We study the phot odissociation dynamics of CS2 in the ultraviolet region using the time-sliced velocity map ion imaging technique.The S(3 Pj)+CS(X1E+)product channels were observed and identified at four wavelengths ...We study the phot odissociation dynamics of CS2 in the ultraviolet region using the time-sliced velocity map ion imaging technique.The S(3 Pj)+CS(X1E+)product channels were observed and identified at four wavelengths of 201.36,203.10,204.85 and 206.61 nm.In the measured images of S(3Pj=2,1,0),the vibrational states of the CS(X1E+)co-products were partially resolved and the vibrational state distributions were determined.Moreover,the product total kinetic energy releases and the anisotropic parameters were derived.The relatively small anisotropic parameter values indicate that the S(3Pj=2丄0)+CS(X1E+)channels are very likely formed via the indirect predissociation process of CS2.The study of the S(3Pj=2,1;0)+CS(X1E+)channels,which come from the spin-orbit coupling dissociation process of CS2,shows that nonadiabatic process plays a role in the ultraviolet photodissociation of CS2.展开更多
Developing new saturable absorbers for use in the mid-infrared region has practical significance for short-pulsed lasers and related scientific and industrial applications.The performance of gold nanorods(GNRs)as satu...Developing new saturable absorbers for use in the mid-infrared region has practical significance for short-pulsed lasers and related scientific and industrial applications.The performance of gold nanorods(GNRs)as saturable absorbers at novel mid-infrared wavelengths needs to be evaluated even though these benefit from ultrafast nonlinear responses and broadband saturable absorption.Passive Q-switching of an LD-pumped 2.3μm Tm:YLF laser using GNRs was successfully realized in this study.Pulses with an 843 ns pulse width and a 6.67 kHz repetition rate were achieved using this Q-switched laser.Results showed that GNRs provide promising passive Q-switches for 2.3μm Tm-doped lasers.展开更多
基金This work was supported by the National Key R&D Program of China(No.2017YFF0104500)the National Natural Science Foundation of China(No.21590802 and No.21473173)the Strategic Priority Research Program of Chinese Academy of Sciences(No.XDB17000000).
文摘We study the phot odissociation dynamics of CS2 in the ultraviolet region using the time-sliced velocity map ion imaging technique.The S(3 Pj)+CS(X1E+)product channels were observed and identified at four wavelengths of 201.36,203.10,204.85 and 206.61 nm.In the measured images of S(3Pj=2,1,0),the vibrational states of the CS(X1E+)co-products were partially resolved and the vibrational state distributions were determined.Moreover,the product total kinetic energy releases and the anisotropic parameters were derived.The relatively small anisotropic parameter values indicate that the S(3Pj=2丄0)+CS(X1E+)channels are very likely formed via the indirect predissociation process of CS2.The study of the S(3Pj=2,1;0)+CS(X1E+)channels,which come from the spin-orbit coupling dissociation process of CS2,shows that nonadiabatic process plays a role in the ultraviolet photodissociation of CS2.
基金Project supported by the National Natural Science Foundation of China(Nos.61875077 and 61911530131)the Natural Science Foundation of the Jiangsu Higher Education Institutions of China(No.18KJA510001)。
文摘Developing new saturable absorbers for use in the mid-infrared region has practical significance for short-pulsed lasers and related scientific and industrial applications.The performance of gold nanorods(GNRs)as saturable absorbers at novel mid-infrared wavelengths needs to be evaluated even though these benefit from ultrafast nonlinear responses and broadband saturable absorption.Passive Q-switching of an LD-pumped 2.3μm Tm:YLF laser using GNRs was successfully realized in this study.Pulses with an 843 ns pulse width and a 6.67 kHz repetition rate were achieved using this Q-switched laser.Results showed that GNRs provide promising passive Q-switches for 2.3μm Tm-doped lasers.
