CO_(2)emission inventory provides fundamental data for climate research and emission mitigation.Currently,most global CO_(2)emission inventories were developed with energy statistics from International Energy Agency(I...CO_(2)emission inventory provides fundamental data for climate research and emission mitigation.Currently,most global CO_(2)emission inventories were developed with energy statistics from International Energy Agency(IEA)and were available at country level with limited source categories.Here,as the first step toward a high-resolution and dynamic updated global CO_(2)emission database,we developed a data-driven approach to construct seamless and highly-resolved energy consumption data cubes for 208 countries/territories,797 sub-country administrative divisions in 29 countries,42 fuel types,and 52 sectors,with the fusion of activity data from 24 international statistics and 65 regional/local statistics.Global CO_(2)emissions from fossil fuel combustion and cement production in 1970–2021 were then estimated with highly-resolved source category(1,484 of total)and sub-country information(797 of total).Specifically,73%of global CO_(2)emissions in 2021 were estimated with sub-country information,providing considerably improved spatial resolution for global CO_(2)emission accounting.With the support of detailed information,the dynamics of global CO_(2)emissions across sectors and fuel types were presented,representing the evolution of global economy and progress of climate mitigation.Remarkable differences of sectoral contribution were found across sub-country administrative divisions within a given country,revealing the uneven distribution of energy and economic structure among different regions.Our estimates were generally consistent with existing databases at aggregated level for global total or large emitters,while large discrepancies were observed for middle and small emitters.Our database,named the Multiresolution Emission Inventory model for Climate and air pollution research(MEIC)is publicly available through http://meicmodel.org.cn with highly-resolved information and timely update,which provides an independent carbon emission accounting data source for climate research.展开更多
Nitrogen oxides(NOx),significant contributors to air pollution and climate change,form aerosols and ozone in the atmosphere.Accurate,timely,and transparent information on NOx emissions is essential for decision-making...Nitrogen oxides(NOx),significant contributors to air pollution and climate change,form aerosols and ozone in the atmosphere.Accurate,timely,and transparent information on NOx emissions is essential for decision-making to mitigate both haze and ozone pollution.However,a comprehensive understanding of the trends and drivers behind anthropogenic NOx emissions from Chinadthe world's largest emitterdhas been lacking since 2020 due to delays in emissions reporting.Here we show a consistent decline in China's NOx emissions from 2020 to 2022,despite increased fossil fuel consumption,utilizing satellite observations as constraints for NOx emission estimates through atmospheric inversion.This reduction is corroborated by data from two independent spaceborne instruments:the TROPOspheric Monitoring Instrument(TROPOMI)and the Ozone Monitoring Instrument(OMI).Notably,a reduction in transport emissions,largely due to the COVID-19 lockdowns,slightly decreased China's NOx emissions in 2020.In subsequent years,2021 and 2022,reductions in NOx emissions were driven by the industry and transport sectors,influenced by stringent air pollution controls.The satellite-based inversion system developed in this study represents a significant advancement in the real-time monitoring of regional air pollution emissions from space.展开更多
Single and joint toxic effects of polycyclic musks including 1,3,4,6,7,8-hexahydro-4,6,6,7,8,8-hexamethylcyclopenta[g]-2- benzopyran (HHCB) and 7-acetyl-1,1,3,4,4,6-hexamethyl-1,2,3,4-tetrahydronapthalene (AHTN) a...Single and joint toxic effects of polycyclic musks including 1,3,4,6,7,8-hexahydro-4,6,6,7,8,8-hexamethylcyclopenta[g]-2- benzopyran (HHCB) and 7-acetyl-1,1,3,4,4,6-hexamethyl-1,2,3,4-tetrahydronapthalene (AHTN) and cadmium (Cd) on seed germination and seedling growth of wheat (Triticum aestivum) were investigated. The results showed that the toxicity sequence of HHCB toxic to wheat seed germination and seedling growth was similar to that of AHTN, that is, germination rate 〉 shoot elongation 〉 root elongation, while the toxicity of Cd was in the sequence of root elongation 〉 shoot elongation 〉 germination rate, according to the LC50 and EC50 values. It is suggested that polycyclic musks and Cd had different toxicological mechanisms. Root and shoot elongation of wheat might be good bioindicators for the contamination of polycyclic musks and Cd in soil. The mixture of polycyclic musks and Cd had synergistic effects on T. aestivum according to the equi-toxic mixture approach when root elongation was selected as the toxicological endpoint. Thus, the joint toxicity of HHCB and Cd was significantly higher than the single toxicity of HHCB or Cd, which was also confirmed by the EC50mix value of the mixture (EC50mix = 0.530 TUrnix). The EC50mix value of the mixture of AHTN and Cd was 0.614 TUmix, which indicated that the mixture toxicity was strengthened when AHTN coexisted with Cd.展开更多
基金supported by the National Natural Science Foundation of China(Grant No.41921005)the Major Project of High Resolution Earth Observation System(Grant No.30Y60B01-9003-22/23)+1 种基金the New Cornerstone Science Foundation through the XPLORER PRIZEthe Tsinghua University Initiative Scientific Research Program(Grant No.20223080041)。
文摘CO_(2)emission inventory provides fundamental data for climate research and emission mitigation.Currently,most global CO_(2)emission inventories were developed with energy statistics from International Energy Agency(IEA)and were available at country level with limited source categories.Here,as the first step toward a high-resolution and dynamic updated global CO_(2)emission database,we developed a data-driven approach to construct seamless and highly-resolved energy consumption data cubes for 208 countries/territories,797 sub-country administrative divisions in 29 countries,42 fuel types,and 52 sectors,with the fusion of activity data from 24 international statistics and 65 regional/local statistics.Global CO_(2)emissions from fossil fuel combustion and cement production in 1970–2021 were then estimated with highly-resolved source category(1,484 of total)and sub-country information(797 of total).Specifically,73%of global CO_(2)emissions in 2021 were estimated with sub-country information,providing considerably improved spatial resolution for global CO_(2)emission accounting.With the support of detailed information,the dynamics of global CO_(2)emissions across sectors and fuel types were presented,representing the evolution of global economy and progress of climate mitigation.Remarkable differences of sectoral contribution were found across sub-country administrative divisions within a given country,revealing the uneven distribution of energy and economic structure among different regions.Our estimates were generally consistent with existing databases at aggregated level for global total or large emitters,while large discrepancies were observed for middle and small emitters.Our database,named the Multiresolution Emission Inventory model for Climate and air pollution research(MEIC)is publicly available through http://meicmodel.org.cn with highly-resolved information and timely update,which provides an independent carbon emission accounting data source for climate research.
基金supported by the National Key R&D Program of China(Grant No.2021YFB3901000)the National Natural Science Foundation of China(Grant No.42105094)the Shenzhen Science,Technology and Innovation Commission(Grant No.WDZC20220810110301001).
文摘Nitrogen oxides(NOx),significant contributors to air pollution and climate change,form aerosols and ozone in the atmosphere.Accurate,timely,and transparent information on NOx emissions is essential for decision-making to mitigate both haze and ozone pollution.However,a comprehensive understanding of the trends and drivers behind anthropogenic NOx emissions from Chinadthe world's largest emitterdhas been lacking since 2020 due to delays in emissions reporting.Here we show a consistent decline in China's NOx emissions from 2020 to 2022,despite increased fossil fuel consumption,utilizing satellite observations as constraints for NOx emission estimates through atmospheric inversion.This reduction is corroborated by data from two independent spaceborne instruments:the TROPOspheric Monitoring Instrument(TROPOMI)and the Ozone Monitoring Instrument(OMI).Notably,a reduction in transport emissions,largely due to the COVID-19 lockdowns,slightly decreased China's NOx emissions in 2020.In subsequent years,2021 and 2022,reductions in NOx emissions were driven by the industry and transport sectors,influenced by stringent air pollution controls.The satellite-based inversion system developed in this study represents a significant advancement in the real-time monitoring of regional air pollution emissions from space.
基金supported by the National Natural Science Foundation of China(No. 20777040)the Ministry of Education of China(No. 707011)
文摘Single and joint toxic effects of polycyclic musks including 1,3,4,6,7,8-hexahydro-4,6,6,7,8,8-hexamethylcyclopenta[g]-2- benzopyran (HHCB) and 7-acetyl-1,1,3,4,4,6-hexamethyl-1,2,3,4-tetrahydronapthalene (AHTN) and cadmium (Cd) on seed germination and seedling growth of wheat (Triticum aestivum) were investigated. The results showed that the toxicity sequence of HHCB toxic to wheat seed germination and seedling growth was similar to that of AHTN, that is, germination rate 〉 shoot elongation 〉 root elongation, while the toxicity of Cd was in the sequence of root elongation 〉 shoot elongation 〉 germination rate, according to the LC50 and EC50 values. It is suggested that polycyclic musks and Cd had different toxicological mechanisms. Root and shoot elongation of wheat might be good bioindicators for the contamination of polycyclic musks and Cd in soil. The mixture of polycyclic musks and Cd had synergistic effects on T. aestivum according to the equi-toxic mixture approach when root elongation was selected as the toxicological endpoint. Thus, the joint toxicity of HHCB and Cd was significantly higher than the single toxicity of HHCB or Cd, which was also confirmed by the EC50mix value of the mixture (EC50mix = 0.530 TUrnix). The EC50mix value of the mixture of AHTN and Cd was 0.614 TUmix, which indicated that the mixture toxicity was strengthened when AHTN coexisted with Cd.