Assessment of harmful impacts and risks of air pollution in case of accidents as well as of long lasting exposition is an important challenge of chemical transport modeling. Sad confirmation of this statement unexpect...Assessment of harmful impacts and risks of air pollution in case of accidents as well as of long lasting exposition is an important challenge of chemical transport modeling. Sad confirmation of this statement unexpectedly has come from the nuclear power plant accident in Fukushima which occurred while this paper was finalized. Two strategies to comply with the task of impact and risk assessment in extended regions like Central Europe or the Balkans are described. The first one is characterized by application of a single model system to an extended domain. The other one is based on the combined application of several chemical transport models designed for the use in various sub-domains in the region under consideration. Advantages and disadvantages exist for both approaches. For instance, the single model strategy allows unified and harmonized assessment of risks in a larger region, whereas the combined model strategy may pro-vide faster and locally more specific response in emergency cases. The single model approach is treated exploiting applications of the EURAD model system. The combined model approach is a novel way of joint use of chemical transport model systems developed for the Balkans. The models are described and the accuracy of simulations carried out with them is briefly demonstrated by comparison of simulated and observed concentrations of air pollutants. Applications regarding the search of sources for high pollution events and the assessment of risks through known sources are exem-plarily discussed.展开更多
The spatial distribution, radiative forcing, and climatic effects of tropospheric ozone in China during summer were investigated by using the regional climate model Reg CM4. The results revealed that the tropospheric ...The spatial distribution, radiative forcing, and climatic effects of tropospheric ozone in China during summer were investigated by using the regional climate model Reg CM4. The results revealed that the tropospheric ozone column concentration was high in East China, Central China, North China, and the Sichuan basin during summer. The increase in tropospheric ozone levels since the industrialization era produced clear-sky shortwave and clear-sky longwave radiative forcing of 0.18 and 0.71 W m^(–2), respectively, which increased the average surface air temperature by 0.06 K and the average precipitation by 0.22 mm day^(–1) over eastern China during summer. In addition, tropospheric ozone increased the land–sea thermal contrast, leading to an enhancement of East Asian summer monsoon circulation over southern China and a weakening over northern China. The notable increase in surface air temperature in northwestern China, East China, and North China could be attributed to the absorption of longwave radiation by ozone, negative cloud amount anomaly, and corresponding positive shortwave radiation anomaly. There was a substantial increase in precipitation in the middle and lower reaches of the Yangtze River. It was related to the enhanced upward motion and the increased water vapor brought by strengthened southerly winds in the lower troposphere.展开更多
文摘Assessment of harmful impacts and risks of air pollution in case of accidents as well as of long lasting exposition is an important challenge of chemical transport modeling. Sad confirmation of this statement unexpectedly has come from the nuclear power plant accident in Fukushima which occurred while this paper was finalized. Two strategies to comply with the task of impact and risk assessment in extended regions like Central Europe or the Balkans are described. The first one is characterized by application of a single model system to an extended domain. The other one is based on the combined application of several chemical transport models designed for the use in various sub-domains in the region under consideration. Advantages and disadvantages exist for both approaches. For instance, the single model strategy allows unified and harmonized assessment of risks in a larger region, whereas the combined model strategy may pro-vide faster and locally more specific response in emergency cases. The single model approach is treated exploiting applications of the EURAD model system. The combined model approach is a novel way of joint use of chemical transport model systems developed for the Balkans. The models are described and the accuracy of simulations carried out with them is briefly demonstrated by comparison of simulated and observed concentrations of air pollutants. Applications regarding the search of sources for high pollution events and the assessment of risks through known sources are exem-plarily discussed.
基金Supported by the National Key Research and Development Plan of China(2016YFC0203303)National(Key)Basic Research and Development(973)Program of China(2014CB441203)+1 种基金National Natural Science Foundation of China(91544230,41621005,41575145,and 41205109)REgional climate–air QUAlity interactions(REQUA)project of Marie Curie Actions International Research Staff Exchange Scheme(IRSES)under the 7th Framework Programme of the European Community(PIRSES-GA-2013-612671)
文摘The spatial distribution, radiative forcing, and climatic effects of tropospheric ozone in China during summer were investigated by using the regional climate model Reg CM4. The results revealed that the tropospheric ozone column concentration was high in East China, Central China, North China, and the Sichuan basin during summer. The increase in tropospheric ozone levels since the industrialization era produced clear-sky shortwave and clear-sky longwave radiative forcing of 0.18 and 0.71 W m^(–2), respectively, which increased the average surface air temperature by 0.06 K and the average precipitation by 0.22 mm day^(–1) over eastern China during summer. In addition, tropospheric ozone increased the land–sea thermal contrast, leading to an enhancement of East Asian summer monsoon circulation over southern China and a weakening over northern China. The notable increase in surface air temperature in northwestern China, East China, and North China could be attributed to the absorption of longwave radiation by ozone, negative cloud amount anomaly, and corresponding positive shortwave radiation anomaly. There was a substantial increase in precipitation in the middle and lower reaches of the Yangtze River. It was related to the enhanced upward motion and the increased water vapor brought by strengthened southerly winds in the lower troposphere.