Soil chronosequences derived from landslides with certain time series are the great avenue to elevate our understanding on the processes of pedogenesis,nutrient dynamics,and ecosystem evolution.However,the constructio...Soil chronosequences derived from landslides with certain time series are the great avenue to elevate our understanding on the processes of pedogenesis,nutrient dynamics,and ecosystem evolution.However,the construction of reliable soil chronosequence from historical landslides remains intricate.Here,we presented a 22,000-year soil chronosequence from multiple landslides on the upper reach of Minjiang River,western China.The variation in a variety of pedogenesis indices and soil nutrients verified the reliability of the chronosequence.The silica-alumina ratio and silica sesquioxide ratio decreased significantly with soil age.This reflected the enrichment of Al/Fe/Ti oxides but the depletion of Si oxides with the soil development.Meanwhile,the values of the Chemical Index of Weathering and the Chemical Index of Alteration increased significantly with soil age,especially from 5 to 89 years.These variations were attributed to the soil weathering,which led to the destruction of soil minerals with the rapid loss of most of cations(e.g.,K,Na,Ca,and Mg)during the soil development.The concentrations of carbon and nitrogen in topsoil increased with soil age,and the carbon accumulation rate slowed significantly from 5,500 to 22,000 years.The total phosphorus concentrations decreased with soil age,suggesting the gradual loss of soil phosphorus with soil development.The results indicate that the landslide chronosequence established on the upper reach of Minjiang River is reliable and delineates a long-term soil development process,which will provide a great platform for further improvement of biogeochemical theories and understanding sustainable vegetation restoration.展开更多
To reveal the potential fungicidal mechanism of 5-((4-((4-chlorophenoxy)methyl)-5-iodo-1H-1,2,3-triazole-1-yl)methyl)-2-methylpyrimidin-4-amine(PA-1)against Botrytis cinerea(B.cinerea),the three-dimensional structure ...To reveal the potential fungicidal mechanism of 5-((4-((4-chlorophenoxy)methyl)-5-iodo-1H-1,2,3-triazole-1-yl)methyl)-2-methylpyrimidin-4-amine(PA-1)against Botrytis cinerea(B.cinerea),the three-dimensional structure of B.cinerea pyruvate dehydrogenase complex E1 component(PDHc-E1)is homology modeled,as the PA-1 shows potent E.coli PDHc-E1 and B.cinerea inhibition.Subsequent molecular docking indicates the PA-1 can tightly bind to B.cinerea PDHc-E1.Molecular dynamic simulation and MM-PBSA calculation both demonstrate that two in-termolecular interactions,π-πstacking and hydrophobic forces,provide the most contributions to the binding of PA-1 and B.cinerea PDHc-E1.Furthermore,the halogen bonding interaction between the iodine atom in PA-1 and OH in Ser181 is also crucial.The present study provides a valuable attempt to homology model the structure of B.cinerea PDHc-E1 and some key factors for the rational structure optimization of PA-1.展开更多
基金funded by the Key Program of the Chinese Academy of Sciences for International Cooperation(131551KYSB20190028)the Key Research and Development Projects Foundation of Sichuan,China(Grants No.2018JZ0075)。
文摘Soil chronosequences derived from landslides with certain time series are the great avenue to elevate our understanding on the processes of pedogenesis,nutrient dynamics,and ecosystem evolution.However,the construction of reliable soil chronosequence from historical landslides remains intricate.Here,we presented a 22,000-year soil chronosequence from multiple landslides on the upper reach of Minjiang River,western China.The variation in a variety of pedogenesis indices and soil nutrients verified the reliability of the chronosequence.The silica-alumina ratio and silica sesquioxide ratio decreased significantly with soil age.This reflected the enrichment of Al/Fe/Ti oxides but the depletion of Si oxides with the soil development.Meanwhile,the values of the Chemical Index of Weathering and the Chemical Index of Alteration increased significantly with soil age,especially from 5 to 89 years.These variations were attributed to the soil weathering,which led to the destruction of soil minerals with the rapid loss of most of cations(e.g.,K,Na,Ca,and Mg)during the soil development.The concentrations of carbon and nitrogen in topsoil increased with soil age,and the carbon accumulation rate slowed significantly from 5,500 to 22,000 years.The total phosphorus concentrations decreased with soil age,suggesting the gradual loss of soil phosphorus with soil development.The results indicate that the landslide chronosequence established on the upper reach of Minjiang River is reliable and delineates a long-term soil development process,which will provide a great platform for further improvement of biogeochemical theories and understanding sustainable vegetation restoration.
基金supported by the National Natural Science Foundation of China (No. 21807084)
文摘To reveal the potential fungicidal mechanism of 5-((4-((4-chlorophenoxy)methyl)-5-iodo-1H-1,2,3-triazole-1-yl)methyl)-2-methylpyrimidin-4-amine(PA-1)against Botrytis cinerea(B.cinerea),the three-dimensional structure of B.cinerea pyruvate dehydrogenase complex E1 component(PDHc-E1)is homology modeled,as the PA-1 shows potent E.coli PDHc-E1 and B.cinerea inhibition.Subsequent molecular docking indicates the PA-1 can tightly bind to B.cinerea PDHc-E1.Molecular dynamic simulation and MM-PBSA calculation both demonstrate that two in-termolecular interactions,π-πstacking and hydrophobic forces,provide the most contributions to the binding of PA-1 and B.cinerea PDHc-E1.Furthermore,the halogen bonding interaction between the iodine atom in PA-1 and OH in Ser181 is also crucial.The present study provides a valuable attempt to homology model the structure of B.cinerea PDHc-E1 and some key factors for the rational structure optimization of PA-1.