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WS2 nanoflakes from nanotubes for electrocatalysis 被引量:11
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作者 Charina L. Choi Ju Feng +4 位作者 Yanguang Li justin wu Alia Zak Reshef Tenne Hongjie Dai 《Nano Research》 SCIE EI CAS CSCD 2013年第12期921-928,共8页
Next-generation catalysts for water splitting are crucial towards a renewable hydrogen economy. MoS2 and WS2 represent earth-abundant, noble metal cathode alternatives with high catalytic activity at edge sites. One c... Next-generation catalysts for water splitting are crucial towards a renewable hydrogen economy. MoS2 and WS2 represent earth-abundant, noble metal cathode alternatives with high catalytic activity at edge sites. One challenge in their development is to nanostructure these materials in order to achieve increased performance through the creation of additional edge sites. In this work, we demonstrate a simple route to form nanostructured-WS2 using sonochemical exfoliation to break interlayer and intralayer bonds in WS2 nanotubes. The resulting few-layer nanoflakes are -100 nm wide with a high density of edge sites. WS2 nanoflakes are utilized as cathodes for the hydrogen evolution reaction (HER) and exhibit superior performance to WS2 nanotubes and bulk particles, with a lower onset potential, shallower Tafel slope and increased current density. Future work may employ ultra-small nanoflakes, dopant atoms, or graphene hybrids to further improve electrocatalytic activity. 展开更多
关键词 tungsten disulfide NANOTUBES NANOSTRUCTURING hydrogen evolution
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