Gas breakthrough pressure is a key parameter to evaluate the sealing capacity of caprock,and it also plays important roles in safety and capacity of CO_(2)geological storage.Based on the published experimental results...Gas breakthrough pressure is a key parameter to evaluate the sealing capacity of caprock,and it also plays important roles in safety and capacity of CO_(2)geological storage.Based on the published experimental results,we present numerical simulations on CO_(2)breakthrough pressure in unsaturated low-permeability rock under 9 multiple P-T conditions(which can keep CO_(2)in gaseous,liquid and supercritical states)and thus,a numerical method which can be used to accurately predict CO_(2)breakthrough pressure on rock-core scale is proposed.The simulation results show that CO_(2)breakthrough pressure and breakthrough time are exponential correlated with P-T conditions.Meanwhile,pressure has stronger effects on experimental results than that of temperature.Moreover,we performed sensitivity studies on the pore distribution indexλ(0.6,0.7,0.8,and 0.9)in van Genuchten-Muale model.Results show that with the increase ofλ,CO_(2)breakthrough pressure and breakthrough time both show decreasing trends.In other words,the larger the value ofλis,the better the permeability of the caprock is,and the worse the CO_(2)sealing capacity is.The numerical method established in this study can provide an important reference for the prediction of gas breakthrough pressure on rock-core scale and for related numerical studies.展开更多
碳捕集与封存(Carbon Capture and Storage,CCS)技术作为缓解全球气候变暖、减少CO_(2)排放的有效路径之一,其潜力评估至关重要。目前CCS技术主要包括CO_(2)强化石油(天然气)开采封存技术、CO_(2)驱替煤层气封存技术以及咸水层CO_(2)封...碳捕集与封存(Carbon Capture and Storage,CCS)技术作为缓解全球气候变暖、减少CO_(2)排放的有效路径之一,其潜力评估至关重要。目前CCS技术主要包括CO_(2)强化石油(天然气)开采封存技术、CO_(2)驱替煤层气封存技术以及咸水层CO_(2)封存技术3类。各类封存技术利用了不同的封存机制,其潜力评估方法也略有差别。油气藏封存和咸水层封存主要利用了构造圈闭储存、束缚空间储存、溶解储存、矿化储存等封存机制,煤层气封存主要利用了吸附封存机制。国内外学者和机构针对各类封存技术提出了相应的计算方法,依据其计算原理可归纳为4类物质平衡封存量计算法、有效容积封存量计算法、溶解机制封存量计算法以及考虑多种捕获机制的综合封存量计算法。通过对各类经典方法及其计算原理进行综述,剖析潜力封存量计算方法的内涵原理和应用场景,分析了CO_(2)地质封存潜力评价方法在实际应用中面临的问题,有助于提升我国的CCS潜力评价质量。展开更多
From 2010 to 2012, the China Geological Survey Center for Hydrogeology and Environmental Geology Survey （CHEGS） carried out the project ＂Potential evaluation and demonstration project of CO2 Geological Storage in C...From 2010 to 2012, the China Geological Survey Center for Hydrogeology and Environmental Geology Survey （CHEGS） carried out the project ＂Potential evaluation and demonstration project of CO2 Geological Storage in China＂. During this project, we developed an evaluation index system and technical methods for the potential and suitability of CO2 geological storage based on China＇s geological conditions, and evaluated the potential and suitability of the primary basins for COz geological storage, in order to draw a series of regional scale maps （at a scale of 1：5000000） and develop an atlas of the main sedimentary basins in China. By using these tools, we delineated many potential targets for CO2 storage. We also built techniques and methods for site selection and the exploration and assessment of CO2 geological storage in deep saline aquifers. Furthermore, through cooperation with the China Shenhua Coal to Liquid and Chemical Co., Ltd., we successfully constructed the first coal-based demonstration project for CO2 geological storage in deep saline aquifers in the Yijinhuoluo Banner of Ordos in the Inner Mongolia Autonomous Region, which brought about the basic preliminary theories, techniques, and methods of geological CO2 storage in deep saline aquifers under China＇s geological conditions.展开更多
基金supported by Open Research Fund of State Key Laboratory of Geomechanics and Geotechnical Engineering,Institute of Rock and Soil Mechanics,Chinese Academy of Sciences(Grant No.SKLGME021010)funded by the National Natural Science Foundation of China(Grant No.41702251 and 42141010)the MOE Key Laboratory of Groundwater Circulation and Environmental Evolution。
文摘Gas breakthrough pressure is a key parameter to evaluate the sealing capacity of caprock,and it also plays important roles in safety and capacity of CO_(2)geological storage.Based on the published experimental results,we present numerical simulations on CO_(2)breakthrough pressure in unsaturated low-permeability rock under 9 multiple P-T conditions(which can keep CO_(2)in gaseous,liquid and supercritical states)and thus,a numerical method which can be used to accurately predict CO_(2)breakthrough pressure on rock-core scale is proposed.The simulation results show that CO_(2)breakthrough pressure and breakthrough time are exponential correlated with P-T conditions.Meanwhile,pressure has stronger effects on experimental results than that of temperature.Moreover,we performed sensitivity studies on the pore distribution indexλ(0.6,0.7,0.8,and 0.9)in van Genuchten-Muale model.Results show that with the increase ofλ,CO_(2)breakthrough pressure and breakthrough time both show decreasing trends.In other words,the larger the value ofλis,the better the permeability of the caprock is,and the worse the CO_(2)sealing capacity is.The numerical method established in this study can provide an important reference for the prediction of gas breakthrough pressure on rock-core scale and for related numerical studies.
文摘碳捕集与封存(Carbon Capture and Storage,CCS)技术作为缓解全球气候变暖、减少CO_(2)排放的有效路径之一,其潜力评估至关重要。目前CCS技术主要包括CO_(2)强化石油(天然气)开采封存技术、CO_(2)驱替煤层气封存技术以及咸水层CO_(2)封存技术3类。各类封存技术利用了不同的封存机制,其潜力评估方法也略有差别。油气藏封存和咸水层封存主要利用了构造圈闭储存、束缚空间储存、溶解储存、矿化储存等封存机制,煤层气封存主要利用了吸附封存机制。国内外学者和机构针对各类封存技术提出了相应的计算方法,依据其计算原理可归纳为4类物质平衡封存量计算法、有效容积封存量计算法、溶解机制封存量计算法以及考虑多种捕获机制的综合封存量计算法。通过对各类经典方法及其计算原理进行综述,剖析潜力封存量计算方法的内涵原理和应用场景,分析了CO_(2)地质封存潜力评价方法在实际应用中面临的问题,有助于提升我国的CCS潜力评价质量。
文摘From 2010 to 2012, the China Geological Survey Center for Hydrogeology and Environmental Geology Survey （CHEGS） carried out the project ＂Potential evaluation and demonstration project of CO2 Geological Storage in China＂. During this project, we developed an evaluation index system and technical methods for the potential and suitability of CO2 geological storage based on China＇s geological conditions, and evaluated the potential and suitability of the primary basins for COz geological storage, in order to draw a series of regional scale maps （at a scale of 1：5000000） and develop an atlas of the main sedimentary basins in China. By using these tools, we delineated many potential targets for CO2 storage. We also built techniques and methods for site selection and the exploration and assessment of CO2 geological storage in deep saline aquifers. Furthermore, through cooperation with the China Shenhua Coal to Liquid and Chemical Co., Ltd., we successfully constructed the first coal-based demonstration project for CO2 geological storage in deep saline aquifers in the Yijinhuoluo Banner of Ordos in the Inner Mongolia Autonomous Region, which brought about the basic preliminary theories, techniques, and methods of geological CO2 storage in deep saline aquifers under China＇s geological conditions.
