Radiocarbon content in biogenic samples is widely used to study the variation of atmospheric CO<sub>2</sub> due to anthropogenic activities. A total of 20 samples of several types of tree leaves, were anal...Radiocarbon content in biogenic samples is widely used to study the variation of atmospheric CO<sub>2</sub> due to anthropogenic activities. A total of 20 samples of several types of tree leaves, were analyzed for this study. Sampling was carried out at the end of the rainy season in 2017 from the surrounding of the SOCOCIM cement factory in Rufisque town. Rufisque is located on the peninsula of Cape Verde, 25 km east of Dakar, where it is the 《south gate》 of the agglomeration. Reference samples of five different species were collected during the same period (2017) from a clean zone. The <sup>14</sup>C method was used for the determination of Δ<sup>14</sup>C values. The data show that the <sup>14</sup>C concentration in the studied sites was significantly lower than the clean area, due to the release of anthropogenic CO<sub>2</sub>. To estimate the Suess effect, the fossil fuel fraction was determined based on equations of mass balance for CO<sub>2</sub> concentration, stable isotopic composition of carbon, and <sup>14</sup>C concentration. The results show that selected locations are affected differently according to their distance from the factory and the wind direction.展开更多
The abundances of heavy elements produced in r-process nucleosynthesis in the early solar system need experimental verification.^(244)Pu could be the heaviest primordial nuclide produced before the formation of the Ea...The abundances of heavy elements produced in r-process nucleosynthesis in the early solar system need experimental verification.^(244)Pu could be the heaviest primordial nuclide produced before the formation of the Earth still being detectable today.As recent attempts failed to confirm the discovery of ^(244)Pu signals at a concentration of 1.0×10^(-18)g/g in bastnaesite reported by Hoffman et al.in this study,the total primordial ^(244)Pu in 450 g bastnaesite sample from Bayan Obo ore (China) was measured using ultrasensitive compact accelerator mass spectrometry (AMS).As no ^(244)Pu signal was detected,an upper limit for the ^(244)Pu in our bastnaesite sample was estimated to be 2.1×10^(-20)g/g at 99%confidence level.展开更多
文摘Radiocarbon content in biogenic samples is widely used to study the variation of atmospheric CO<sub>2</sub> due to anthropogenic activities. A total of 20 samples of several types of tree leaves, were analyzed for this study. Sampling was carried out at the end of the rainy season in 2017 from the surrounding of the SOCOCIM cement factory in Rufisque town. Rufisque is located on the peninsula of Cape Verde, 25 km east of Dakar, where it is the 《south gate》 of the agglomeration. Reference samples of five different species were collected during the same period (2017) from a clean zone. The <sup>14</sup>C method was used for the determination of Δ<sup>14</sup>C values. The data show that the <sup>14</sup>C concentration in the studied sites was significantly lower than the clean area, due to the release of anthropogenic CO<sub>2</sub>. To estimate the Suess effect, the fossil fuel fraction was determined based on equations of mass balance for CO<sub>2</sub> concentration, stable isotopic composition of carbon, and <sup>14</sup>C concentration. The results show that selected locations are affected differently according to their distance from the factory and the wind direction.
基金financially supported by the National Natural Science Foundation of China (Nos. 11675150, 12005197 and 12175201)。
文摘The abundances of heavy elements produced in r-process nucleosynthesis in the early solar system need experimental verification.^(244)Pu could be the heaviest primordial nuclide produced before the formation of the Earth still being detectable today.As recent attempts failed to confirm the discovery of ^(244)Pu signals at a concentration of 1.0×10^(-18)g/g in bastnaesite reported by Hoffman et al.in this study,the total primordial ^(244)Pu in 450 g bastnaesite sample from Bayan Obo ore (China) was measured using ultrasensitive compact accelerator mass spectrometry (AMS).As no ^(244)Pu signal was detected,an upper limit for the ^(244)Pu in our bastnaesite sample was estimated to be 2.1×10^(-20)g/g at 99%confidence level.
