For a long time,the existence of single-atom catalysts(SACs),consisting of isolated atoms stabilized in a specific support,was not detected due to limitations in available characterization techniques.Over the past two...For a long time,the existence of single-atom catalysts(SACs),consisting of isolated atoms stabilized in a specific support,was not detected due to limitations in available characterization techniques.Over the past two decades,however,the ability to synthesize and characterize these systems has opened the way toward designing and testing a new class of potential catalysts[1].展开更多
CONSPECTUS:Single-atom catalysis(SAC)is a fascinating and rapidly growing field in heterogeneous catalysis.In less than 20 years,this has become one of the most widely investigated subjects by the catalytic community ...CONSPECTUS:Single-atom catalysis(SAC)is a fascinating and rapidly growing field in heterogeneous catalysis.In less than 20 years,this has become one of the most widely investigated subjects by the catalytic community for various good reasons:the ability to synthesize active catalysts using a minimum amount of precious metals,the expected higher selectivity of SACs compared to assemblies of nanoparticles of variable sizes,and the fact that SACs represent a bridge between homogeneous and heterogeneous catalysis.展开更多
文摘For a long time,the existence of single-atom catalysts(SACs),consisting of isolated atoms stabilized in a specific support,was not detected due to limitations in available characterization techniques.Over the past two decades,however,the ability to synthesize and characterize these systems has opened the way toward designing and testing a new class of potential catalysts[1].
基金supported by the Fondazione Cariplo Project“Carbon dioxide conversion into energy-rich molecules with tailored catalysts-CO2ENRICH”the Italian Ministry of University and Research(MUR)through PRIN Project 20179337R7。
文摘CONSPECTUS:Single-atom catalysis(SAC)is a fascinating and rapidly growing field in heterogeneous catalysis.In less than 20 years,this has become one of the most widely investigated subjects by the catalytic community for various good reasons:the ability to synthesize active catalysts using a minimum amount of precious metals,the expected higher selectivity of SACs compared to assemblies of nanoparticles of variable sizes,and the fact that SACs represent a bridge between homogeneous and heterogeneous catalysis.
