94.3%)classifiers.The TENG-based SPMV offers a reliable solution in the healthcare system for non-invasive and long-term monitoring,promoting the development of triboelectric-based wearable electronics.展开更多
The rapid development of wearable electronics requires its energy supply part to be flexible,wearable,integratable and sustainable.However,some of the energy supply units cannot meet these requirements at the same tim...The rapid development of wearable electronics requires its energy supply part to be flexible,wearable,integratable and sustainable.However,some of the energy supply units cannot meet these requirements at the same time,and there is also a capacity limitation of the energy storage units,and the development of sustainable wearable self-charging power supplies is crucial.Here,we report a wearable sustainable energy harvesting-storage hybrid self-charging power textile.The power textile consists of a coaxial fiber-shaped polylactic acid/reduced graphene oxide/polypyrrole(PLA-rGO-PPy)triboelectric nanogenerator(fiber-TENG)that can harvest low-frequency and irregular energy during human motion as a power generation unit,and a novel coaxial fiber-shaped supercapacitor(fiber-SC)prepared by functionalized loading of a wet-spinning graphene oxide fiber as an energy storage unit.The fiber-TENG is flexible,knittable,wearable and adaptable for integration with various portable electronics.The coaxial fiber-SC has high volumetric energy density and good cycling stability.The fiber-TENG and fiber-SC are flexible yarn structures for wearable continuous human movement energy harvesting and storage as on-body self-charging power systems,with light-weight,ease of preparation,great portability and wide applicability.The integrated power textile can provide an efficient route for sustainable working of wearable electronics.展开更多
Currently,the gradual depletion of fossil resources and the large amount of plastic waste are causing serious harm to the land and marine ecology.The rapid development of wearable smart fibers is accompanied by rapid ...Currently,the gradual depletion of fossil resources and the large amount of plastic waste are causing serious harm to the land and marine ecology.The rapid development of wearable smart fibers is accompanied by rapid growth in the material demand for fibers,and the development of green and high-performance biomass-based fibers has become an important research topic to reduce the dependence on synthetic fiber materials and the harm to the environment.Here,chitosan is first prepared from the waste material by chemical methods.Then the chitosan-based self-powered induction fibers are prepared by electrospinning core wire technique.Chitosan-based self-powered sensing fiber is ultra-light and flexible,which can achieve about 2500 collisions without damaging the surface.Chitosan-based self-powered sensing fiber can also be used in smart home sensing applications to control home appliance switches with a light touch,which has a great application prospect in smart home and wearable fields.展开更多
The importance ofocean exploration and underwater monitoring is becoming vital,due to the abundant biological,mineral energy,and other resources in the ocean.Here,a self-powered underwater cable-based triboelectric na...The importance ofocean exploration and underwater monitoring is becoming vital,due to the abundant biological,mineral energy,and other resources in the ocean.Here,a self-powered underwater cable-based triboelectric nanogenerator(TENG)is demonstrated for underwater monitoring of mechanical motion/triggering as wllas searching and rescuing inthe sea.Using a novel double-layer winding method combined with ferroelectric polarization,a self-powered cable-structured sensor with a stable electrical output has been manufactured,which can accurately respond to a variety of external mechanical stimuli.A self-powered cable sensing network woven using smart cables can comprehensively transmit information,such as the plane osition anddivedhofasumersbeMorereiely,can analyzeitsdrtionfmovemnt,seedand pathaong w transmiting information such as the submersible's size and momentum.The developed self-powered sensor based on the cable-based TENG not only has low cost and simple structure but also exhibits working accuracy and stability.Finally,the proposed work provides new ideas for future seabed exploration and ocean monitoring.展开更多
基金financially supported by the National Key R&D Program of China(Grant Nos.2016YFA0202704 and 2019YFA0706900)the Beijing Municipal Natural Science Foundation(Grant No.2212052)+1 种基金the China Postdoctoral Science Foundation(Grant No.2019T120390)the Jiangsu Planned Projects for Postdoctoral research funds(Grant No.2018K018A)。
文摘It is of great importance to explore a creative route to improve the degradation e ciency of organic pollutants in wastewater.Herein,we construct a unique hybrid system by combining self-powered triboelectric nanogenerator(TENG)with carbon dots-TiO_(2)sheets doped three-dimensional graphene oxide photocatalyst(3 DGA@CDs-TNs),which can significantly enhance the degradation e ciency of brilliant green(BG)and direct blue 5 B(DB)owing to the powerful interaction of TENG and 3 DGA@CDs-TNs photocatalyst.The power output of TENG can be applied for wastewater purification directly,which exhibits a selfpowered electrocatalytic technology.Furthermore,the results also verify that TENG can replace conventional electric catalyst to remove pollutants e ectively from wastewater without any consumption.Subsequently,the unstable fragments and the plausible removal pathways of the two pollutants are proposed.Our work sheds light on the development of e cient and sustainable TENG/photocatalyst system,opening up new opportunities and possibilities for comprehensive utilization of random energy.
基金the National Natural Science Foundation of China(No.22109012)Natural Science Foundation of the Beijing Municipality(Nos.L222037 and 2212052)the Fundamental Research Funds for the Central Universities(No.E1E46805).
文摘Textile-based electronic devices have attracted increasing interest in recent years due to their wearability,breathability,comfort.Among them,textile-based triboelectric nanogenerators(T-TENGs)exhibit remarkable advantages in mechanical energy harvesting and self-powered sensing.However,there are still some key challenges to the development and application of triboelectric fibers(the basic unit of T-TENG).Scalable production and large-scale integration are still significant factors hindering its application.At the same time,there are some difficulties to overcome in the manufacturing process,such as achieving good stretchability and a quick production,overcoming incompatibility between conductive and triboelectric materials.In this study,triboelectric fibers are produced continuously by one-step coaxial wet spinning.They are only 0.18 mm in diameter and consist of liquid metal(LM)core and polyurethane(PU)sheath.Due to the good mechanical properties between them,there is no interface incompatibility of the triboelectric fibers.In addition,triboelectric fibers can be made into large areas of T-TENG by means of digital embroidery and plain weave.The T-TENGs can be used for energy harvesting and self-powered sensing.When they are fixed on the forearm can monitor various strokes in badminton.This work provides a promising strategy for the large-scale fabrication and large-area integration of triboelectric fibers,promotes the development of wearable T-TENGs.
基金the China Postdoctoral Science Foundation(Grant No.2023TQ0316)the National Natural Science Foundation of China(Grant No.52273046).
文摘Wearable electronics are advancing towards miniaturization and flexibility.However,traditional energy supply methods have largely hindered their development.An effective solution to this problem is to convert human mechanical energy into electricity to power wearable electronic devices.Therefore,it is greatly attractive to design flexible,foldable and even stretchable energy harvesting devices.Herein,we use the electrospinning and kirigami approach to develop a type of highly stretchable kirigami-patterned nanofiber-based triboelectric nanogenerator(K-TENG).Due to its innovative structural design,the K-TENG can achieve a tensile strain of 220%,independent of the tensile properties of the material itself.When a person swings their arms,the K-TENG fixed to the clothing can convert mechanical energy from human movement into electrical energy.The produced electricity can directly drive 50 LED lights and a digital watch,or be stored in a lithium battery to charge the smartwatch and smartphone,respectively.This study employs a new method to fabricate a stretchable triboelectric nanogenerator and demonstrates its promising applications in wearable power technology.
基金the National Key R&D Program of China(No.2021YFA1201601)the National Natural Science Foundation of China(No.22109012)+1 种基金Natural Science Foundation of Beijing(No.2212052)the Fundamental Research Funds for the Central Universities(No.E1E46805).
文摘With increasing work pressure in modern society,prolonged sedentary positions with poor sitting postures can cause physical and psychological problems,including obesity,muscular disorders,and myopia.In this paper,we present a self-powered sitting position monitoring vest(SPMV)based on triboelectric nanogenerators(TENGs)to achieve accurate real-time posture recognition through an integrated machine learning algorithm.The SPMV achieves high sensitivity(0.16 mV/Pa),favorable stretchability(10%),good stability(12,000 cycles),and machine washability(10 h)by employing knitted double threads interlaced with conductive fiber and nylon yarn.Utilizing a knitted structure and sensor arrays that are stitched into different parts of the clothing,the SPMV offers a non-invasive method of recognizing different sitting postures,providing feedback,and warning users while enhancing long-term wearing comfortability.It achieves a posture recognition accuracy of 96.6%using the random forest classifier,which is higher than the logistic regression(95.5%)and decision tree(94.3%)classifiers.The TENG-based SPMV offers a reliable solution in the healthcare system for non-invasive and long-term monitoring,promoting the development of triboelectric-based wearable electronics.
基金The authors are grateful for the support received from the National Natural Science Foundation of China(No.22109012)Natural Science Foundation of the Beijing Municipality(Nos.2212052 and L222037)the Fundamental Research Funds for the Central Universities(No.E1E46805).
文摘The rapid development of wearable electronics requires its energy supply part to be flexible,wearable,integratable and sustainable.However,some of the energy supply units cannot meet these requirements at the same time,and there is also a capacity limitation of the energy storage units,and the development of sustainable wearable self-charging power supplies is crucial.Here,we report a wearable sustainable energy harvesting-storage hybrid self-charging power textile.The power textile consists of a coaxial fiber-shaped polylactic acid/reduced graphene oxide/polypyrrole(PLA-rGO-PPy)triboelectric nanogenerator(fiber-TENG)that can harvest low-frequency and irregular energy during human motion as a power generation unit,and a novel coaxial fiber-shaped supercapacitor(fiber-SC)prepared by functionalized loading of a wet-spinning graphene oxide fiber as an energy storage unit.The fiber-TENG is flexible,knittable,wearable and adaptable for integration with various portable electronics.The coaxial fiber-SC has high volumetric energy density and good cycling stability.The fiber-TENG and fiber-SC are flexible yarn structures for wearable continuous human movement energy harvesting and storage as on-body self-charging power systems,with light-weight,ease of preparation,great portability and wide applicability.The integrated power textile can provide an efficient route for sustainable working of wearable electronics.
基金The authors are grateful for the support received from National Natural Science Foundation of China(Grant No.22109012)Natural Science Foundation of the Beijing Municipality(Grant No.2212052)the Fundamental Research Funds for the Central Universities(Grant No.E1E46805).
文摘Currently,the gradual depletion of fossil resources and the large amount of plastic waste are causing serious harm to the land and marine ecology.The rapid development of wearable smart fibers is accompanied by rapid growth in the material demand for fibers,and the development of green and high-performance biomass-based fibers has become an important research topic to reduce the dependence on synthetic fiber materials and the harm to the environment.Here,chitosan is first prepared from the waste material by chemical methods.Then the chitosan-based self-powered induction fibers are prepared by electrospinning core wire technique.Chitosan-based self-powered sensing fiber is ultra-light and flexible,which can achieve about 2500 collisions without damaging the surface.Chitosan-based self-powered sensing fiber can also be used in smart home sensing applications to control home appliance switches with a light touch,which has a great application prospect in smart home and wearable fields.
基金support received from the National Key R&D Project from Minister of Science and Technology(Grant no.2021YFA1201601)National Natural Science Foundation of China(Grant no.22109012)+1 种基金the Beijing Municipal Natural Science Foundation(Grant no.22i2052)and the Fundamental Research Funds for the Central Universities(Grant no.E1E46805).
文摘The importance ofocean exploration and underwater monitoring is becoming vital,due to the abundant biological,mineral energy,and other resources in the ocean.Here,a self-powered underwater cable-based triboelectric nanogenerator(TENG)is demonstrated for underwater monitoring of mechanical motion/triggering as wllas searching and rescuing inthe sea.Using a novel double-layer winding method combined with ferroelectric polarization,a self-powered cable-structured sensor with a stable electrical output has been manufactured,which can accurately respond to a variety of external mechanical stimuli.A self-powered cable sensing network woven using smart cables can comprehensively transmit information,such as the plane osition anddivedhofasumersbeMorereiely,can analyzeitsdrtionfmovemnt,seedand pathaong w transmiting information such as the submersible's size and momentum.The developed self-powered sensor based on the cable-based TENG not only has low cost and simple structure but also exhibits working accuracy and stability.Finally,the proposed work provides new ideas for future seabed exploration and ocean monitoring.