同步硝化反硝化(simultaneous nitrification and denitrification,SND)是一种节能型废水处理工艺,但C/N对SBR系统SND及活性污泥微生物种群的影响机理尚不清楚。本试验以人工模拟废水为研究对象,采用4组不同碳氮比(C/N)系统(R_(0)、R_(5...同步硝化反硝化(simultaneous nitrification and denitrification,SND)是一种节能型废水处理工艺,但C/N对SBR系统SND及活性污泥微生物种群的影响机理尚不清楚。本试验以人工模拟废水为研究对象,采用4组不同碳氮比(C/N)系统(R_(0)、R_(5)、R_(10)和R_(15))对比分析了C/N对SBR系统SND及活性污泥微生物种群的影响,并通过高通量测序测定了SBR活性污泥系统微生物多样性。结果表明,C/N与SND效能的实现及提高显著正相关,随着C/N的升高,SBR系统SND率(19.2%→25.7%→35.0%→74.0%)和SND反应速率[(16.1→21.4→30.2→57.2)mg·(gSS·d)^(–)]显著升高,且R_(10)和R_(15)系统分别在第215和120周期后,SND对总氮去除贡献率达到63.7%和89%。高通量测序结果表明,门水平微生物具有较高的多样性,达到19门,主要包括变形菌门(55.10%),拟杆菌门(17.40%),蓝细菌门(7.90%),疣微菌门(5.00%)和硝化螺旋菌门(2.80%),其中变形门是优势菌种,并且属水平上也具有较高的多样性,数量达到112种以上,其中动胶菌属为优势菌属,且R_(0)系统内硝化螺旋菌属的相对丰度是R_(5)、R_(10)和R_(15)的106倍。此外,SBR活性污泥系统中包含反硝化菌的门和属主要由变形门、拟杆菌门和厚壁菌门中的22个菌属所组成。展开更多
The water-energy nexus has garnered worldwide interest.Current dual-functional research aimed at coproducing freshwater and electricity faces significant challenges,including sub-optimal capacities("1+1<2"...The water-energy nexus has garnered worldwide interest.Current dual-functional research aimed at coproducing freshwater and electricity faces significant challenges,including sub-optimal capacities("1+1<2"),poor inter-functional coordination,high carbon footprints,and large costs.Mainstream water-toelectricity conversions are often compromised owing to functionality separation and erratic gradients.Herein,we present a sustainable strategy based on renewable biomass that addresses these issues by jointly achieving competitive solar-evaporative desalination and robust clean electricity generation.Using hydrothermally activated basswood,our solar desalination exceeded the 100% efficiency bottleneck even under reduced solar illumination.Through simple size-tuning,we achieved a high evaporation rate of 3.56 kg h^(-1)m^(-2)and an efficiency of 149.1%,representing 128%-251% of recent values without sophisticated surface engineering.By incorporating an electron-ion nexus with interfacial Faradaic electron circulation and co-ion-predominated micro-tunnel hydrodynamic flow,we leveraged free energy from evaporation to generate long-term electricity(0.38 W m^(-3)for over 14 d),approximately 322% of peer performance levels.This inter-functional nexus strengthened dual functionalities and validated general engineering practices.Our presented strategy holds significant promise for global human–society–environment sustainability.展开更多
文摘同步硝化反硝化(simultaneous nitrification and denitrification,SND)是一种节能型废水处理工艺,但C/N对SBR系统SND及活性污泥微生物种群的影响机理尚不清楚。本试验以人工模拟废水为研究对象,采用4组不同碳氮比(C/N)系统(R_(0)、R_(5)、R_(10)和R_(15))对比分析了C/N对SBR系统SND及活性污泥微生物种群的影响,并通过高通量测序测定了SBR活性污泥系统微生物多样性。结果表明,C/N与SND效能的实现及提高显著正相关,随着C/N的升高,SBR系统SND率(19.2%→25.7%→35.0%→74.0%)和SND反应速率[(16.1→21.4→30.2→57.2)mg·(gSS·d)^(–)]显著升高,且R_(10)和R_(15)系统分别在第215和120周期后,SND对总氮去除贡献率达到63.7%和89%。高通量测序结果表明,门水平微生物具有较高的多样性,达到19门,主要包括变形菌门(55.10%),拟杆菌门(17.40%),蓝细菌门(7.90%),疣微菌门(5.00%)和硝化螺旋菌门(2.80%),其中变形门是优势菌种,并且属水平上也具有较高的多样性,数量达到112种以上,其中动胶菌属为优势菌属,且R_(0)系统内硝化螺旋菌属的相对丰度是R_(5)、R_(10)和R_(15)的106倍。此外,SBR活性污泥系统中包含反硝化菌的门和属主要由变形门、拟杆菌门和厚壁菌门中的22个菌属所组成。
基金supported by the National Natural Science Foundation of China(U21A20162 and 52261145701)the 2115 Talent Development Program of China Agricultural University。
文摘The water-energy nexus has garnered worldwide interest.Current dual-functional research aimed at coproducing freshwater and electricity faces significant challenges,including sub-optimal capacities("1+1<2"),poor inter-functional coordination,high carbon footprints,and large costs.Mainstream water-toelectricity conversions are often compromised owing to functionality separation and erratic gradients.Herein,we present a sustainable strategy based on renewable biomass that addresses these issues by jointly achieving competitive solar-evaporative desalination and robust clean electricity generation.Using hydrothermally activated basswood,our solar desalination exceeded the 100% efficiency bottleneck even under reduced solar illumination.Through simple size-tuning,we achieved a high evaporation rate of 3.56 kg h^(-1)m^(-2)and an efficiency of 149.1%,representing 128%-251% of recent values without sophisticated surface engineering.By incorporating an electron-ion nexus with interfacial Faradaic electron circulation and co-ion-predominated micro-tunnel hydrodynamic flow,we leveraged free energy from evaporation to generate long-term electricity(0.38 W m^(-3)for over 14 d),approximately 322% of peer performance levels.This inter-functional nexus strengthened dual functionalities and validated general engineering practices.Our presented strategy holds significant promise for global human–society–environment sustainability.
