High-quality narrow bandgap semiconductors nanowires(NWs)challenge the flexible near-infrared(NIR)photodetectors in next-generation imaging,data communication,environmental monitoring,and bioimaging applications.In th...High-quality narrow bandgap semiconductors nanowires(NWs)challenge the flexible near-infrared(NIR)photodetectors in next-generation imaging,data communication,environmental monitoring,and bioimaging applications.In this work,complementary metal oxide semiconductor-compatible metal of Ag is deposited on glass as the growth catalyst for the surfactantassisted chemical vapor deposition of GaSb NWs.The uniform morphology,balance stoichiometry,high-quality crystallinity,and phase purity of as-prepared NWs are checked by scanning electron microscopy,energy dispersive X-ray spectroscopy,high-resolution transmission electron microscopy,and X-ray diffraction.The electrical properties of as-prepared NWs are studied by constructing back-gated field-effect-transistors,displaying a high I_(on)/I_(off) ratio of 10^(4) and high peak hole mobility of 400 cm^(2)/(V·s).Benefiting from the excellent electrical and mechanical flexibility properties,the as-fabricated NW flexible NIR photodetector exhibits high sensitivity and excellent photoresponse,with responsivity as high as 618 A/W and detectivity as high as 6.7×10^(10) Jones.Furthermore,there is no obvious decline in NIR photodetection behavior,even after parallel and perpendicular folding with 1200 cycles.展开更多
During the past decades, glacier mass loss is becoming increasingly significant worldwide but knowledge about the acceleration is still limited despite its potentially profound impacts on sea level rise, water resourc...During the past decades, glacier mass loss is becoming increasingly significant worldwide but knowledge about the acceleration is still limited despite its potentially profound impacts on sea level rise, water resources availability and glacial hazards. In this study, we analyzed the acceleration of glacier mass loss based on in-situ measurements and on the latest compilation dataset of direct and geodetic observations for the period 1961–2016. The results showed that the rate of glacier mass loss has increased worldwide during the past decades. At the global scale, the rate of glacier mass loss has been accelerating at 5.76±1.35 Gt a-2 as well as 0.0074±0.0016 m w.e.a-2 on mass balance(refer to the area-averaged mass change value) during the whole period. At regional scales, for mass change rate, the heavily glacierized regions excluding Antarctic and Subantarctic exhibited a larger acceleration compared to other regions. The highest acceleration of mass change was found in Alaska glaciers(1.33±0.47 Gt a-2) over the full period. As for mass balance, high acceleration occurred on the regions with small glaciers as well as on the heavily glacierized regions. Central Europe exhibited the highest acceleration(0.024±0.0088 m w.e.a-2) during 1961–2016. High level of consistency between the acceleration and temperature implies that climate warming had a significant effect on the accelerating of glacier mass loss. Moreover, acceleration of the contribution from the Greenland ice sheet(0.028 to0.070 mm a-2) and Antarctic ice sheet(0.023 to 0.058 mm a-2) to sea level rise exceeds acceleration of the contribution from global glaciers(0.019±0.013 mm a-2). These results will improve our understanding of the glacier retreat in response to climate change and provide critical information for improving mitigation strategies for impacts that may be caused by glacier melting.展开更多
Perovskite/MoS2hybrid thin film transistor photodetectors consist of few-layered MoS2and CH3NH3PbI3film with various thickness prepared by two-step vacuum deposition.By implementing perovskite CH3NH3PbI3film onto the ...Perovskite/MoS2hybrid thin film transistor photodetectors consist of few-layered MoS2and CH3NH3PbI3film with various thickness prepared by two-step vacuum deposition.By implementing perovskite CH3NH3PbI3film onto the MoS2flake,the perovskite/MoS2hybrid photodetector exhibited a photoresponsivity of 104A/W and fast response time of about 40 ms.Improvement of photodetection performance is attributed to the balance between light absorption in the perovskite layer and an effective transfer of photogenerated carriers from perovskite entering the MoS2channel.This work may provide guidance to develop high-performance hybrid structure optoelectronic devices.展开更多
基金the National Key R&D Program of China (No.2017YFA0305500)National Natural Science Foundation of China (Nos.61904096,11504207)+3 种基金Taishan Scholars Program of Shandong Province (No.tsqn201812006)Shandong Univ ersity Youth Innovation Supporting Program (No.2019-KJN020)Shandong University Multidisciplinary Research and Innovation Team of Young Scholars (No.2020QNQT015)“Outstanding youth scholar and Qilu young scholar” programs of Shandong University.
文摘High-quality narrow bandgap semiconductors nanowires(NWs)challenge the flexible near-infrared(NIR)photodetectors in next-generation imaging,data communication,environmental monitoring,and bioimaging applications.In this work,complementary metal oxide semiconductor-compatible metal of Ag is deposited on glass as the growth catalyst for the surfactantassisted chemical vapor deposition of GaSb NWs.The uniform morphology,balance stoichiometry,high-quality crystallinity,and phase purity of as-prepared NWs are checked by scanning electron microscopy,energy dispersive X-ray spectroscopy,high-resolution transmission electron microscopy,and X-ray diffraction.The electrical properties of as-prepared NWs are studied by constructing back-gated field-effect-transistors,displaying a high I_(on)/I_(off) ratio of 10^(4) and high peak hole mobility of 400 cm^(2)/(V·s).Benefiting from the excellent electrical and mechanical flexibility properties,the as-fabricated NW flexible NIR photodetector exhibits high sensitivity and excellent photoresponse,with responsivity as high as 618 A/W and detectivity as high as 6.7×10^(10) Jones.Furthermore,there is no obvious decline in NIR photodetection behavior,even after parallel and perpendicular folding with 1200 cycles.
基金supported by the Strategic Priority Research Program of the Chinese Academy of Sciences (Grant No. XDA19070501)the National Natural Science Foundation of China (Grant Nos. 41730751, 41671066, 41871059 & 41871055)。
文摘During the past decades, glacier mass loss is becoming increasingly significant worldwide but knowledge about the acceleration is still limited despite its potentially profound impacts on sea level rise, water resources availability and glacial hazards. In this study, we analyzed the acceleration of glacier mass loss based on in-situ measurements and on the latest compilation dataset of direct and geodetic observations for the period 1961–2016. The results showed that the rate of glacier mass loss has increased worldwide during the past decades. At the global scale, the rate of glacier mass loss has been accelerating at 5.76±1.35 Gt a-2 as well as 0.0074±0.0016 m w.e.a-2 on mass balance(refer to the area-averaged mass change value) during the whole period. At regional scales, for mass change rate, the heavily glacierized regions excluding Antarctic and Subantarctic exhibited a larger acceleration compared to other regions. The highest acceleration of mass change was found in Alaska glaciers(1.33±0.47 Gt a-2) over the full period. As for mass balance, high acceleration occurred on the regions with small glaciers as well as on the heavily glacierized regions. Central Europe exhibited the highest acceleration(0.024±0.0088 m w.e.a-2) during 1961–2016. High level of consistency between the acceleration and temperature implies that climate warming had a significant effect on the accelerating of glacier mass loss. Moreover, acceleration of the contribution from the Greenland ice sheet(0.028 to0.070 mm a-2) and Antarctic ice sheet(0.023 to 0.058 mm a-2) to sea level rise exceeds acceleration of the contribution from global glaciers(0.019±0.013 mm a-2). These results will improve our understanding of the glacier retreat in response to climate change and provide critical information for improving mitigation strategies for impacts that may be caused by glacier melting.
基金Project supported by the National Natural Science Foundation of China(Nos.11374070,61327009 214320051)the Strategic Priority Research Program of the Chinese Academy of Sciences(No.XDA09040201)
文摘Perovskite/MoS2hybrid thin film transistor photodetectors consist of few-layered MoS2and CH3NH3PbI3film with various thickness prepared by two-step vacuum deposition.By implementing perovskite CH3NH3PbI3film onto the MoS2flake,the perovskite/MoS2hybrid photodetector exhibited a photoresponsivity of 104A/W and fast response time of about 40 ms.Improvement of photodetection performance is attributed to the balance between light absorption in the perovskite layer and an effective transfer of photogenerated carriers from perovskite entering the MoS2channel.This work may provide guidance to develop high-performance hybrid structure optoelectronic devices.
