Since the invention of optical tweezers,optical manipulation has advanced significantly in scientific areas such as atomic physics,optics and biological science.Especially in the past decade,numerous optical beams and...Since the invention of optical tweezers,optical manipulation has advanced significantly in scientific areas such as atomic physics,optics and biological science.Especially in the past decade,numerous optical beams and nanoscale devices have been proposed to mechanically act on nanoparticles in increasingly precise,stable and flexible ways.Both the linear and angular momenta of light can be exploited to produce optical tractor beams,tweezers and optical torque from the microscale to the nanoscale.Research on optical forces helps to reveal the nature of light–matter interactions and to resolve the fundamental aspects,which require an appropriate description of momenta and the forces on objects in matter.In this review,starting from basic theories and computational approaches,we highlight the latest optical trapping configurations and their applications in bioscience,as well as recent advances down to the nanoscale.Finally,we discuss the future prospects of nanomanipulation,which has considerable potential applications in a variety of scientific fields and everyday life.展开更多
The determination of optical force as a consequence of momentum transfer is inevitably subject to the use of the proper momentum density and stress tensor.It is imperative and valuable to consider the intrinsic scheme...The determination of optical force as a consequence of momentum transfer is inevitably subject to the use of the proper momentum density and stress tensor.It is imperative and valuable to consider the intrinsic scheme of photon momentum transfer,particularly when a particle is embedded in a complex dielectric environment.Typically,we consider a particle submerged in an inhomogeneous background composed of different dielectric materials,excluding coherent illumination or hydrodynamic effects.A ray-tracing method is adopted to capture the direct process of momentum transfer from the complex background medium,and this approach is validated using the modified Einstein–Laub method,which uses only the interior fields of the particle in the calculation.In this way,debates regarding the calculation of the force with different stress tensors using exterior fields can be avoided.Our suggested interpretation supports only the Minkowski approach for the optical momentum transfer to the embedded scatterer while rejecting Peierls’s and Abraham’s approaches,though the momentum of a stably moving photon in a continuous background medium should be considered to be of the Abraham type.Our interpretation also provides a novel method of realizing a tractor beam for the exertion of negative force that offers an alternative to the use of negative-index materials,optical gain,or highly non-paraxial or multiple-light interference.展开更多
Bismuth oxides are important battery materials owing to their ability to electrochemically react and alloy with Li,which results in a high capacity level,which substantially exceeds that of graphite anodes.However,thi...Bismuth oxides are important battery materials owing to their ability to electrochemically react and alloy with Li,which results in a high capacity level,which substantially exceeds that of graphite anodes.However,this high Li-storage capability is often compromised by the poor electrochemical cyclability and rate capability of bismuth oxides.To address these challenges,in this study,we design a hybrid architecture composed of reduced graphene oxide (rGO) nanosheets decorated with ultrafine Bi2O2.33 nanodots (denoted as Bi2O2.33/rGO),based on the selective and controlled hydrolysis of a Bi precursor on graphene oxide and subsequent crystallization via solvothermal treatment.Because of its high conductivity,large accessible area,and inherent flexibility,the Bi2O2.33/rGO hybrid exhibits stable and robust Li storage (346 mA·h·g-1 over 600 cycles at 10 C),significantly outperforming previously reported Bi-based materials.This superb performance indicates that decorating rGO nanosheets with ultrafine nanodots may introduce new possibilities for the development of stable and robust metal-oxide electrodes.展开更多
In this work, we present a multi-channel nonreciprocal waveguide, which is composed of a gyrotropic-bounded dielectric on the bottom and a plasmonic material on the top. The Lorentz reciprocity in the time-invariant s...In this work, we present a multi-channel nonreciprocal waveguide, which is composed of a gyrotropic-bounded dielectric on the bottom and a plasmonic material on the top. The Lorentz reciprocity in the time-invariant system is broken when applying an external static magnetic field on the gyrotropic material. The nonreciprocal emission from the dipole source located in the center of the waveguide is observed in extended waveband channels. The proposed heterostructure serves as a photonic dichroism once the dielectric is replaced by a nonlinear material.The associated second harmonic generated in the nonlinear process can be separated from the fundamental signal under proper magnetic field intensity. Our findings may provide significant guidance for designing nonreciprocal photonic devices with superiorities of a tunable waveband, multiple channels, and small footprint.展开更多
基金support from the National University of Singapore(no.R-263-000-678-133)supported by the Spanish MINECO grants FIS2012-36113-C03-03,FIS2014-55563-REDC and FIS2015-69295-C3-1-P+2 种基金support from the National Natural Science Foundation of China(no.11504252)the Natural Science Foundation for the Youth of Jiangsu Province(no.BK20150306)the Natural Science Foundation for Colleges and Universities in Jiangsu Province of China(no.15KJB140008).
文摘Since the invention of optical tweezers,optical manipulation has advanced significantly in scientific areas such as atomic physics,optics and biological science.Especially in the past decade,numerous optical beams and nanoscale devices have been proposed to mechanically act on nanoparticles in increasingly precise,stable and flexible ways.Both the linear and angular momenta of light can be exploited to produce optical tractor beams,tweezers and optical torque from the microscale to the nanoscale.Research on optical forces helps to reveal the nature of light–matter interactions and to resolve the fundamental aspects,which require an appropriate description of momenta and the forces on objects in matter.In this review,starting from basic theories and computational approaches,we highlight the latest optical trapping configurations and their applications in bioscience,as well as recent advances down to the nanoscale.Finally,we discuss the future prospects of nanomanipulation,which has considerable potential applications in a variety of scientific fields and everyday life.
基金CWQ acknowledges financial support from the National University of Singapore(Grant No.R-263-000-678-133)ZW acknowledges support from the Packard Fellowship in Science and Engineering and the Alfred P.Sloan Research Fellowship.CWQ and WD contributed equally。
文摘The determination of optical force as a consequence of momentum transfer is inevitably subject to the use of the proper momentum density and stress tensor.It is imperative and valuable to consider the intrinsic scheme of photon momentum transfer,particularly when a particle is embedded in a complex dielectric environment.Typically,we consider a particle submerged in an inhomogeneous background composed of different dielectric materials,excluding coherent illumination or hydrodynamic effects.A ray-tracing method is adopted to capture the direct process of momentum transfer from the complex background medium,and this approach is validated using the modified Einstein–Laub method,which uses only the interior fields of the particle in the calculation.In this way,debates regarding the calculation of the force with different stress tensors using exterior fields can be avoided.Our suggested interpretation supports only the Minkowski approach for the optical momentum transfer to the embedded scatterer while rejecting Peierls’s and Abraham’s approaches,though the momentum of a stably moving photon in a continuous background medium should be considered to be of the Abraham type.Our interpretation also provides a novel method of realizing a tractor beam for the exertion of negative force that offers an alternative to the use of negative-index materials,optical gain,or highly non-paraxial or multiple-light interference.
基金We acknowledge the financial support of the National Natural Science Foundation of China (Nos. 51672182 and 51302181), the Natural Science Foundation of Jiangsu Province (No. BK20151219), and the Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD).
文摘Bismuth oxides are important battery materials owing to their ability to electrochemically react and alloy with Li,which results in a high capacity level,which substantially exceeds that of graphite anodes.However,this high Li-storage capability is often compromised by the poor electrochemical cyclability and rate capability of bismuth oxides.To address these challenges,in this study,we design a hybrid architecture composed of reduced graphene oxide (rGO) nanosheets decorated with ultrafine Bi2O2.33 nanodots (denoted as Bi2O2.33/rGO),based on the selective and controlled hydrolysis of a Bi precursor on graphene oxide and subsequent crystallization via solvothermal treatment.Because of its high conductivity,large accessible area,and inherent flexibility,the Bi2O2.33/rGO hybrid exhibits stable and robust Li storage (346 mA·h·g-1 over 600 cycles at 10 C),significantly outperforming previously reported Bi-based materials.This superb performance indicates that decorating rGO nanosheets with ultrafine nanodots may introduce new possibilities for the development of stable and robust metal-oxide electrodes.
基金National Natural Science Foundation of China(NSFC)(11504252,61701246)Natural Science Research of Jiangsu Higher Education Institutions of China(17KJB140014)+3 种基金Natural Science Foundation of Jiangsu Province(BK20150306)China Postdoctoral Science Foundation(2018M630596)Priority Academic Program Development of Jiangsu Higher Education InstitutionsMinistry of Education-Singapore(MOE)(2017-T1-001-239(RG91/17(S)),MOE2015-T2-1-145)
文摘In this work, we present a multi-channel nonreciprocal waveguide, which is composed of a gyrotropic-bounded dielectric on the bottom and a plasmonic material on the top. The Lorentz reciprocity in the time-invariant system is broken when applying an external static magnetic field on the gyrotropic material. The nonreciprocal emission from the dipole source located in the center of the waveguide is observed in extended waveband channels. The proposed heterostructure serves as a photonic dichroism once the dielectric is replaced by a nonlinear material.The associated second harmonic generated in the nonlinear process can be separated from the fundamental signal under proper magnetic field intensity. Our findings may provide significant guidance for designing nonreciprocal photonic devices with superiorities of a tunable waveband, multiple channels, and small footprint.