NiFe layered double hydroxides(NiFe LDHs)have been intensively developed for the oxygen evolution reaction(OER)in alkaline media;however,their unsatisfactory hydrogen evolution reaction(HER)performance limits their pr...NiFe layered double hydroxides(NiFe LDHs)have been intensively developed for the oxygen evolution reaction(OER)in alkaline media;however,their unsatisfactory hydrogen evolution reaction(HER)performance limits their practical application in overall water splitting.Herein,a simple and efficient one-step electrodeposition method is used to accomplish in situ growth of NiFe LDHsNiFe alloy gradient hybrid coatings on a carbon cloth(CC).Within the binder-free electrode,NiFe LDHs nanosheets with a low-crystalline nature exhibit highly active bifunctional OER/HER activities,and the NiFe alloy acts as a stable electron highway and strong skeleton bridge between NiFe LDHs and the CC.When the electrodes are simultaneously employed as the cathode and anode for overall water splitting,they require low cell potentials of 1.441 V at10 mA·cm^(-2)and 1.703 V at 100 mA·cm^(-2),respectively,and they demonstrate outstanding stability at a current density greater than 100 mA·cm^(-2)for more than 100 h.This is one of the best bifunctional OER and HER catalysts for overall water splitting.Both lattice defects and surface reconstructions crucially contribute to the bifunctional OER/HER activities of NiFe LDHs.This simple and scalable synthesis approach presents an intriguing paradigm for industrial production,and the fabricated electrode has potential application in high-current-density water splitting.展开更多
Existing tracking algorithms often suffer from the drift and lost problems caused by factors such as pose variation, illumination change, occlusion and motion. Therefore, developing a robust and effective tracker is s...Existing tracking algorithms often suffer from the drift and lost problems caused by factors such as pose variation, illumination change, occlusion and motion. Therefore, developing a robust and effective tracker is still a challenging task. In this paper, we propose a real-time compressive tracking based on online Hough forest. The gray and texture features of discrete samples are extracted and compressed via the random measurement matrix. Online Hough forest classifier is used to vote the location probability of the target, and it optimizes the confidence map estimation for the target detection. The location of target being tracked is determined by combining the upper frame of the target center location and the probability confidence map of the incremental Hough forest. Finally, the classifier parameters are updated online by introducing the illumination variation and target occlusion feedback mechanism adaptively. The experiments with state-of-the-art algorithms on challenging sequences demonstrated that the proposed algorithm can effectively enhance the robustness and accuracy, and inherit the real-time performance of the compressive tracking algorithm.展开更多
基金financially supported by the Fundamental Research Funds for the Central Universities,JLU(No.45122031B004)。
文摘NiFe layered double hydroxides(NiFe LDHs)have been intensively developed for the oxygen evolution reaction(OER)in alkaline media;however,their unsatisfactory hydrogen evolution reaction(HER)performance limits their practical application in overall water splitting.Herein,a simple and efficient one-step electrodeposition method is used to accomplish in situ growth of NiFe LDHsNiFe alloy gradient hybrid coatings on a carbon cloth(CC).Within the binder-free electrode,NiFe LDHs nanosheets with a low-crystalline nature exhibit highly active bifunctional OER/HER activities,and the NiFe alloy acts as a stable electron highway and strong skeleton bridge between NiFe LDHs and the CC.When the electrodes are simultaneously employed as the cathode and anode for overall water splitting,they require low cell potentials of 1.441 V at10 mA·cm^(-2)and 1.703 V at 100 mA·cm^(-2),respectively,and they demonstrate outstanding stability at a current density greater than 100 mA·cm^(-2)for more than 100 h.This is one of the best bifunctional OER and HER catalysts for overall water splitting.Both lattice defects and surface reconstructions crucially contribute to the bifunctional OER/HER activities of NiFe LDHs.This simple and scalable synthesis approach presents an intriguing paradigm for industrial production,and the fabricated electrode has potential application in high-current-density water splitting.
基金supported by National Natural Science Foundation of China(No.61203343)Natural Science Foundation of Hebei Province(No.E2014209106)+1 种基金Science and Technology Research Project of Hebei Provincial Department of Education(Nos.QN2016102 and QN2016105)the Graduate Student Innovation Fund of North China University of Science and Technology(No.2016S10)
文摘Existing tracking algorithms often suffer from the drift and lost problems caused by factors such as pose variation, illumination change, occlusion and motion. Therefore, developing a robust and effective tracker is still a challenging task. In this paper, we propose a real-time compressive tracking based on online Hough forest. The gray and texture features of discrete samples are extracted and compressed via the random measurement matrix. Online Hough forest classifier is used to vote the location probability of the target, and it optimizes the confidence map estimation for the target detection. The location of target being tracked is determined by combining the upper frame of the target center location and the probability confidence map of the incremental Hough forest. Finally, the classifier parameters are updated online by introducing the illumination variation and target occlusion feedback mechanism adaptively. The experiments with state-of-the-art algorithms on challenging sequences demonstrated that the proposed algorithm can effectively enhance the robustness and accuracy, and inherit the real-time performance of the compressive tracking algorithm.