Number concentration and distribution of airborne particles in the size range 5.6 to 560 nm diameter were measured in Beijing for a 15-d period in winter 2005. Dally average number concentrations of nucleation mode (...Number concentration and distribution of airborne particles in the size range 5.6 to 560 nm diameter were measured in Beijing for a 15-d period in winter 2005. Dally average number concentrations of nucleation mode (5.6-20 um), Aitken mode (20-100 um), and accumulation mode (100-560 um) particles, and total particles were 17500, 32000, 4000, and 53500 cm^-3, respectively. Average particle size distribution was monomodal with a mode diameter of about 40 um at night and bimodal with mode diameters of about 10 and about 40 um during the daytime. New particle formation events, which were connected to diurnal variation of nucleation mode particles, were observed in more than half of the observation days. The events often started around 10:00-11:00 Chinese Standard Time (CST) and ended up after 3-4 h. Concentrations of Aitken and accumulation mode particles increased from midnight and reached their maxima at about 10:00 CST, and then decreased and became the lowest in the afternoon. Analysis of diurnal cycles in traffic volume and meteorological parameters revealed that the accumulation of the particles in Aitken and accumulation modes in the morning was influenced by formation of an inversion and increase in vehicle emission, and dispersion of such particles in the afternoon was associated with more effective vertical mixing and higher wind speed.展开更多
A method that enables the user to assess air pollution originated from vehicle emission in the urban center was described by taking Macao as an example. The method involved the use of mathematical models for the calcu...A method that enables the user to assess air pollution originated from vehicle emission in the urban center was described by taking Macao as an example. The method involved the use of mathematical models for the calculation of urban pollutant emissions and concentrations, of which a revised MOBILE5 was adopted to calculate the emission factors and two dispersion models of CAR and OSPM were used to calculate the long term and short term concentrations within street canyons, respectively. The results show consistency with the monitoring data, and some conclusions of controlling vehicle emissions are given based on the calculation results.展开更多
基金Project supported by the National Natural Science Foundation of China(No.20477020)the National Science Fund for Distinguished Young Scholars(No.20625722).
文摘Number concentration and distribution of airborne particles in the size range 5.6 to 560 nm diameter were measured in Beijing for a 15-d period in winter 2005. Dally average number concentrations of nucleation mode (5.6-20 um), Aitken mode (20-100 um), and accumulation mode (100-560 um) particles, and total particles were 17500, 32000, 4000, and 53500 cm^-3, respectively. Average particle size distribution was monomodal with a mode diameter of about 40 um at night and bimodal with mode diameters of about 10 and about 40 um during the daytime. New particle formation events, which were connected to diurnal variation of nucleation mode particles, were observed in more than half of the observation days. The events often started around 10:00-11:00 Chinese Standard Time (CST) and ended up after 3-4 h. Concentrations of Aitken and accumulation mode particles increased from midnight and reached their maxima at about 10:00 CST, and then decreased and became the lowest in the afternoon. Analysis of diurnal cycles in traffic volume and meteorological parameters revealed that the accumulation of the particles in Aitken and accumulation modes in the morning was influenced by formation of an inversion and increase in vehicle emission, and dispersion of such particles in the afternoon was associated with more effective vertical mixing and higher wind speed.
文摘A method that enables the user to assess air pollution originated from vehicle emission in the urban center was described by taking Macao as an example. The method involved the use of mathematical models for the calculation of urban pollutant emissions and concentrations, of which a revised MOBILE5 was adopted to calculate the emission factors and two dispersion models of CAR and OSPM were used to calculate the long term and short term concentrations within street canyons, respectively. The results show consistency with the monitoring data, and some conclusions of controlling vehicle emissions are given based on the calculation results.