Submerged arc plasma technology was assessed for the removal of phenols from wastewater.The OH radicals generated from the boundary between the plasma and waste solution were considered as a significant factor on the ...Submerged arc plasma technology was assessed for the removal of phenols from wastewater.The OH radicals generated from the boundary between the plasma and waste solution were considered as a significant factor on the degradation reaction.In this study,the effects of highly energetic electrons released from the submerged arc plasma were mainly studied.The highly energetic electrons directly broke the strong chemical bond and locally increased the reaction temperatures in solution.The effects of the submerged-arc plasma on the decomposition of phenol are discussed in terms of the input energy and initial concentration.The single use of submerged arc plasma easily decomposed the phenol but did not increase the mineralization efficiency.Therefore,the submerged arc plasma,coupled with the ozone injection,was investigated.The submerged arc plasma combined with ozone injection had a synergic effect,which led to significant improvements in mineralization with only a small increase in input energy.The decomposition mechanism of phenol by the submerged arc plasma with the ozone was analyzed.展开更多
基金the Korea Institute of Energy Technology Evaluation and Planning(KETEP)and the Ministry of Trade,Industry&Energy(MOTIE)of the Republic of Korea(No.20194030202340)the Basic Science Research Program through the National Research Foundation of Korea(NRF)grant funded by the Korea government(MSIT)(No.2019R1A2C1006816).
文摘Submerged arc plasma technology was assessed for the removal of phenols from wastewater.The OH radicals generated from the boundary between the plasma and waste solution were considered as a significant factor on the degradation reaction.In this study,the effects of highly energetic electrons released from the submerged arc plasma were mainly studied.The highly energetic electrons directly broke the strong chemical bond and locally increased the reaction temperatures in solution.The effects of the submerged-arc plasma on the decomposition of phenol are discussed in terms of the input energy and initial concentration.The single use of submerged arc plasma easily decomposed the phenol but did not increase the mineralization efficiency.Therefore,the submerged arc plasma,coupled with the ozone injection,was investigated.The submerged arc plasma combined with ozone injection had a synergic effect,which led to significant improvements in mineralization with only a small increase in input energy.The decomposition mechanism of phenol by the submerged arc plasma with the ozone was analyzed.
