Magnetic topological materials have attracted much attention due to the correlation between topology and magnetism.Recent studies suggest that EuCd_(2)As_(2) is an antiferromagnetic topological material.Here by carryi...Magnetic topological materials have attracted much attention due to the correlation between topology and magnetism.Recent studies suggest that EuCd_(2)As_(2) is an antiferromagnetic topological material.Here by carrying out thorough magnetic,electrical and thermodynamic property measurements,we discover a long-time relaxation of the magnetic susceptibility in EuCd_(2)As_(2).The(001)in-plane magnetic susceptibility at 5 K is found to continuously increase up to∼10%over the time of∼14 hours.The magnetic relaxation is anisotropic and strongly depends on the temperature and the applied magnetic field.These results will stimulate further theoretical and experimental studies to understand the origin of the relaxation process and its effect on the electronic structure and physical properties of the magnetic topological materials.展开更多
The search for quantum spin liquid(QSL) materials has attracted significant attention in the field of condensed matter physics in recent years, however so far only a handful of them are considered as candidates hostin...The search for quantum spin liquid(QSL) materials has attracted significant attention in the field of condensed matter physics in recent years, however so far only a handful of them are considered as candidates hosting QSL ground state. Owning to their geometrically frustrated structures, Kagome materials are ideal systems to realize QSL. We synthesize the kagome structured material claringbullite(Cu_4(OH)_6FCl) and then replace inter-layer Cu with Zn to form Cu_3Zn(OH)_6FCl. Comprehensive measurements reveal that doping Zn^(2+) ions transforms magnetically ordered Cu_4(OH)_6FCl into a non-magnetic QSL candidate Cu_3Zn(OH)_6FCl. Therefore,the successful syntheses of Cu_4(OH)_6FCl and Cu_3Zn(OH)_6FCl provide not only a new platform for the study of QSL but also a novel pathway of investigating the transition between QSL and magnetically ordered systems.展开更多
Superconductivity on the border of the long-range magnetic order has been discovered in Mn P under high pressures. In order to investigate the nature of the magnetic properties adjacent to the superconducting state, w...Superconductivity on the border of the long-range magnetic order has been discovered in Mn P under high pressures. In order to investigate the nature of the magnetic properties adjacent to the superconducting state, we performed zero-field 31 P NMR for Mn P single crystal under ambient and hydrostatic pressure of 2 GPa, respectively. Radio frequency power level was used to determine whether NMR signal originates from a helical state or not. When 2 GPa pressure was applied, the signal from helical state exists even above 160 K, while that from the ferromagnetic phase was not observed. Our NMR results indicate that the magnetic phase which is adjacent to the superconducting state is in a helical magnetic structure.展开更多
Measurements of magnetic and transport properties were performed on needle-shaped single crystals of Ce_(12)Fe_(57.5)As_(41)and La_(12)Fe_(57.5)As_(41).The availability of a complete set of data enabled a side-by-side...Measurements of magnetic and transport properties were performed on needle-shaped single crystals of Ce_(12)Fe_(57.5)As_(41)and La_(12)Fe_(57.5)As_(41).The availability of a complete set of data enabled a side-by-side comparison between these two rare earth compounds.Both compounds exhibited multiple magnetic orders within 2-300 K and metamagnetic transitions at various fields.Ferromagnetic transitions with Curie temperatures of 100 and 125 K were found for Ce_(12)Fe_(57.5)As_(41)and La_(12)Fe_(57.5)As_(41),respectively,followed by antiferromagnetic type spin reorientations near Curie temperatures.The magnetic properties underwent complex evolution in the magnetic field for both compounds.An antiferromagnetic phase transition at about 60 K and 0.2 T was observed merely for Ce_(12)Fe_(57.5)As_(41).The field-induced magnetic phase transition occurred from antiferromagnetic to ferromagnetic structure.A strong magnetocrystalline anisotropy was evident from magnetization measurements of Ce_(12)Fe_(57.5)As_(41).A temperature-field phase diagram was present for these two rare earth systems.In addition,a logarithmic temperature dependence of electrical resistivity was observed in the two compounds within a large temperature range of 150-300 K,which is rarely found in 3D-based compounds.It may be related to Kondo scattering described by independent localized Fe 3d moments interacting with conduction electrons.展开更多
基金Supported by the National Key Research and Development Program of China(Grant Nos.2016YFA0300600 and 2018YFA0305600)the National Natural Science Foundation of China(Grant No.11974404)+1 种基金the Strategic Priority Research Program(B)of the Chinese Academy of Sciences(Grant No.XDB33000000)the Youth Innovation Promotion Association of CAS(Grant No.2017013).
文摘Magnetic topological materials have attracted much attention due to the correlation between topology and magnetism.Recent studies suggest that EuCd_(2)As_(2) is an antiferromagnetic topological material.Here by carrying out thorough magnetic,electrical and thermodynamic property measurements,we discover a long-time relaxation of the magnetic susceptibility in EuCd_(2)As_(2).The(001)in-plane magnetic susceptibility at 5 K is found to continuously increase up to∼10%over the time of∼14 hours.The magnetic relaxation is anisotropic and strongly depends on the temperature and the applied magnetic field.These results will stimulate further theoretical and experimental studies to understand the origin of the relaxation process and its effect on the electronic structure and physical properties of the magnetic topological materials.
基金Supported by the National Key Research and Development Program(2016YFA0300502,2017YFA0302901,2016YFA0300604 and 2016YFA0300501)the Strategic Priority Research Program of the Chinese Academy of Sciences(XDB28000000,XDB07020100and QYZDB-SSW-SLH043)the National Natural Science Foundation of China under Grant Nos 11421092,11574359,11674370,11774399,11474330 and U1732154
文摘The search for quantum spin liquid(QSL) materials has attracted significant attention in the field of condensed matter physics in recent years, however so far only a handful of them are considered as candidates hosting QSL ground state. Owning to their geometrically frustrated structures, Kagome materials are ideal systems to realize QSL. We synthesize the kagome structured material claringbullite(Cu_4(OH)_6FCl) and then replace inter-layer Cu with Zn to form Cu_3Zn(OH)_6FCl. Comprehensive measurements reveal that doping Zn^(2+) ions transforms magnetically ordered Cu_4(OH)_6FCl into a non-magnetic QSL candidate Cu_3Zn(OH)_6FCl. Therefore,the successful syntheses of Cu_4(OH)_6FCl and Cu_3Zn(OH)_6FCl provide not only a new platform for the study of QSL but also a novel pathway of investigating the transition between QSL and magnetically ordered systems.
基金supported by the National Basic Research Program of China(Grant No.2015CB921300)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB07020200)
文摘Superconductivity on the border of the long-range magnetic order has been discovered in Mn P under high pressures. In order to investigate the nature of the magnetic properties adjacent to the superconducting state, we performed zero-field 31 P NMR for Mn P single crystal under ambient and hydrostatic pressure of 2 GPa, respectively. Radio frequency power level was used to determine whether NMR signal originates from a helical state or not. When 2 GPa pressure was applied, the signal from helical state exists even above 160 K, while that from the ferromagnetic phase was not observed. Our NMR results indicate that the magnetic phase which is adjacent to the superconducting state is in a helical magnetic structure.
基金supported by the National Natural Science Foundation of China(Grant Nos.11674375,and 11634015)the National Basic Research Program of China(Grant Nos.2015CB921300,and 2017YFA0302901)and the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB07020200)
文摘Measurements of magnetic and transport properties were performed on needle-shaped single crystals of Ce_(12)Fe_(57.5)As_(41)and La_(12)Fe_(57.5)As_(41).The availability of a complete set of data enabled a side-by-side comparison between these two rare earth compounds.Both compounds exhibited multiple magnetic orders within 2-300 K and metamagnetic transitions at various fields.Ferromagnetic transitions with Curie temperatures of 100 and 125 K were found for Ce_(12)Fe_(57.5)As_(41)and La_(12)Fe_(57.5)As_(41),respectively,followed by antiferromagnetic type spin reorientations near Curie temperatures.The magnetic properties underwent complex evolution in the magnetic field for both compounds.An antiferromagnetic phase transition at about 60 K and 0.2 T was observed merely for Ce_(12)Fe_(57.5)As_(41).The field-induced magnetic phase transition occurred from antiferromagnetic to ferromagnetic structure.A strong magnetocrystalline anisotropy was evident from magnetization measurements of Ce_(12)Fe_(57.5)As_(41).A temperature-field phase diagram was present for these two rare earth systems.In addition,a logarithmic temperature dependence of electrical resistivity was observed in the two compounds within a large temperature range of 150-300 K,which is rarely found in 3D-based compounds.It may be related to Kondo scattering described by independent localized Fe 3d moments interacting with conduction electrons.