To solve the problem of long response time when users obtain suitable cutting parameters through the Internet based platform,a case-based reasoning framework is proposed.Specifically,a Hamming distance and Euclidean d...To solve the problem of long response time when users obtain suitable cutting parameters through the Internet based platform,a case-based reasoning framework is proposed.Specifically,a Hamming distance and Euclidean distance combined method is designed to measure the similarity of case features which have both numeric and category properties.In addition,AHP(Analytic Hierarchy Process)and entropy weight method are integrated to provide features weight,where both user preferences and comprehensive impact of the index have been concerned.Grey relation analysis is used to obtain the similarity of a new problem and alternative cases.Finally,a platform is also developed on Visual Studio 2015,and a case study is demonstrated to verify the practicality and efficiency of the proposed method.This method can obtain cutting parameters which is suitable without iterative calculation.Compared with the traditional PSO(Particle swarm optimization algorithm)and GA(Genetic algorithm),it can obtain faster response speed.This method can provide ideas for selecting processing parameters in industrial production.While guaranteeing the characteristic information is similar,this approach can select processing parameters which is the most appropriate for the production process and a lot of time can be saved.展开更多
A microgrid(MG)refers to a set of loads,generation resources and energy storage systems acting as a controllable load or a generator to supply power and heating to a local area.The MG-generated power management is a c...A microgrid(MG)refers to a set of loads,generation resources and energy storage systems acting as a controllable load or a generator to supply power and heating to a local area.The MG-generated power management is a central topic for MG design and operation.The existence of dispersed generation(DG)resources has faced MG management with new issues.Depending on the level of exchanges between an MG and the main grid,the MG operation states can be divided into independent or grid-connected ones.Energy management in MGs aims to supply power at the lowest cost for optimal load response.This study examines MG energy management in two operational modes of islanded and grid-connected,and proposes a structure with two control layers(primary and secondary)for energy management.At the principal level of control,the energy management system is determined individually for all MG by taking into consideration the probability constraints and RES uncertainty by the Weibull the probability density function(PDF),generation resources’power as well as the generation surplus and deficit of each MG.Then,the information of the power surplus and deficit of each MG must be sent to the central energy management system.To confirm the proposed structure,a case system with two MGs and a condensive load is simulated by using a multi-time harmony search algorithm.Several scenarios are applied to evaluate the performance of this algorithm.The findings clearly show the effectiveness of the proposed system in the energy management of several MGs,leading to the optimal performance of the resources per MG.Moreover,the proposed control scheme properly controls the MG and grid’s performance in their interactions and offers a high level of robustness,stable behavior under different conditions and high quality of power supply.展开更多
Controlled and switchable adhesion is commonly observed in biological systems.In recent years,many scholars have focused on making switchable bio-inspired adhesives.However,making a bio-inspired adhesive with high adh...Controlled and switchable adhesion is commonly observed in biological systems.In recent years,many scholars have focused on making switchable bio-inspired adhesives.However,making a bio-inspired adhesive with high adhesion performance and excellent dynamic switching properties is still a challenge.A Shape Memory Polymer Bio-inspired Adhesive(SMPBA)was successfully developed,well realizing high adhesion(about 337 kPa),relatively low preload(about90 kPa),high adhesion-to-preload ratio(about 3.74),high switching ratio(about 6.74),and easy detachment,which are attributed to the controlled modulus and contact area by regulating temperature and the Shape Memory Effect(SME).Furthermore,SMPBA exhibits adhesion strength of80–337 kPa on various surfaces(silicon,iron,and aluminum)with different roughness(Ra=0.021–10.280)because of the conformal contact,reflecting outstanding surface adaptability.The finite element analysis verifies the bending ability under different temperatures,while the adhesion model analyzes the influence of preload on contact area and adhesion.Furthermore,an Unmanned Aerial Vehicle(UAV)landing device with SMPBA was designed and manufactured to achieve UAV landing on and detaching from various surfaces.This study provides a novel switchable bio-inspired adhesive and UAV landing method.展开更多
Purely organic room-temperature phosphors,which have received extensive attention as emerging stateof-the-art luminescent materials in various fields,have a longer lifetime than fluorophores.The energy gap law and El-...Purely organic room-temperature phosphors,which have received extensive attention as emerging stateof-the-art luminescent materials in various fields,have a longer lifetime than fluorophores.The energy gap law and El-Sayed’s rule provide clear design principles for the development of organic room-temperature phosphorescence.Therefore,the incorporation of heteroatoms(such as sulfur and phosphorus)usually promotes the intersystem crossing rate and increases the 3(π,π*)configuration to realize long lifetimes.Furthermore,boron-containing phosphors not only display excellent phosphorescence properties but also expand El-Sayed’s rule without(n,π*)transitions.This review summarizes recent work on organic phosphorescence of heterocycles with boron,sulfur,and phosphorus heteroatoms and highlights the significance of the guidelines for constructing efficient phosphorescence molecules.This work is instrumental in further diversifying the pool of phosphorescent molecules and developing new and effective design strategies.展开更多
To understand the deformation mechanism of molecular crystals under mechanical forces will accelerate the molecular design and preparation of deformable crystals.Herein,the relationship between structural halogenation...To understand the deformation mechanism of molecular crystals under mechanical forces will accelerate the molecular design and preparation of deformable crystals.Herein,the relationship between structural halogenation and molecular-level stacking,micro/nanoscale surface morphology,and macroscopic mechanical properties are investigated.Elastic crystals of halo-pyrimidinyl carbazoles(CzM-Cl,CzM-Br and CzM-I)with lamellar structure and brittle crystal(CzM-F)were quantitatively analyzed by crystal energy framework(CEF)providing the inter/intralayer interaction energy(Inter/Intra-IE).It is revealed that the elastic crystals bend under external force as a result from stronger Intra-IE to prevent cleavage and weaker Inter-IE for the short-range movement of molecules on the slip plane.This research will provide an insight for the molecular design of flexible crystals and facilitate the development of next-generation smart crystal materials.展开更多
The power electronic transformer(PET) has recently emerged as a type of power converter. It features the basic functions of power conversion and isolation as well as additional functions related to power quality contr...The power electronic transformer(PET) has recently emerged as a type of power converter. It features the basic functions of power conversion and isolation as well as additional functions related to power quality control. A novel PET for a distribution grid called a flexible power distribution unit is proposed in this paper, and the energy exchange mechanism between the network and the load is revealed. A 30 kW 600 VAC/220 VAC/110 VDC medium-frequency isolated prototype is developed and demonstrated. This paper also presents key control strategies of the PET for electrical distribution grid applications,especially under grid voltage disturbance conditions.Moreover, stability issues related to the grid-connected three-phase PET are discussed and verified with an impedance-based analysis. The PET prototype is tested, and it passes the voltage-disturbance ride-through function. The experimental results verify the power quality control abilities of the PET.展开更多
A hybrid structure consisting of boron-doped porous carbon spheres and graphene (BPCS-G) has been designed and synthesized toward solving the polysulfide- shuttle problem, which is the most critical issue of current...A hybrid structure consisting of boron-doped porous carbon spheres and graphene (BPCS-G) has been designed and synthesized toward solving the polysulfide- shuttle problem, which is the most critical issue of current Li-S batteries. The proposed hybrid structure showing high surface area (870 m^2.g^-1) and high B-dopant content (6.51 wt.%) simultaneously offers both physical confinement and chemical absorption of polysulfides. On one hand, the abundant-pore structure ensures high sulfur loading, facilitates fast charge transfer, and restrains polysulfide migration during cycling. On the other hand, our density functional theory calculations demonstrate that the B dopant is capable of chemically binding polysulfides. As a consequence of such dual polysulfide confinement, the BPCS-G/S cathode prepared with 70 wt.% sulfur loading presents a high reversible capacity of 1,174 mAh.g^-1 at 0.02 C, a high rate capacity of 396 mAh·g^-1 at 5 G and good cyclability over 500 cycles with only 0.05% capacity decay per cycle. The present work provides an efficient and cost-effective platform for the scalable synthesis of high-performance carbon-based materials for advanced Li-S batteries.展开更多
Laser flash photolysis and sodium dodecyl sulfate-polyacrylamide gel electrophoresis(SDS-PAGE) experiments were carried out to study the photosensitive damage induced by pazufloxacin(PAX) and the protection of lysozym...Laser flash photolysis and sodium dodecyl sulfate-polyacrylamide gel electrophoresis(SDS-PAGE) experiments were carried out to study the photosensitive damage induced by pazufloxacin(PAX) and the protection of lysozyme(Lyso) by ferulic acid(FCA), an active antioxidant. Transient absorption spectra revealed electron transfer from Lyso and FCA to 3PAX*, with respective bimolecular reaction rate constants of 6.3×107 and 1.4×1010 dm3/(mol s). A pulse radiolysis study was also performed to investigate the formation of Lyso radical cations. Results showed that FCA effectively inhibited the cross-linking of protein induced by fluoroquinolones. Finally, a mechanism of the protective effect of FCA on Lyso was proposed.展开更多
The traffic and user have significant impacts on the electric vehicle(EV)charging load but are not considered in the existing research.We propose a novel integrated simulation framework considering the traffic,the use...The traffic and user have significant impacts on the electric vehicle(EV)charging load but are not considered in the existing research.We propose a novel integrated simulation framework considering the traffic,the user,and power grid as well as the EV traveling,parking and charging based on cellular automaton(CA).The traffic is modeled by the traffic module of the proposed framework based on CA,while the power grid and user are modeled in the EV charging module.The traffic flow,user’s charging preference,user’s charging satisfaction,and the total supply capability(TSC)in the surveyed region are considered in the proposed framework.Two cases are carried out to show the interactions between the user and power grid.It is shown that the proposed framework can accurately simulate the interactions among traffic situation,user's behavior and TSC,which are significantly lacking in the existing research.The proposed framework is scalable in considering additional interrelated elements.展开更多
Organic phosphorescence materials demonstrate potential optoelectronic applications due to their remarkably ultralong organic phosphorescence(UOP)lifetime and abundant optical characteristics prior to the fluorescence...Organic phosphorescence materials demonstrate potential optoelectronic applications due to their remarkably ultralong organic phosphorescence(UOP)lifetime and abundant optical characteristics prior to the fluorescence materials.For a better insight into the intrinsic relationship among regioisomeric molecules,crystalline interactions,and phosphorescence properties,three crystalline dicarbazol-9-yl pyrazine-based regioisomers with para-,meta-and ortho-convergent substitutions(p-DCzP,m-DCzP,and o-DCzP)were designed and presented gradually increased UOP lifetimes prolonging from 63.14,127.93 to 350.46 ms,respectively,due to the regioisomerism effect(RIE)which would be an effective strategy for better understanding of structure-property of UOP materials.展开更多
Additive manufacturing(AM)has gained extensive attention and tremendous research due to its advantages of fabricating complex-shaped parts without the need of casting mold.However,distortion is a known issue for many ...Additive manufacturing(AM)has gained extensive attention and tremendous research due to its advantages of fabricating complex-shaped parts without the need of casting mold.However,distortion is a known issue for many AM technologies,which decreases the precision of as-built parts.Like fusion welding,the local high-energy input generates residual stresses,which can adversely affect the fatigue performance of AM parts.To the best of the authors’knowledge,a comprehensive review does not exist regarding the distortion and residual stresses dedicated for AM,despite some work has explored the interrelationship between the two.The present review is aimed to fill in the identified knowledge gap,by first describing the evolution of distortion and residual stresses for a range of AM processes,and second assessing their influencing factors.This allows us to elucidate their formation mechanisms from both the micro-and macro-scales.Moreover,approaches which have been successfully adopted to mitigate both the distortion and residual stresses are reviewed.It is anticipated that this review paper opens many opportunities to increase the success rate of AM parts by improving the dimension precision and fatigue life.展开更多
Two electron-deficient azaacenes including di-and tetra-cyanodiazafluorene(DCAF and TCAF)with the advantages of deep lowest unoccupied molecular orbital(LUMO),green-synthesis,low-cost,simply purification method,excell...Two electron-deficient azaacenes including di-and tetra-cyanodiazafluorene(DCAF and TCAF)with the advantages of deep lowest unoccupied molecular orbital(LUMO),green-synthesis,low-cost,simply purification method,excellent yields have been obtained,characterized and used as electron injection materials(EIMs)in three groups of electroluminescence devices.Device B with TCAF as EIM exhibited the best performance including turn-on voltage of 5.0 V,stronger maximum luminance intensity of 31,549 cd/m2,higher luminance efficiency of 62.34 cd/A and larger power efficiency of 21.74 lm/W which are 0.53,6.7,9.3 and 15.3 times than that of device A with DCAF as EIMs,respectively.The enhanced interfacial electron injection ability of TCAF than that of DCAF is supported by its better electron mobility in electron-only device,deeper LUMO(-4.52 eV),and stronger electronic affinity.Best external quantum efficiency of 16.56%was achieved with optimized thicknesses of TCAF as EIM and TPBi as electron transporting layer.As a new comer of acceptor family,TCAF would push forward organic electronics with more fascinating and significant applications.展开更多
基金the Sichuan Science and Technology Program(Nos.23ZHCG0049,2023YFG0078,23ZHCG0030,2021ZDZX0007)SCU-SUINING Project(2022CDSN-14).
文摘To solve the problem of long response time when users obtain suitable cutting parameters through the Internet based platform,a case-based reasoning framework is proposed.Specifically,a Hamming distance and Euclidean distance combined method is designed to measure the similarity of case features which have both numeric and category properties.In addition,AHP(Analytic Hierarchy Process)and entropy weight method are integrated to provide features weight,where both user preferences and comprehensive impact of the index have been concerned.Grey relation analysis is used to obtain the similarity of a new problem and alternative cases.Finally,a platform is also developed on Visual Studio 2015,and a case study is demonstrated to verify the practicality and efficiency of the proposed method.This method can obtain cutting parameters which is suitable without iterative calculation.Compared with the traditional PSO(Particle swarm optimization algorithm)and GA(Genetic algorithm),it can obtain faster response speed.This method can provide ideas for selecting processing parameters in industrial production.While guaranteeing the characteristic information is similar,this approach can select processing parameters which is the most appropriate for the production process and a lot of time can be saved.
文摘A microgrid(MG)refers to a set of loads,generation resources and energy storage systems acting as a controllable load or a generator to supply power and heating to a local area.The MG-generated power management is a central topic for MG design and operation.The existence of dispersed generation(DG)resources has faced MG management with new issues.Depending on the level of exchanges between an MG and the main grid,the MG operation states can be divided into independent or grid-connected ones.Energy management in MGs aims to supply power at the lowest cost for optimal load response.This study examines MG energy management in two operational modes of islanded and grid-connected,and proposes a structure with two control layers(primary and secondary)for energy management.At the principal level of control,the energy management system is determined individually for all MG by taking into consideration the probability constraints and RES uncertainty by the Weibull the probability density function(PDF),generation resources’power as well as the generation surplus and deficit of each MG.Then,the information of the power surplus and deficit of each MG must be sent to the central energy management system.To confirm the proposed structure,a case system with two MGs and a condensive load is simulated by using a multi-time harmony search algorithm.Several scenarios are applied to evaluate the performance of this algorithm.The findings clearly show the effectiveness of the proposed system in the energy management of several MGs,leading to the optimal performance of the resources per MG.Moreover,the proposed control scheme properly controls the MG and grid’s performance in their interactions and offers a high level of robustness,stable behavior under different conditions and high quality of power supply.
基金financial support from the National Natural Science Foundation of China(No.51605220)the Jiangsu Province Natural Science Foundation,China(No.BK20160793)+1 种基金the Postgraduate Research and Practice Innovation Program of Nanjing University of Aeronautics and Astronautics,China(No.xcxjh20210514)the Fundamental Research Funds for the Central Universities,China(No.XCA2205406)。
文摘Controlled and switchable adhesion is commonly observed in biological systems.In recent years,many scholars have focused on making switchable bio-inspired adhesives.However,making a bio-inspired adhesive with high adhesion performance and excellent dynamic switching properties is still a challenge.A Shape Memory Polymer Bio-inspired Adhesive(SMPBA)was successfully developed,well realizing high adhesion(about 337 kPa),relatively low preload(about90 kPa),high adhesion-to-preload ratio(about 3.74),high switching ratio(about 6.74),and easy detachment,which are attributed to the controlled modulus and contact area by regulating temperature and the Shape Memory Effect(SME).Furthermore,SMPBA exhibits adhesion strength of80–337 kPa on various surfaces(silicon,iron,and aluminum)with different roughness(Ra=0.021–10.280)because of the conformal contact,reflecting outstanding surface adaptability.The finite element analysis verifies the bending ability under different temperatures,while the adhesion model analyzes the influence of preload on contact area and adhesion.Furthermore,an Unmanned Aerial Vehicle(UAV)landing device with SMPBA was designed and manufactured to achieve UAV landing on and detaching from various surfaces.This study provides a novel switchable bio-inspired adhesive and UAV landing method.
基金the Ministry of Education and Synergetic Innovation Center for Organic Electronics and Information Displays,LiaoNing Revitalization Talents Program(grant no.XLYC1902111)and the Key Projects of the Department of Education,Liaoning Province(grant no.LZD202005)for their financial support of this research.
文摘Purely organic room-temperature phosphors,which have received extensive attention as emerging stateof-the-art luminescent materials in various fields,have a longer lifetime than fluorophores.The energy gap law and El-Sayed’s rule provide clear design principles for the development of organic room-temperature phosphorescence.Therefore,the incorporation of heteroatoms(such as sulfur and phosphorus)usually promotes the intersystem crossing rate and increases the 3(π,π*)configuration to realize long lifetimes.Furthermore,boron-containing phosphors not only display excellent phosphorescence properties but also expand El-Sayed’s rule without(n,π*)transitions.This review summarizes recent work on organic phosphorescence of heterocycles with boron,sulfur,and phosphorus heteroatoms and highlights the significance of the guidelines for constructing efficient phosphorescence molecules.This work is instrumental in further diversifying the pool of phosphorescent molecules and developing new and effective design strategies.
基金the primary financial support by the National Natural Science Foundation of China (No. 21975126)the open research fund from Anhui Province Key Laboratory of Optoelectronic Materials Science and Technology+1 种基金the Technology and Research Innovation in University of Jiangsu Province (No.KYCX21_0772)the Ministry of Education and Synergetic Innovation Center for Organic Electronics and Information Displays
文摘To understand the deformation mechanism of molecular crystals under mechanical forces will accelerate the molecular design and preparation of deformable crystals.Herein,the relationship between structural halogenation and molecular-level stacking,micro/nanoscale surface morphology,and macroscopic mechanical properties are investigated.Elastic crystals of halo-pyrimidinyl carbazoles(CzM-Cl,CzM-Br and CzM-I)with lamellar structure and brittle crystal(CzM-F)were quantitatively analyzed by crystal energy framework(CEF)providing the inter/intralayer interaction energy(Inter/Intra-IE).It is revealed that the elastic crystals bend under external force as a result from stronger Intra-IE to prevent cleavage and weaker Inter-IE for the short-range movement of molecules on the slip plane.This research will provide an insight for the molecular design of flexible crystals and facilitate the development of next-generation smart crystal materials.
基金supported in part by the National Basic Research Program of China(No.2016YFB0900404)the National Natural Science Foundation of China(No.51477030,No.51207023)+2 种基金the Cooperative Innovation Fund of Jiangsu Province–the Prospective and Joint Research Project(No.BY2015070-18)the Basic and Prospective Science and Technology Project of State Grid Corporation of China(No.PD71-17-024)the Fundamental Research Funds for the Central Universities(No.2242017K40159)
文摘The power electronic transformer(PET) has recently emerged as a type of power converter. It features the basic functions of power conversion and isolation as well as additional functions related to power quality control. A novel PET for a distribution grid called a flexible power distribution unit is proposed in this paper, and the energy exchange mechanism between the network and the load is revealed. A 30 kW 600 VAC/220 VAC/110 VDC medium-frequency isolated prototype is developed and demonstrated. This paper also presents key control strategies of the PET for electrical distribution grid applications,especially under grid voltage disturbance conditions.Moreover, stability issues related to the grid-connected three-phase PET are discussed and verified with an impedance-based analysis. The PET prototype is tested, and it passes the voltage-disturbance ride-through function. The experimental results verify the power quality control abilities of the PET.
文摘A hybrid structure consisting of boron-doped porous carbon spheres and graphene (BPCS-G) has been designed and synthesized toward solving the polysulfide- shuttle problem, which is the most critical issue of current Li-S batteries. The proposed hybrid structure showing high surface area (870 m^2.g^-1) and high B-dopant content (6.51 wt.%) simultaneously offers both physical confinement and chemical absorption of polysulfides. On one hand, the abundant-pore structure ensures high sulfur loading, facilitates fast charge transfer, and restrains polysulfide migration during cycling. On the other hand, our density functional theory calculations demonstrate that the B dopant is capable of chemically binding polysulfides. As a consequence of such dual polysulfide confinement, the BPCS-G/S cathode prepared with 70 wt.% sulfur loading presents a high reversible capacity of 1,174 mAh.g^-1 at 0.02 C, a high rate capacity of 396 mAh·g^-1 at 5 G and good cyclability over 500 cycles with only 0.05% capacity decay per cycle. The present work provides an efficient and cost-effective platform for the scalable synthesis of high-performance carbon-based materials for advanced Li-S batteries.
基金supported by the National Natural Science Foundation of China(21173252)
文摘Laser flash photolysis and sodium dodecyl sulfate-polyacrylamide gel electrophoresis(SDS-PAGE) experiments were carried out to study the photosensitive damage induced by pazufloxacin(PAX) and the protection of lysozyme(Lyso) by ferulic acid(FCA), an active antioxidant. Transient absorption spectra revealed electron transfer from Lyso and FCA to 3PAX*, with respective bimolecular reaction rate constants of 6.3×107 and 1.4×1010 dm3/(mol s). A pulse radiolysis study was also performed to investigate the formation of Lyso radical cations. Results showed that FCA effectively inhibited the cross-linking of protein induced by fluoroquinolones. Finally, a mechanism of the protective effect of FCA on Lyso was proposed.
基金This work was supported by the National Natural Science Foundation of China(No.51936003).
文摘The traffic and user have significant impacts on the electric vehicle(EV)charging load but are not considered in the existing research.We propose a novel integrated simulation framework considering the traffic,the user,and power grid as well as the EV traveling,parking and charging based on cellular automaton(CA).The traffic is modeled by the traffic module of the proposed framework based on CA,while the power grid and user are modeled in the EV charging module.The traffic flow,user’s charging preference,user’s charging satisfaction,and the total supply capability(TSC)in the surveyed region are considered in the proposed framework.Two cases are carried out to show the interactions between the user and power grid.It is shown that the proposed framework can accurately simulate the interactions among traffic situation,user's behavior and TSC,which are significantly lacking in the existing research.The proposed framework is scalable in considering additional interrelated elements.
基金supported by the National Natural Science Foundation of China(Nos.21975126,51673095,21875104,21875191,21603104)the Natural Science Foundation of Jiangsu Province(Nos.BK20171470,BK20160991,BK20150064,BK20130912)+1 种基金973 Program(No.2015CB932200)Ministry of Education and Synergetic Innovation Center for Organic Electronics and Information Displays for financial support
文摘Organic phosphorescence materials demonstrate potential optoelectronic applications due to their remarkably ultralong organic phosphorescence(UOP)lifetime and abundant optical characteristics prior to the fluorescence materials.For a better insight into the intrinsic relationship among regioisomeric molecules,crystalline interactions,and phosphorescence properties,three crystalline dicarbazol-9-yl pyrazine-based regioisomers with para-,meta-and ortho-convergent substitutions(p-DCzP,m-DCzP,and o-DCzP)were designed and presented gradually increased UOP lifetimes prolonging from 63.14,127.93 to 350.46 ms,respectively,due to the regioisomerism effect(RIE)which would be an effective strategy for better understanding of structure-property of UOP materials.
基金National Key Research and Development Program of China(Grant No.2018YFB1105400)National Natural Science Foundation of China(Grant No.51475238)+2 种基金Key Research and Development Program of Jiangsu Provincial Department of Science and Technology of China(Grant No.BE2019002)China Post-Doctoral Fund(Grant No.2020M671475)UK's Engineering and Physical Sciences Research Council,and EPSRC Early Career Fellowship Scheme[EP/R043973/1].
文摘Additive manufacturing(AM)has gained extensive attention and tremendous research due to its advantages of fabricating complex-shaped parts without the need of casting mold.However,distortion is a known issue for many AM technologies,which decreases the precision of as-built parts.Like fusion welding,the local high-energy input generates residual stresses,which can adversely affect the fatigue performance of AM parts.To the best of the authors’knowledge,a comprehensive review does not exist regarding the distortion and residual stresses dedicated for AM,despite some work has explored the interrelationship between the two.The present review is aimed to fill in the identified knowledge gap,by first describing the evolution of distortion and residual stresses for a range of AM processes,and second assessing their influencing factors.This allows us to elucidate their formation mechanisms from both the micro-and macro-scales.Moreover,approaches which have been successfully adopted to mitigate both the distortion and residual stresses are reviewed.It is anticipated that this review paper opens many opportunities to increase the success rate of AM parts by improving the dimension precision and fatigue life.
基金the National Natural Science Foundation of China(Nos.21975126,51673095,21875104,21875191,21603104)the Natural Science Foundation of Jiangsu Province(Nos.BK20171470,BK20160991,BK20150064,BK20130912)+1 种基金973 Program(No.2015CB932200)Ministry of Education and Synergetic Innovation Center for Organic Electronics and Information Displays for financial support
文摘Two electron-deficient azaacenes including di-and tetra-cyanodiazafluorene(DCAF and TCAF)with the advantages of deep lowest unoccupied molecular orbital(LUMO),green-synthesis,low-cost,simply purification method,excellent yields have been obtained,characterized and used as electron injection materials(EIMs)in three groups of electroluminescence devices.Device B with TCAF as EIM exhibited the best performance including turn-on voltage of 5.0 V,stronger maximum luminance intensity of 31,549 cd/m2,higher luminance efficiency of 62.34 cd/A and larger power efficiency of 21.74 lm/W which are 0.53,6.7,9.3 and 15.3 times than that of device A with DCAF as EIMs,respectively.The enhanced interfacial electron injection ability of TCAF than that of DCAF is supported by its better electron mobility in electron-only device,deeper LUMO(-4.52 eV),and stronger electronic affinity.Best external quantum efficiency of 16.56%was achieved with optimized thicknesses of TCAF as EIM and TPBi as electron transporting layer.As a new comer of acceptor family,TCAF would push forward organic electronics with more fascinating and significant applications.