Investigating the characteristics and transformation of water-soluble carbonaceous matter in the cryosphere regions is important for understanding biogeochemical process in the earth system.Water-soluble carbonaceous ...Investigating the characteristics and transformation of water-soluble carbonaceous matter in the cryosphere regions is important for understanding biogeochemical process in the earth system.Water-soluble carbonaceous matter is a heterogeneous mixture of organic compounds that is soluble in aquatic environments.Despite its importance,we still lack systematic understanding for dissolved organic carbon(DOC)in several aspects including exact chemical composition and physical interactions with microorganisms,glacier meltwater.This review presents the chemical composition and physical properties of glacier DOC deposited through anthropogenic emission,terrestrial,and biogenic sources.We present the molecular composition of DOC and its effect over snow albedo and associated radiative forcings.Results indicate that DOC in snow/ice is made up of aromatic protein-like species,fulvic acid-like materials,and humic acid-like materials.Light-absorbing impurities in surface snow and glacier ice cause considerable albedo reduction and the associated radiative forcing is definitely positive.Water-soluble carbonaceous matter dominated the carbon transport in the high-altitude glacial area.Owing to prevailing global warming and projected increase in carbon emission,the glacial DOC is expected to release,which will have strong underlying impacts on cryosphere ecosystem.The results of this work have profound implications for better understanding the carbon cycle in high altitude cryosphere regions.A new compilation of globally distributed work is required,including large-scale measurements of glacial DOC over high-altitude cryosphere regions,to overcome and address the scientific challenges to constrain climate impacts of light-absorbing impurities related processes in Earth system and climate models.展开更多
Precipitation plays a crucial role in the water cycle of Northwest China.Obtaining accurate precipitation data is crucial for regional water resource management,hydrological forecasting,flood control and drought relie...Precipitation plays a crucial role in the water cycle of Northwest China.Obtaining accurate precipitation data is crucial for regional water resource management,hydrological forecasting,flood control and drought relief.Currently,the applicability of multi-source precipitation products for long time series in Northwest China has not been thoroughly evaluated.In this study,precipitation data from 183 meteorological stations in Northwest China from 1979 to 2020 were selected to assess the regional applicability of four precipitation products(the fifth generation of European Centre for Medium-Range Weather Forecasts(ECMWF)atmospheric reanalysis of the global climate(ERA5),Global Precipitation Climatology Centre(GPCC),Climatic Research Unit gridded Time Series Version 4.07(CRU TS v4.07,hereafter CRU),and Tropical Rainfall Measuring Mission(TRMM))based on the following statistical indicators:correlation coefficient,root mean square error(RMSE),relative bias(RB),mean absolute error(MAE),probability of detection(POD),false alarm ratio(FAR),and equitable threat score(ETS).The results showed that precipitation in Northwest China was generally high in the east and low in the west,and exhibited an increasing trend from 1979 to 2020.Compared with the station observations,ERA5 showed a larger spatial distribution difference than the other products.The overall overestimation of multi-year average precipitation was approximately 200.00 mm and the degree of overestimation increased with increasing precipitation intensity.The multi-year average precipitation of GPCC and CRU was relatively close to that of station observations.The trend of annual precipitation of TRMM was overestimated in high-altitude regions and the eastern part of Lanzhou with more precipitation.At the monthly scale,GPCC performed well but underestimated precipitation in the Tarim Basin(RB=-4.11%),while ERA5 and TRMM exhibited poor accuracy in high-altitude regions.ERA5 had a large bias(RB≥120.00%)in winter months and a strong dispersion(RMSE≥35.00 mm)in summer months.TRMM showed a relatively low correlation with station observations in winter months(correlation coefficients≤0.70).The capture performance analysis showed that ERA5,GPCC,and TRMM had lower POD and ETS values and higher FAR values in Northwest China as the precipitation intensity increased.ERA5 showed a high capture performance for small precipitation events and a slower decreasing trend of POD as the precipitation intensity increased.GPCC had the lowest FAR values.TRMM was statistically ineffective for predicting the occurrence of daily precipitation events.The findings provide a reference for data users to select appropriate datasets in Northwest China and for data developers to develop new precipitation products in the future.展开更多
Glaciers in the Pamir region are experiencing rapid melting and receding due to climate change,which has a significant implication for the Amu Darya river basin.Predominantly,surging glaciers,which undergo unpredictab...Glaciers in the Pamir region are experiencing rapid melting and receding due to climate change,which has a significant implication for the Amu Darya river basin.Predominantly,surging glaciers,which undergo unpredictable advances,are potentially leading to the obstruction of high-altitude river channels and also glacial lake outburst floods.decrease of-703.5±30.0 m.There is a substantial increase in the number(from 19 to 75)and area(from 4889.7±0.6 m2 to 15345.5±0.6 m2)of RGS lakes along with supra-glacier ponds based on a comparison of ArcGIS base map in 2011 and high-resolution UAV data in 2023.For M glacier,number of lakes increased from 4 to 22 but the lake area declined from 10715.2±0.6 to 365.6±0.6 m2.It was noted that the largest lake in 2011 with an area of 10406.4±0.6 m2 at the southeastern portion of the glacier was not observed in 2023 due to outburst.Both the glaciers have substantially impacted the river flow(Abdukahor river)by obstructing a significant proportion of river channel in recent years and might cause outburst floods.These findings enhance the understanding of glacier dynamics and their impacts on the surrounding areas,emphasizing the urgent need for continued monitoring and appropriate management strategies,with a specific focus on surging glaciers and the associated risks.展开更多
Microplastics(MPs)become ubiquitous in soil and are an environmental and public health concern worldwide.However,the status of MPs in natural and farmland soils in remote areas remains poorly understood.In this study,...Microplastics(MPs)become ubiquitous in soil and are an environmental and public health concern worldwide.However,the status of MPs in natural and farmland soils in remote areas remains poorly understood.In this study,we investigated the characteristics of MPs in natural and farmland soils along two transects in the Qilian Mountains of the northern Tibetan Plateau.The average abundance of MPs in natural and farmland soils was 29,778 and 56,123 items kg^(-1),respectively,with a detection size range of 10-1000μm.MPs in the size range of 10-100μm accounted for 84.1%of particles detected.Among the 21 polymers detected,polyethylene dominated in both farmland and natural soils.The shape of MPs was dominated by fragments(95.8%),followed by fibers(3.8%)and beads(0.4%).The abundance of MPs was positively correlated with increasing altitude in natural soils.There was no significant correlation between the abundance of MPs and soil physicochemical properties due to the narrow range of values of soil physicochemical properties.With the growing concern regarding MPs pollution,research on the status of MPs in high altitude and remote areas is critical to understanding their global cycle.展开更多
基金supported by the second Tibetan Plateau Scientific Expedition and Research Program(STEP)(2019QZKK0605)the National Natural Science Foundation of China(41971080)the support of Youth Innovation Promotion Association CAS(2021429)。
文摘Investigating the characteristics and transformation of water-soluble carbonaceous matter in the cryosphere regions is important for understanding biogeochemical process in the earth system.Water-soluble carbonaceous matter is a heterogeneous mixture of organic compounds that is soluble in aquatic environments.Despite its importance,we still lack systematic understanding for dissolved organic carbon(DOC)in several aspects including exact chemical composition and physical interactions with microorganisms,glacier meltwater.This review presents the chemical composition and physical properties of glacier DOC deposited through anthropogenic emission,terrestrial,and biogenic sources.We present the molecular composition of DOC and its effect over snow albedo and associated radiative forcings.Results indicate that DOC in snow/ice is made up of aromatic protein-like species,fulvic acid-like materials,and humic acid-like materials.Light-absorbing impurities in surface snow and glacier ice cause considerable albedo reduction and the associated radiative forcing is definitely positive.Water-soluble carbonaceous matter dominated the carbon transport in the high-altitude glacial area.Owing to prevailing global warming and projected increase in carbon emission,the glacial DOC is expected to release,which will have strong underlying impacts on cryosphere ecosystem.The results of this work have profound implications for better understanding the carbon cycle in high altitude cryosphere regions.A new compilation of globally distributed work is required,including large-scale measurements of glacial DOC over high-altitude cryosphere regions,to overcome and address the scientific challenges to constrain climate impacts of light-absorbing impurities related processes in Earth system and climate models.
基金supported by the National Key Research and Development Program of China(2023YFC3206300)the National Natural Science Foundation of China(42477529,42371145,42261026)+2 种基金the China-Pakistan Joint Program of the Chinese Academy of Sciences(046GJHZ2023069MI)the Gansu Provincial Science and Technology Program(22ZD6FA005)the National Cryosphere Desert Data Center(E01Z790201).
文摘Precipitation plays a crucial role in the water cycle of Northwest China.Obtaining accurate precipitation data is crucial for regional water resource management,hydrological forecasting,flood control and drought relief.Currently,the applicability of multi-source precipitation products for long time series in Northwest China has not been thoroughly evaluated.In this study,precipitation data from 183 meteorological stations in Northwest China from 1979 to 2020 were selected to assess the regional applicability of four precipitation products(the fifth generation of European Centre for Medium-Range Weather Forecasts(ECMWF)atmospheric reanalysis of the global climate(ERA5),Global Precipitation Climatology Centre(GPCC),Climatic Research Unit gridded Time Series Version 4.07(CRU TS v4.07,hereafter CRU),and Tropical Rainfall Measuring Mission(TRMM))based on the following statistical indicators:correlation coefficient,root mean square error(RMSE),relative bias(RB),mean absolute error(MAE),probability of detection(POD),false alarm ratio(FAR),and equitable threat score(ETS).The results showed that precipitation in Northwest China was generally high in the east and low in the west,and exhibited an increasing trend from 1979 to 2020.Compared with the station observations,ERA5 showed a larger spatial distribution difference than the other products.The overall overestimation of multi-year average precipitation was approximately 200.00 mm and the degree of overestimation increased with increasing precipitation intensity.The multi-year average precipitation of GPCC and CRU was relatively close to that of station observations.The trend of annual precipitation of TRMM was overestimated in high-altitude regions and the eastern part of Lanzhou with more precipitation.At the monthly scale,GPCC performed well but underestimated precipitation in the Tarim Basin(RB=-4.11%),while ERA5 and TRMM exhibited poor accuracy in high-altitude regions.ERA5 had a large bias(RB≥120.00%)in winter months and a strong dispersion(RMSE≥35.00 mm)in summer months.TRMM showed a relatively low correlation with station observations in winter months(correlation coefficients≤0.70).The capture performance analysis showed that ERA5,GPCC,and TRMM had lower POD and ETS values and higher FAR values in Northwest China as the precipitation intensity increased.ERA5 showed a high capture performance for small precipitation events and a slower decreasing trend of POD as the precipitation intensity increased.GPCC had the lowest FAR values.TRMM was statistically ineffective for predicting the occurrence of daily precipitation events.The findings provide a reference for data users to select appropriate datasets in Northwest China and for data developers to develop new precipitation products in the future.
基金funded by the Gansu Provincial Science and Technology Program(22ZD6FA005)Gansu Postdoctoral Science Foundation(Grant number-E339880204)。
文摘Glaciers in the Pamir region are experiencing rapid melting and receding due to climate change,which has a significant implication for the Amu Darya river basin.Predominantly,surging glaciers,which undergo unpredictable advances,are potentially leading to the obstruction of high-altitude river channels and also glacial lake outburst floods.decrease of-703.5±30.0 m.There is a substantial increase in the number(from 19 to 75)and area(from 4889.7±0.6 m2 to 15345.5±0.6 m2)of RGS lakes along with supra-glacier ponds based on a comparison of ArcGIS base map in 2011 and high-resolution UAV data in 2023.For M glacier,number of lakes increased from 4 to 22 but the lake area declined from 10715.2±0.6 to 365.6±0.6 m2.It was noted that the largest lake in 2011 with an area of 10406.4±0.6 m2 at the southeastern portion of the glacier was not observed in 2023 due to outburst.Both the glaciers have substantially impacted the river flow(Abdukahor river)by obstructing a significant proportion of river channel in recent years and might cause outburst floods.These findings enhance the understanding of glacier dynamics and their impacts on the surrounding areas,emphasizing the urgent need for continued monitoring and appropriate management strategies,with a specific focus on surging glaciers and the associated risks.
基金financial support from the National Natural Science Foundation of China(42322105,42071082)Outstanding Youth Fund of Gansu Province(23JRRA612)。
文摘Microplastics(MPs)become ubiquitous in soil and are an environmental and public health concern worldwide.However,the status of MPs in natural and farmland soils in remote areas remains poorly understood.In this study,we investigated the characteristics of MPs in natural and farmland soils along two transects in the Qilian Mountains of the northern Tibetan Plateau.The average abundance of MPs in natural and farmland soils was 29,778 and 56,123 items kg^(-1),respectively,with a detection size range of 10-1000μm.MPs in the size range of 10-100μm accounted for 84.1%of particles detected.Among the 21 polymers detected,polyethylene dominated in both farmland and natural soils.The shape of MPs was dominated by fragments(95.8%),followed by fibers(3.8%)and beads(0.4%).The abundance of MPs was positively correlated with increasing altitude in natural soils.There was no significant correlation between the abundance of MPs and soil physicochemical properties due to the narrow range of values of soil physicochemical properties.With the growing concern regarding MPs pollution,research on the status of MPs in high altitude and remote areas is critical to understanding their global cycle.
