Growth dynamics of epitaxiai (Ba, Sr)TiO3 thin films deposited at different temperatures on SrRuO3/SrTiO3 substrates by pulsed laser deposition is investigated by transmission electron microscopy. The films exhibit ...Growth dynamics of epitaxiai (Ba, Sr)TiO3 thin films deposited at different temperatures on SrRuO3/SrTiO3 substrates by pulsed laser deposition is investigated by transmission electron microscopy. The films exhibit a layered structure comprising sublayers with distinctive features in regard to the remaining strain, density of misfit dislocations and/or lattice defects, and growth habit. We correlate these temperature-dependent features with the predominant misfit-strain relaxation mechanisms for each one of the detected growth regimes. The thickness dependence of the film structure is discussed within the framework of the predictions for a kineticaily modified Stranski-Krastanov growth mode.展开更多
基金Supported by the National Natural Science Foundation of China and the Spanish Education and Science Ministry under the Ramón y Cajal Programme.
文摘Growth dynamics of epitaxiai (Ba, Sr)TiO3 thin films deposited at different temperatures on SrRuO3/SrTiO3 substrates by pulsed laser deposition is investigated by transmission electron microscopy. The films exhibit a layered structure comprising sublayers with distinctive features in regard to the remaining strain, density of misfit dislocations and/or lattice defects, and growth habit. We correlate these temperature-dependent features with the predominant misfit-strain relaxation mechanisms for each one of the detected growth regimes. The thickness dependence of the film structure is discussed within the framework of the predictions for a kineticaily modified Stranski-Krastanov growth mode.