Two-dimensional (2D) materials generally have unusual confined electro-strong interaction in a plane and can physical and chemical properties owing to the exhibit obvious anisotropy and a significant quantum-confine...Two-dimensional (2D) materials generally have unusual confined electro-strong interaction in a plane and can physical and chemical properties owing to the exhibit obvious anisotropy and a significant quantum-confinement effect, thus showing great promise in many fields. Some 2D materials, such as graphene and MXenes, have recently exhibited extraordinary electromagnetic-wave shielding and absorbing performance, which is attributed to their special electrical behavior, large specific surface area, and low mass density. Compared with traditional microwave attenuating materials, 2D materials have several obvious inherent advantages. First, similar to other nanomaterials, 2D materials have a very large specific surface area and can provide numerous interfaces for the enhanced interfacial polarization as well as the reflection and scattering of electromagnetic waves. Second, 2D materials have a particular 2D morphology with ultrasmall thickness, which is not only beneficial for the penetration and dissipation of electromagnetic waves through the 2D nanosheets, giving rise to multiple reflections and the dissipation of electromagnetic energy, but is also conducive to the design and fabrication of various well-defined structures, such as layer-by-layer assemblies, core-shell particles, and porous foam, for broadband attenuation of electromagnetic waves. Third, owing to their good processability, 2D materials can be integrated into various multifunctional composites for multimode attenuation of electromagnetic energy. In addition to behaving as microwave reflectors and absorbers, 2D materials can act as impedance regulators and provide structural support for good impedance matching and setup of the optimal structure. Numerous studies indicate that 2D materials are among the most promising microwave attenuation materials. In view of the rapid development and enormous advancement of 2D materials in shielding and absorbing electromagnetic wave, there is a strong need to summarize the recent research results in this field for presenting a comprehensive view and providing helpful suggestions for future development.展开更多
The development of flexible capacitive pressure sensors has wide application prospects in the fields of electronic skin and intelligent wearable electronic devices,but it is still a great challenge to fabricate capaci...The development of flexible capacitive pressure sensors has wide application prospects in the fields of electronic skin and intelligent wearable electronic devices,but it is still a great challenge to fabricate capacitive sensors with high sensitivity.Few reports have considered the use of interdigital electrode structures to improve the sensitivity of capacitive pressure sensors.In this work,a new strategy for the fabrication of a high-performance capacitive flexible pressure sensor based on MXene/polyvinylpyrrolidone(PVP)by an interdigital electrode is reported.By increasing the number of interdigital electrodes and selecting the appropriate dielectric layer,the sensitivity of the capacitive sensor can be improved.The capacitive sensor based on MXene/PVP here has a high sensitivity(~1.25 kPa^(−1)),low detection limit(~0.6 Pa),wide sensing range(up to 294 kPa),fast response and recovery times(~30/15 ms)and mechanical stability of 10000 cycles.The presented sensor here can be used for various pressure detection applications,such as finger pressing,wrist pulse measuring,breathing,swallowing and speech recognition.This work provides a new method of using interdigital electrodes to fabricate a highly sensitive capacitive sensor with very promising application prospects in flexible sensors and wearable electronics.展开更多
基金This work was supported by the National Key R&D Program of China (Grant No. 2016YFE0204200), and the National Natural Science Foundation of China (NSFC, Grant Nos. 51702009 and 21771017).
文摘Two-dimensional (2D) materials generally have unusual confined electro-strong interaction in a plane and can physical and chemical properties owing to the exhibit obvious anisotropy and a significant quantum-confinement effect, thus showing great promise in many fields. Some 2D materials, such as graphene and MXenes, have recently exhibited extraordinary electromagnetic-wave shielding and absorbing performance, which is attributed to their special electrical behavior, large specific surface area, and low mass density. Compared with traditional microwave attenuating materials, 2D materials have several obvious inherent advantages. First, similar to other nanomaterials, 2D materials have a very large specific surface area and can provide numerous interfaces for the enhanced interfacial polarization as well as the reflection and scattering of electromagnetic waves. Second, 2D materials have a particular 2D morphology with ultrasmall thickness, which is not only beneficial for the penetration and dissipation of electromagnetic waves through the 2D nanosheets, giving rise to multiple reflections and the dissipation of electromagnetic energy, but is also conducive to the design and fabrication of various well-defined structures, such as layer-by-layer assemblies, core-shell particles, and porous foam, for broadband attenuation of electromagnetic waves. Third, owing to their good processability, 2D materials can be integrated into various multifunctional composites for multimode attenuation of electromagnetic energy. In addition to behaving as microwave reflectors and absorbers, 2D materials can act as impedance regulators and provide structural support for good impedance matching and setup of the optimal structure. Numerous studies indicate that 2D materials are among the most promising microwave attenuation materials. In view of the rapid development and enormous advancement of 2D materials in shielding and absorbing electromagnetic wave, there is a strong need to summarize the recent research results in this field for presenting a comprehensive view and providing helpful suggestions for future development.
基金The work was supported by the‘5G+medical and health application pilot project’approved from the Ministry of Industry and Information Technology of Chinathe National Natural Science Foundation of China(NSFC Grant No.21771017)the Fundamental Research Funds for the Central Universities(YWF-21-BJ-J-313).
文摘The development of flexible capacitive pressure sensors has wide application prospects in the fields of electronic skin and intelligent wearable electronic devices,but it is still a great challenge to fabricate capacitive sensors with high sensitivity.Few reports have considered the use of interdigital electrode structures to improve the sensitivity of capacitive pressure sensors.In this work,a new strategy for the fabrication of a high-performance capacitive flexible pressure sensor based on MXene/polyvinylpyrrolidone(PVP)by an interdigital electrode is reported.By increasing the number of interdigital electrodes and selecting the appropriate dielectric layer,the sensitivity of the capacitive sensor can be improved.The capacitive sensor based on MXene/PVP here has a high sensitivity(~1.25 kPa^(−1)),low detection limit(~0.6 Pa),wide sensing range(up to 294 kPa),fast response and recovery times(~30/15 ms)and mechanical stability of 10000 cycles.The presented sensor here can be used for various pressure detection applications,such as finger pressing,wrist pulse measuring,breathing,swallowing and speech recognition.This work provides a new method of using interdigital electrodes to fabricate a highly sensitive capacitive sensor with very promising application prospects in flexible sensors and wearable electronics.