Coherent combination of laser beam is an important and challenging area of high power laser science. And how to evaluate the high power laser by coherent beam combination is a new research spot. Formulas for the radia...Coherent combination of laser beam is an important and challenging area of high power laser science. And how to evaluate the high power laser by coherent beam combination is a new research spot. Formulas for the radiated intensity distributions of coherent combined Gaussian beam array are derived via Fraunhofer scalar diffraction model by utilizing representations of the cross-spectral density of the far field. Effects of beam array numbers and separate distances etc. on far field radiated profiles are shown and analyzed. A new conception named power in the bucket of the main lobe (PIMm) is advanced to measure the beam quality of combined beams. This evaluation method is useful for efficiently determining the peak irradiance and power in the bucket for single emitting apertures of general shape.展开更多
Excited-states play a crucial role in the optical absorption and luminescence of solids and hence their accurate information is highly desired. Herein, we attempt to seize the excited-states information of Mn^(4+)ions...Excited-states play a crucial role in the optical absorption and luminescence of solids and hence their accurate information is highly desired. Herein, we attempt to seize the excited-states information of Mn^(4+)ions in K_(2)SiF_(6) microcrystals via measuring and calculating their variable-temperature photoluminescence excitation(PLE) spectra. At cryogenic temperatures, an unpredicted splitting of the high-excited-state is observed. Moreover, the two-split high-excited-state levels are further revealed to primarily couple with the two hyperfine split modes of quasi-localized ν2 vibration in the distorted Mn-F_(6) octahedral configuration,whereas the coupling strengths are found to be substantially different from each other. The slightly split vibrational mode is firmly supported by the low-temperature Raman spectra. Jahn-Teller lattice distortion is believed to be responsible for the observed splitting of the electronic high-excited-state and the quasi-localized vibrational mode.展开更多
Radiative cooling without energy consumption and environmental pollution holds great promise as the next-generation cooling technology.To date,daytime radiative cooling performance is still slightly low,especially in ...Radiative cooling without energy consumption and environmental pollution holds great promise as the next-generation cooling technology.To date,daytime radiative cooling performance is still slightly low,especially in humid areas.In this work,we demonstrated that nanoporous polyethylene(Nano PE)film can improve solar reflectivity from 96%to 99%,thus boosting radiative cooling performance.Moreover,the experimental results in humid areas indicate that Nano PE films can improve radiative cooling performance by∼76%in a clear day and 120%in a day with few clouds.Additionally,compared with ordinary PE films,thin Nano PE films have significantly higher weather fastness and mechanical strength.More importantly,nano PE films can scatter part of visible light,thus suppressing the generation of light pollution in practical applications.Lastly,the modeling results reveal that with Nano PE films,more than 95%of China’s areas can achieve daytime cooling performance.Our work can boost the development of radiative cooling technology with a very low cost.展开更多
文摘Coherent combination of laser beam is an important and challenging area of high power laser science. And how to evaluate the high power laser by coherent beam combination is a new research spot. Formulas for the radiated intensity distributions of coherent combined Gaussian beam array are derived via Fraunhofer scalar diffraction model by utilizing representations of the cross-spectral density of the far field. Effects of beam array numbers and separate distances etc. on far field radiated profiles are shown and analyzed. A new conception named power in the bucket of the main lobe (PIMm) is advanced to measure the beam quality of combined beams. This evaluation method is useful for efficiently determining the peak irradiance and power in the bucket for single emitting apertures of general shape.
基金supported by the National Natural Science Foundation of China (Grant Nos. 12074324, and 11374247)the Science, Technology, and Innovation Commission of Shenzhen Municipality (Grant Nos. JCJY20180508163404043, and JCYJ20170818141709893)。
文摘Excited-states play a crucial role in the optical absorption and luminescence of solids and hence their accurate information is highly desired. Herein, we attempt to seize the excited-states information of Mn^(4+)ions in K_(2)SiF_(6) microcrystals via measuring and calculating their variable-temperature photoluminescence excitation(PLE) spectra. At cryogenic temperatures, an unpredicted splitting of the high-excited-state is observed. Moreover, the two-split high-excited-state levels are further revealed to primarily couple with the two hyperfine split modes of quasi-localized ν2 vibration in the distorted Mn-F_(6) octahedral configuration,whereas the coupling strengths are found to be substantially different from each other. The slightly split vibrational mode is firmly supported by the low-temperature Raman spectra. Jahn-Teller lattice distortion is believed to be responsible for the observed splitting of the electronic high-excited-state and the quasi-localized vibrational mode.
基金financially supported by the National Natural Science Foundation of China(12074324 and 11374247)the Science,Technology,and Innovation Commission of Shenzhen Municipality(JCJY20180508163404043 and JCYJ20170818141709893)。
基金This work was supported by National Engineering Laboratory for Digital Construction and Evaluation Technology of Urban Rail Tran-sit(No.2021HJ01)Tianjin University Innovation Project(No.2020YJSB087).
文摘Radiative cooling without energy consumption and environmental pollution holds great promise as the next-generation cooling technology.To date,daytime radiative cooling performance is still slightly low,especially in humid areas.In this work,we demonstrated that nanoporous polyethylene(Nano PE)film can improve solar reflectivity from 96%to 99%,thus boosting radiative cooling performance.Moreover,the experimental results in humid areas indicate that Nano PE films can improve radiative cooling performance by∼76%in a clear day and 120%in a day with few clouds.Additionally,compared with ordinary PE films,thin Nano PE films have significantly higher weather fastness and mechanical strength.More importantly,nano PE films can scatter part of visible light,thus suppressing the generation of light pollution in practical applications.Lastly,the modeling results reveal that with Nano PE films,more than 95%of China’s areas can achieve daytime cooling performance.Our work can boost the development of radiative cooling technology with a very low cost.
