Analyzing gene network structure is an important way to discover and understand some unknown relevant functions and regulatory mechanisms of organism at the molecular level. In this work, mutual information networks a...Analyzing gene network structure is an important way to discover and understand some unknown relevant functions and regulatory mechanisms of organism at the molecular level. In this work, mutual information networks and Boolean logic networks are constructed using the methods of reverse modeling based on gene expression profiles in lung tissues with and without cancer. The comparison of these network structures shows that average degree, the proportion of non-isolated nodes, average betweenness and average coreness can distinguish the networks corresponding to the lung tissues with and without cancer. According to the difference of degree, betweenness and coreness of each gene in these networks, nine structural key genes are obtained. Seven of them which are related to lung cancer are supported by literatures. The remaining two genes AKT1 and RBL may have important roles in the formation, development and metastasis of lung cancer. Furthermore, the contrast of these logic networks suggests that the distributions of logic types are obviously different. The structural differences can help us to understand the mechanism of formation and development of lung cancer.展开更多
The exfoliation of bulk 2H-molybdenum disulfide(2H-MoS_(2))into few-layer nanosheets with 1T-phase and controlled layers represents a daunting challenge towards the device applications of MoS_(2).Conventional ion inte...The exfoliation of bulk 2H-molybdenum disulfide(2H-MoS_(2))into few-layer nanosheets with 1T-phase and controlled layers represents a daunting challenge towards the device applications of MoS_(2).Conventional ion intercalation assisted exfoliation needs the use of hazardous n-butyllithium and/or elaborate control of the intercalation potential to avoid the decomposition of the MoS_(2).This work reports a facile strategy by intercalating Li ions electrochemically with ether-based electrolyte into the van der Waals(vdW)channels of MoS_(2),which successfully avoids the decomposition of MoS_(2)at low potentials.The co-intercalation of Li+and the ether solvent into MoS_(2)makes a first-order phase transformation,forming a superlattice phase,which preserves the layered structure and hence enables the exfoliation of bulk 2H-MoS_(2)into bilayer nanosheets with 1T-phase.Compared with the pristine 2H-MoS_(2),the bilayer 1T-MoS_(2)nanosheets exhibit better electrocatalytic performance for the hydrogen evolution reaction(HER).This facile method should be easily extended to the exfoliation of various transition metal dichalcogenides(TMDs).展开更多
NIST(National Institute of Standards and Technology) statistical test recognized as the most authoritative is widely used in verifying the randomness of binary sequences. The Non-overlapping Template Matching Test as ...NIST(National Institute of Standards and Technology) statistical test recognized as the most authoritative is widely used in verifying the randomness of binary sequences. The Non-overlapping Template Matching Test as the 7 th test of the NIST Test Suit is remarkably time consuming and the slow performance is one of the major hurdles in the testing process. In this paper, we present an efficient bit-parallel matching algorithm and segmented scan-based strategy for execution on Graphics Processing Unit(GPU) using NVIDIA Compute Unified Device Architecture(CUDA). Experimental results show the significant performance improvement of the parallelized Non-overlapping Template Matching Test, the running speed is 483 times faster than the original NIST implementation without attenuating the test result accuracy.展开更多
MXene is a new type of layered two-dimensional transition metal carbide materials differing from graphene, demonstrating intriguing chemical/physical properties. Here the chemical modification of MXene and next fabric...MXene is a new type of layered two-dimensional transition metal carbide materials differing from graphene, demonstrating intriguing chemical/physical properties. Here the chemical modification of MXene and next fabrication of core-shell MXene-COOH@(PEI/PAA)_n composites have been investigated. The obtained MXene-based composites were treated with gold nanoparticles to form MXene—COOH@(PEI/PAA)_n@AuNPs nanocomposites, and their catalytic properties for nitro-compounds were studied. The prepared nanocomposites demonstrated good catalytic activity and reproducibility, showing potential applications in composite catalysts and environmental fields.展开更多
Learning hydrophobic phenomena from nature is always a promising approach to design the superhydrophobic surface.Purple orchid leaf which processes superhydrophobicity is an ideal plant model,and through mimicking its...Learning hydrophobic phenomena from nature is always a promising approach to design the superhydrophobic surface.Purple orchid leaf which processes superhydrophobicity is an ideal plant model,and through mimicking its structure,the surface with excellent hydrophobicity is able to be obtained.However,the unclear of the diversity in wettability during the different vegetation stages and the absence of its relation to the surface morphology limits the further enhancement of the inspired structure.Here,we analyze the wettability difference as the leaf grows from tender to mature and then to senescent.Combining with the variation of surface morphology and chemical composition,the well-developed micro-scale basic unit bumps with dense nano-scale waxy layer on the surface are proven to be responsible for the best hydrophobicity of the mature leaf.The presence of the undeveloped or damaged micro-nano hierarchical structure reduces the formation of air pockets at the interface,leading to the decrease of the wettability for leaves at other stages.Moreover,by fabricating artificial leaves,the nano-waxy layer is proved to be more effective than that of the micro-bumps on the surface wettability.The results of study are of a great significance for guiding the design and fabrication of plant-inspired bionic superhydrophobic surface.展开更多
Electrochemical lithiation/delithiation of electrodes induces chemical strain cycling that causes fatigue and other harmful influences on lithium-ion batteries.In this work,a homemade in situ measurement device was us...Electrochemical lithiation/delithiation of electrodes induces chemical strain cycling that causes fatigue and other harmful influences on lithium-ion batteries.In this work,a homemade in situ measurement device was used to characterize simultaneously chemical strain and nominal state of charge,especially residual chemical strain and residual nominal state of charge,in graphite-based electrodes at various temperatures.The measurements indicate that raising the testing temperature from 20℃ to 60℃ decreases the chemical strain at the same nominal state of charge during cycling,while residual chemical strain and residual nominal state of charge increase with the increase of temperature.Furthermore,a novel electrochemicalmechanical model is developed to evaluate quantitatively the chemical strain caused by a solid electrolyte interface(SEI)and the partial molar volume of Li in the SEI at different temperatures.The present study will definitely stimulate future investigations on the electro-chemo-mechanics coupling behaviors in lithium-ion batteries.展开更多
Electrochemical lithiation/delithiation of electrodes induces chemical strain cycling that causes fatigue and other harmful influences on lithium-ion batteries.In this work,a homemade in situ measurement device was us...Electrochemical lithiation/delithiation of electrodes induces chemical strain cycling that causes fatigue and other harmful influences on lithium-ion batteries.In this work,a homemade in situ measurement device was used to characterize simultaneously chemical strain and nominal state of charge,especially residual chemical strain and residual nominal state of charge,in graphite-based electrodes at various temperatures.The measurements indicate that raising the testing temperature from 20℃ to 60℃ decreases the chemical strain at the same nominal state of charge during cycling,while residual chemical strain and residual nominal state of charge increase with the increase of temperature.Furthermore,a novel electrochemicalmechanical model is developed to evaluate quantitatively the chemical strain caused by a solid electrolyte interface(SEI)and the partial molar volume of Li in the SEI at different temperatures.The present study will definitely stimulate future investigations on the electro-chemo-mechanics coupling behaviors in lithium-ion batteries.展开更多
Surgical electrodes rely on thermal effect of high-frequency current and are a widely used medical tool for cutting and coagulating biological tissue.However,tissue adhesion on the electrode surface and thermal injury...Surgical electrodes rely on thermal effect of high-frequency current and are a widely used medical tool for cutting and coagulating biological tissue.However,tissue adhesion on the electrode surface and thermal injury to adjacent tissue are serious problems in surgery that can affect cutting performance.A bionic microstriped structure mimicking a banana leaf was constructed on the electrode via nanosecond laser surface texturing,followed by silanization treatment,to enhance lyophobicity.The effect of initial,simple grid-textured,and bionic electrodes with different wettabilities on tissue adhesion and thermal injury were investigated using horizontal and vertical cutting modes.Results showed that the bionic electrode with high lyophobicity can effectively reduce tissue adhesion mass and thermal injury depth/area compared with the initial electrode.The formation mechanism of adhered tissue was discussed in terms of morphological features,and the potential mechanism for antiadhesion and heat dissipation of the bionic electrode was revealed.Furthermore,we evaluated the influence of groove depth on tissue adhesion and thermal injury and then verified the antiadhesion stability of the bionic electrode.This study demonstrates a promising approach for improving the cutting performance of surgical electrodes.展开更多
The Furongian Series of the Cambrian in the Tarim Craton(NW China)is mainly composed of crystalline dolostones,and is an important target for oil and gas exploration.The chronostratigraphic framework of the Furongian ...The Furongian Series of the Cambrian in the Tarim Craton(NW China)is mainly composed of crystalline dolostones,and is an important target for oil and gas exploration.The chronostratigraphic framework of the Furongian Series in the Tarim Craton has not yet been established due to the scarcity of fossils and the absence of the Steptoean Positive Carbon Isotope Excursion(SPICE),which is the primary global carbon isotope excursion of the Furongian Series.In this study,the SPICE was discovered by examining the carbon isotopes of the representative drilling wells in the West Platform and East Basin.A positive carbon isotope anomaly withδ13C values ranging from 1.5‰to 1.9‰(PDB),were found in the middle of the Xiaqiulitag Formation of the three drilling wells in the West Platform,and a positive excursion withδ13C values up to 4.0‰(PDB),which is correlated with the SPICE,was found in the lower limestone of the Tuershaketag Formation in the East Basin.Based on the carbon isotopic data and chemostratigraphic correlation,the chronostratigraphic framework of the Furongian Series across different facies in the Tarim Craton is preliminarily established.The basal boundary of the Furongian Series was preliminarily defined by the occurrence of the SPICE.Aweak positive anomaly ofδ13C was observed at the base of the Penglaiba Formation of the three boreholes in the West Platform and the top of the Tuershaketag Formation of Tadong-2 well.We propose that the positive anomaly of the carbon isotope above the weak negative anomaly at the base of the Penglaiba Formation and the top of the Tuershaketag Formation can be used to define the Cambrian-Ordovician boundary in the Tarim Craton.展开更多
The sandstone of the third member of the Funing Formation(E1f3)in the northern slope zone of the Gaoyou Sag has the typical characteristics of high porosity and ultralow permeability,which makes it difficult for oil t...The sandstone of the third member of the Funing Formation(E1f3)in the northern slope zone of the Gaoyou Sag has the typical characteristics of high porosity and ultralow permeability,which makes it difficult for oil to flow.In this study,the lithological characteristics,sedimentary facies,diagenetic characteristics,pore struc-ture,and seepage ability of this sandstone are characterized in detail.Correlation analysis is used to reveal the reason for the sandstone high porosity-low permeability phenom-enon in the study area.The results indicate that this phenomenon is controlled mainly by the following three factors:1)the sedimentary environment is the initial affecting factor,whereby the deposition of a large number of fine-grained materials reduces the primary pores of sandstone.2)The Funing Formation has undergone strong compaction and cementation,which have led to the removal of most of the primary pores and a reduction in size of the throat channels.3)Owing to fluid activity during the later stage of diagenesis,sandstone underwent intense dissolution and a large number of particles(feldspar and lithic debris)formed many dissolution pores(accounting for nearly 60%of the total pore space).Among these factors,dissolution has contributed the most to the development of high porosity-low permeability phenomenon.This is mainly attributed to the inhomogeneous dissolution process,whereby the degree of particle dissolution(e.g.feldspar)exceeds that of cementing minerals(clay and carbonate minerals).The secondary dissolution pores have increased the porosity of sandstone in the study area;however,the pore connectivity(permeability)has not been significantly improved,thus resulting in the special high porosity-low permeability characteristics of this sandstone.展开更多
Carbon-based material has been regarded as one of the most promising electrode materials for potassium-ion batteries(PIBs).However,the battery performance based on reported porous carbon electrodes is still unsatisfac...Carbon-based material has been regarded as one of the most promising electrode materials for potassium-ion batteries(PIBs).However,the battery performance based on reported porous carbon electrodes is still unsatisfactory,while the in-depth K-ion storage mechanism remains relatively ambiguous.Herein,we propose a facile“in situ self-template bubbling”method for synthesizing interlayer-tuned hierarchically porous carbon with different metallic ions,which delivers superior K-ion storage performance,especially the high reversible capacity(360.6 mAh·g^(−1)@0.05 A·g^(−1)),excellent rate capability(158.6 mAh·g^(−1)@10.0 A·g^(−1))and ultralong high-rate cycling stability(82.8%capacity retention after 2,000 cycles at 5.0 A·g^(−1)).Theoretical simulation reveals the correlations between interlayer distance and K-ion diffusion kinetics.Experimentally,deliberately designed consecutive cyclic voltammetry(CV)measurements,ex situ Raman tests,galvanostatic intermittent titration technique(GITT)method decipher the origin of the excellent rate performance by disentangling the synergistic effect of interlayer and pore-structure engineering.Considering the facile preparation strategy,superior electrochemical performance and insightful mechanism investigations,this work may deepen the fundamental understandings of carbon-based PIBs and related energy storage devices like sodium-ion batteries,aluminum-ion batteries,electrochemical capacitors,and dual-ion batteries.展开更多
Solar energy has attracted a lot of attention because it is clean and has no pollution.However,due to the partially shaded condition,the photovoltaic array cannot work uniformly at the maximum power point,resulting in...Solar energy has attracted a lot of attention because it is clean and has no pollution.However,due to the partially shaded condition,the photovoltaic array cannot work uniformly at the maximum power point,resulting in a large power loss.To improve this problem,the research of the maximum power point tracking(MPPT)algorithm is discussed by scholars.In this paper,an improved particle swarm optimization(PSO)algorithm is proposed to achieve the goal of MPPT,which uses Newton interpolation-assisted conventional PSO.After tracking to the maximum power point,the Newton interpolation method is used to calculate the maximum power point,reduce the number of iterations of the conventional PSO algorithm and reduce the steady-state oscillation.The simulation is carried out in MATLAB^(■)/Simulink^(■)and compared with conventional PSO.The results show that the improved PSO has better tracking ac-curacy and speed than the conventional algorithm,and the initial tracking speed is increased by>30%.展开更多
ZnO films containing Er and Ge nanocrystals(nc-Ge) were synthesized and their photoluminescence(PL) properties were studied. Visible and near-infrared PL intensities are found to be greatly increased in nc-Ge-containi...ZnO films containing Er and Ge nanocrystals(nc-Ge) were synthesized and their photoluminescence(PL) properties were studied. Visible and near-infrared PL intensities are found to be greatly increased in nc-Ge-containing film. Er-related 1.54 μm emission has been investigated under several excitation conditions upon different kinds of Ge, Er codoped ZnO thin films. 1.54 μm PL enhancement accompanied by the appearance of nc-Ge implies a significant correlation between nc-Ge and PL emission of Er^(3+). The increased intensity of 1.54 μm in Ge:Er:ZnO film is considered to come from the joint effect of the local potential distortion around Er^(3+)and the possibleenergy transfer from nc-Ge to Er^(3+).展开更多
文摘Analyzing gene network structure is an important way to discover and understand some unknown relevant functions and regulatory mechanisms of organism at the molecular level. In this work, mutual information networks and Boolean logic networks are constructed using the methods of reverse modeling based on gene expression profiles in lung tissues with and without cancer. The comparison of these network structures shows that average degree, the proportion of non-isolated nodes, average betweenness and average coreness can distinguish the networks corresponding to the lung tissues with and without cancer. According to the difference of degree, betweenness and coreness of each gene in these networks, nine structural key genes are obtained. Seven of them which are related to lung cancer are supported by literatures. The remaining two genes AKT1 and RBL may have important roles in the formation, development and metastasis of lung cancer. Furthermore, the contrast of these logic networks suggests that the distributions of logic types are obviously different. The structural differences can help us to understand the mechanism of formation and development of lung cancer.
基金the National Natural Science Foundation of China(No.12374003)the Guangdong Basic and Applied Basic Research Foundation(No.2022A1515012349)+1 种基金the Shenzhen Science and Technology Program(Nos.RCBS20200714114920129 and JCYJ20220531095208019)the Guangzhou Municipal Science and Technology Project(No.2023A03J0003).
文摘The exfoliation of bulk 2H-molybdenum disulfide(2H-MoS_(2))into few-layer nanosheets with 1T-phase and controlled layers represents a daunting challenge towards the device applications of MoS_(2).Conventional ion intercalation assisted exfoliation needs the use of hazardous n-butyllithium and/or elaborate control of the intercalation potential to avoid the decomposition of the MoS_(2).This work reports a facile strategy by intercalating Li ions electrochemically with ether-based electrolyte into the van der Waals(vdW)channels of MoS_(2),which successfully avoids the decomposition of MoS_(2)at low potentials.The co-intercalation of Li+and the ether solvent into MoS_(2)makes a first-order phase transformation,forming a superlattice phase,which preserves the layered structure and hence enables the exfoliation of bulk 2H-MoS_(2)into bilayer nanosheets with 1T-phase.Compared with the pristine 2H-MoS_(2),the bilayer 1T-MoS_(2)nanosheets exhibit better electrocatalytic performance for the hydrogen evolution reaction(HER).This facile method should be easily extended to the exfoliation of various transition metal dichalcogenides(TMDs).
基金supported in part by Shanxi Scholarship Council of China(Grant No.2017-key-2)the Natural Science Foundation of Shanxi Province(Grant No.201801D121145)+1 种基金the Natural Science Foundation of China(NSFC)(Grant No.61731014,61705157,61927811)the Program for Guangdong Introducing Innovative and Entrepreneurial Teams。
文摘NIST(National Institute of Standards and Technology) statistical test recognized as the most authoritative is widely used in verifying the randomness of binary sequences. The Non-overlapping Template Matching Test as the 7 th test of the NIST Test Suit is remarkably time consuming and the slow performance is one of the major hurdles in the testing process. In this paper, we present an efficient bit-parallel matching algorithm and segmented scan-based strategy for execution on Graphics Processing Unit(GPU) using NVIDIA Compute Unified Device Architecture(CUDA). Experimental results show the significant performance improvement of the parallelized Non-overlapping Template Matching Test, the running speed is 483 times faster than the original NIST implementation without attenuating the test result accuracy.
基金financially supported by the National Natural Science Foundation of China (Nos.21473153 and 51771162)Support Program for the Top Young Talents of Hebei Province,China Postdoctoral Science Foundation (No.2015M580214)+1 种基金the Scientific and Technological Research and Development Program of Qinhuangdao City (No.201701B004)Undergraduate Training Programs for Innovation and Entrepreneurship of Yanshan University (No.CXXL2017227)
文摘MXene is a new type of layered two-dimensional transition metal carbide materials differing from graphene, demonstrating intriguing chemical/physical properties. Here the chemical modification of MXene and next fabrication of core-shell MXene-COOH@(PEI/PAA)_n composites have been investigated. The obtained MXene-based composites were treated with gold nanoparticles to form MXene—COOH@(PEI/PAA)_n@AuNPs nanocomposites, and their catalytic properties for nitro-compounds were studied. The prepared nanocomposites demonstrated good catalytic activity and reproducibility, showing potential applications in composite catalysts and environmental fields.
基金This work was financially supported by the National Key R&D Program of China(Grant No.2020YFB1711300)the National Natural Science Foundation of China(Grant No.52275425)the Natural Science Foundation of Guangdong Province for Distinguished Young Scholars(Grant No.2021B1515020087).
文摘Learning hydrophobic phenomena from nature is always a promising approach to design the superhydrophobic surface.Purple orchid leaf which processes superhydrophobicity is an ideal plant model,and through mimicking its structure,the surface with excellent hydrophobicity is able to be obtained.However,the unclear of the diversity in wettability during the different vegetation stages and the absence of its relation to the surface morphology limits the further enhancement of the inspired structure.Here,we analyze the wettability difference as the leaf grows from tender to mature and then to senescent.Combining with the variation of surface morphology and chemical composition,the well-developed micro-scale basic unit bumps with dense nano-scale waxy layer on the surface are proven to be responsible for the best hydrophobicity of the mature leaf.The presence of the undeveloped or damaged micro-nano hierarchical structure reduces the formation of air pockets at the interface,leading to the decrease of the wettability for leaves at other stages.Moreover,by fabricating artificial leaves,the nano-waxy layer is proved to be more effective than that of the micro-bumps on the surface wettability.The results of study are of a great significance for guiding the design and fabrication of plant-inspired bionic superhydrophobic surface.
基金supported by research grants from the National Key R&D Program of China(No.2017YFB0701604)Guangdong Basic and Applied Basic Research Foundation(No.2020A1515110798)+1 种基金Shenzhen Science and Technology Program(Grant No.RCBS20200714114920129)S.Sun also acknowledges the National Natural Science Foundation of China(Grant Nos.11672168 and 12072179)for financial support.
文摘Electrochemical lithiation/delithiation of electrodes induces chemical strain cycling that causes fatigue and other harmful influences on lithium-ion batteries.In this work,a homemade in situ measurement device was used to characterize simultaneously chemical strain and nominal state of charge,especially residual chemical strain and residual nominal state of charge,in graphite-based electrodes at various temperatures.The measurements indicate that raising the testing temperature from 20℃ to 60℃ decreases the chemical strain at the same nominal state of charge during cycling,while residual chemical strain and residual nominal state of charge increase with the increase of temperature.Furthermore,a novel electrochemicalmechanical model is developed to evaluate quantitatively the chemical strain caused by a solid electrolyte interface(SEI)and the partial molar volume of Li in the SEI at different temperatures.The present study will definitely stimulate future investigations on the electro-chemo-mechanics coupling behaviors in lithium-ion batteries.
基金supported by research grants from the National Key R&D Program of China(No.2017YFB0701604)Guangdong Basic and Applied Basic Research Foundation(No.2020A1515110798)+1 种基金Shenzhen Science and Technology Program(Grant No.RCBS20200714114920129)S.Sun also acknowledges the National Natural Science Foundation of China(Grant Nos.11672168 and 12072179)for financial support.
文摘Electrochemical lithiation/delithiation of electrodes induces chemical strain cycling that causes fatigue and other harmful influences on lithium-ion batteries.In this work,a homemade in situ measurement device was used to characterize simultaneously chemical strain and nominal state of charge,especially residual chemical strain and residual nominal state of charge,in graphite-based electrodes at various temperatures.The measurements indicate that raising the testing temperature from 20℃ to 60℃ decreases the chemical strain at the same nominal state of charge during cycling,while residual chemical strain and residual nominal state of charge increase with the increase of temperature.Furthermore,a novel electrochemicalmechanical model is developed to evaluate quantitatively the chemical strain caused by a solid electrolyte interface(SEI)and the partial molar volume of Li in the SEI at different temperatures.The present study will definitely stimulate future investigations on the electro-chemo-mechanics coupling behaviors in lithium-ion batteries.
基金supported by the National Key R&D Program of China (Grant No.2019YFE0126300)the Natural Science Foundation of Guangdong Province,China (Grant Nos.2019A1515011530 and 2021B1515020087).
文摘Surgical electrodes rely on thermal effect of high-frequency current and are a widely used medical tool for cutting and coagulating biological tissue.However,tissue adhesion on the electrode surface and thermal injury to adjacent tissue are serious problems in surgery that can affect cutting performance.A bionic microstriped structure mimicking a banana leaf was constructed on the electrode via nanosecond laser surface texturing,followed by silanization treatment,to enhance lyophobicity.The effect of initial,simple grid-textured,and bionic electrodes with different wettabilities on tissue adhesion and thermal injury were investigated using horizontal and vertical cutting modes.Results showed that the bionic electrode with high lyophobicity can effectively reduce tissue adhesion mass and thermal injury depth/area compared with the initial electrode.The formation mechanism of adhered tissue was discussed in terms of morphological features,and the potential mechanism for antiadhesion and heat dissipation of the bionic electrode was revealed.Furthermore,we evaluated the influence of groove depth on tissue adhesion and thermal injury and then verified the antiadhesion stability of the bionic electrode.This study demonstrates a promising approach for improving the cutting performance of surgical electrodes.
基金supported by the School Research Startup Expenses of Harbin Institute of Technology(Shenzhen)(DD29100027)the National Natural Science Foundation of China(52002094)+2 种基金China Postdoctoral Science Foundation(2019M661276)Guangdong Basic and AppliedBasic Research Foundation(2019A1515110756)the High-level Talents Discipline Construction Fund of Shandong University(31370089963078)。
基金supported by the National Science and Technology Major Project(Grant Nos.2016ZX05004-004&2017ZX05008-005)。
文摘The Furongian Series of the Cambrian in the Tarim Craton(NW China)is mainly composed of crystalline dolostones,and is an important target for oil and gas exploration.The chronostratigraphic framework of the Furongian Series in the Tarim Craton has not yet been established due to the scarcity of fossils and the absence of the Steptoean Positive Carbon Isotope Excursion(SPICE),which is the primary global carbon isotope excursion of the Furongian Series.In this study,the SPICE was discovered by examining the carbon isotopes of the representative drilling wells in the West Platform and East Basin.A positive carbon isotope anomaly withδ13C values ranging from 1.5‰to 1.9‰(PDB),were found in the middle of the Xiaqiulitag Formation of the three drilling wells in the West Platform,and a positive excursion withδ13C values up to 4.0‰(PDB),which is correlated with the SPICE,was found in the lower limestone of the Tuershaketag Formation in the East Basin.Based on the carbon isotopic data and chemostratigraphic correlation,the chronostratigraphic framework of the Furongian Series across different facies in the Tarim Craton is preliminarily established.The basal boundary of the Furongian Series was preliminarily defined by the occurrence of the SPICE.Aweak positive anomaly ofδ13C was observed at the base of the Penglaiba Formation of the three boreholes in the West Platform and the top of the Tuershaketag Formation of Tadong-2 well.We propose that the positive anomaly of the carbon isotope above the weak negative anomaly at the base of the Penglaiba Formation and the top of the Tuershaketag Formation can be used to define the Cambrian-Ordovician boundary in the Tarim Craton.
文摘The sandstone of the third member of the Funing Formation(E1f3)in the northern slope zone of the Gaoyou Sag has the typical characteristics of high porosity and ultralow permeability,which makes it difficult for oil to flow.In this study,the lithological characteristics,sedimentary facies,diagenetic characteristics,pore struc-ture,and seepage ability of this sandstone are characterized in detail.Correlation analysis is used to reveal the reason for the sandstone high porosity-low permeability phenom-enon in the study area.The results indicate that this phenomenon is controlled mainly by the following three factors:1)the sedimentary environment is the initial affecting factor,whereby the deposition of a large number of fine-grained materials reduces the primary pores of sandstone.2)The Funing Formation has undergone strong compaction and cementation,which have led to the removal of most of the primary pores and a reduction in size of the throat channels.3)Owing to fluid activity during the later stage of diagenesis,sandstone underwent intense dissolution and a large number of particles(feldspar and lithic debris)formed many dissolution pores(accounting for nearly 60%of the total pore space).Among these factors,dissolution has contributed the most to the development of high porosity-low permeability phenomenon.This is mainly attributed to the inhomogeneous dissolution process,whereby the degree of particle dissolution(e.g.feldspar)exceeds that of cementing minerals(clay and carbonate minerals).The secondary dissolution pores have increased the porosity of sandstone in the study area;however,the pore connectivity(permeability)has not been significantly improved,thus resulting in the special high porosity-low permeability characteristics of this sandstone.
基金This work was supported by School Research Startup Expenses of Harbin Institute of Technology(Shenzhen)(No.DD29100027)the National Natural Science Foundation of China(No.52002094)+2 种基金Guangdong Basic and Applied Basic Research Foundation(No.2019A1515110756)China Postdoctoral Science Foundation(No.2019M661276)High-level Talents’Discipline Construction Fund of Shandong University(No.31370089963078).
文摘Carbon-based material has been regarded as one of the most promising electrode materials for potassium-ion batteries(PIBs).However,the battery performance based on reported porous carbon electrodes is still unsatisfactory,while the in-depth K-ion storage mechanism remains relatively ambiguous.Herein,we propose a facile“in situ self-template bubbling”method for synthesizing interlayer-tuned hierarchically porous carbon with different metallic ions,which delivers superior K-ion storage performance,especially the high reversible capacity(360.6 mAh·g^(−1)@0.05 A·g^(−1)),excellent rate capability(158.6 mAh·g^(−1)@10.0 A·g^(−1))and ultralong high-rate cycling stability(82.8%capacity retention after 2,000 cycles at 5.0 A·g^(−1)).Theoretical simulation reveals the correlations between interlayer distance and K-ion diffusion kinetics.Experimentally,deliberately designed consecutive cyclic voltammetry(CV)measurements,ex situ Raman tests,galvanostatic intermittent titration technique(GITT)method decipher the origin of the excellent rate performance by disentangling the synergistic effect of interlayer and pore-structure engineering.Considering the facile preparation strategy,superior electrochemical performance and insightful mechanism investigations,this work may deepen the fundamental understandings of carbon-based PIBs and related energy storage devices like sodium-ion batteries,aluminum-ion batteries,electrochemical capacitors,and dual-ion batteries.
基金supported by a grant from the Science and Technology Research Project of Jilin Provincial Department of Education(no.JJKH20210260KJ).
文摘Solar energy has attracted a lot of attention because it is clean and has no pollution.However,due to the partially shaded condition,the photovoltaic array cannot work uniformly at the maximum power point,resulting in a large power loss.To improve this problem,the research of the maximum power point tracking(MPPT)algorithm is discussed by scholars.In this paper,an improved particle swarm optimization(PSO)algorithm is proposed to achieve the goal of MPPT,which uses Newton interpolation-assisted conventional PSO.After tracking to the maximum power point,the Newton interpolation method is used to calculate the maximum power point,reduce the number of iterations of the conventional PSO algorithm and reduce the steady-state oscillation.The simulation is carried out in MATLAB^(■)/Simulink^(■)and compared with conventional PSO.The results show that the improved PSO has better tracking ac-curacy and speed than the conventional algorithm,and the initial tracking speed is increased by>30%.
基金National Natural Science Foundation of China(NSFC)(11475105)
文摘ZnO films containing Er and Ge nanocrystals(nc-Ge) were synthesized and their photoluminescence(PL) properties were studied. Visible and near-infrared PL intensities are found to be greatly increased in nc-Ge-containing film. Er-related 1.54 μm emission has been investigated under several excitation conditions upon different kinds of Ge, Er codoped ZnO thin films. 1.54 μm PL enhancement accompanied by the appearance of nc-Ge implies a significant correlation between nc-Ge and PL emission of Er^(3+). The increased intensity of 1.54 μm in Ge:Er:ZnO film is considered to come from the joint effect of the local potential distortion around Er^(3+)and the possibleenergy transfer from nc-Ge to Er^(3+).