In a Dirac semimetal, the massless Dirac fermion has zero chirality, leading to surface states connected adiabatically to a topologically trivial surface state as well as vanishing anomalous Hall effect. Recently, it ...In a Dirac semimetal, the massless Dirac fermion has zero chirality, leading to surface states connected adiabatically to a topologically trivial surface state as well as vanishing anomalous Hall effect. Recently, it is predicted that in the nonrelativistic limit of certain collinear antiferromagnets, there exists a type of chiral“Dirac-like” fermion, whose dispersion manifests four-fold degenerate crossing points formed by spin-degenerate linear bands, with topologically protected Fermi arcs. Such an unconventional chiral fermion, protected by a hidden SU(2) symmetry in the hierarchy of an enhanced crystallographic group, namely spin space group, is not experimentally verified yet. Here, by angle-resolved photoemission spectroscopy measurements, we reveal the surface origin of the electron pocket at the Fermi surface in collinear antiferromagnet CoNb3S6. Combining with neutron diffraction and first-principles calculations, we suggest a multidomain collinear antiferromagnetic configuration, rendering the the existence of the Fermi-arc surface states induced by chiral Dirac-like fermions.Our work provides spectral evidence of the chiral Dirac-like fermion caused by particular spin symmetry in CoNb_(3)S_(6), paving an avenue for exploring new emergent phenomena in antiferromagnets with unconventional quasiparticle excitations.展开更多
We have investigated the electronic states of clean Fe(001) and oxygen adsorbed Fe(001)–p(1 × 1)-O films epitaxially grown on MgO(001) substrates by means of polarization-dependent angle-resolved photoemission s...We have investigated the electronic states of clean Fe(001) and oxygen adsorbed Fe(001)–p(1 × 1)-O films epitaxially grown on MgO(001) substrates by means of polarization-dependent angle-resolved photoemission spectroscopy(ARPES)and extensive density-functional theory(DFT) calculations. The observed Fermi surfaces and band dispersions of pure Fe near the Fermi level were modified upon oxygen adsorption. By the detailed comparison of ARPES and DFT results of the oxygen adsorbed Fe surface, we have clarified the orbital-dependent p–d hybridization in the topmost and second Fe layers.Furthermore, the observed energy levels and Fermi wave numbers for the oxygen adsorbed Fe surface were deviated from the DFT calculations depending on the orbital characters and momentum directions, indicating an anisotropic interplay of the electron correlation and p–d hybridization effects in the surface region.展开更多
基金supported by the National Key R&D Program of China (Grant Nos. 2020YFA0308900 and 2022YFA1403700)the National Natural Science Foundation of China (Grant Nos. 12074163, 12134020, 11974157, 12104255, 12004159, and 12374146)+8 种基金Guangdong Provincial Key Laboratory for Computational Science and Material Design (Grant No. 2019B030301001)the Science, Technology and Innovation Commission of Shenzhen Municipality (Grant Nos. ZDSYS20190902092905285 and KQTD20190929173815000)Guangdong Basic and Applied Basic Research Foundation (Grant Nos. 2022B1515020046, 2021B1515130007, 2022A1515011915, 2019A1515110712, and 2022B1515130005)Shenzhen Science and Technology Program (Grant Nos. RCJC20221008092722009 and RCBS20210706092218039)the Guangdong Innovative and Entrepreneurial Research Team Program (Grant No. 2019ZT08C044)the beam time awarded by Australia’s Nuclear Science and Technology Organisation (ANSTO) (Grant No. P8130)the Materials and Life Science Experimental Facility of the Japan Proton Accelerator Research Complex (J-PARC) was performed under a user program (Proposal No. 2019B0140)performed at the Hiroshima Synchrotron Radiation Center (HiSOR) of Japan (Grant Nos. 22BG023 and 22BG029)Shanghai Synchrotron Radiation Facility (SSRF) BL03U (Grant No. 2022-SSRF-PT-020848)。
文摘In a Dirac semimetal, the massless Dirac fermion has zero chirality, leading to surface states connected adiabatically to a topologically trivial surface state as well as vanishing anomalous Hall effect. Recently, it is predicted that in the nonrelativistic limit of certain collinear antiferromagnets, there exists a type of chiral“Dirac-like” fermion, whose dispersion manifests four-fold degenerate crossing points formed by spin-degenerate linear bands, with topologically protected Fermi arcs. Such an unconventional chiral fermion, protected by a hidden SU(2) symmetry in the hierarchy of an enhanced crystallographic group, namely spin space group, is not experimentally verified yet. Here, by angle-resolved photoemission spectroscopy measurements, we reveal the surface origin of the electron pocket at the Fermi surface in collinear antiferromagnet CoNb3S6. Combining with neutron diffraction and first-principles calculations, we suggest a multidomain collinear antiferromagnetic configuration, rendering the the existence of the Fermi-arc surface states induced by chiral Dirac-like fermions.Our work provides spectral evidence of the chiral Dirac-like fermion caused by particular spin symmetry in CoNb_(3)S_(6), paving an avenue for exploring new emergent phenomena in antiferromagnets with unconventional quasiparticle excitations.
基金Present address Synchrotron Radiation Research Center,National Institutes for Quantum and Radiological Science and Technology,1-1-1 Kouto,Sayo,Hyogo679-5148,Japan
文摘We have investigated the electronic states of clean Fe(001) and oxygen adsorbed Fe(001)–p(1 × 1)-O films epitaxially grown on MgO(001) substrates by means of polarization-dependent angle-resolved photoemission spectroscopy(ARPES)and extensive density-functional theory(DFT) calculations. The observed Fermi surfaces and band dispersions of pure Fe near the Fermi level were modified upon oxygen adsorption. By the detailed comparison of ARPES and DFT results of the oxygen adsorbed Fe surface, we have clarified the orbital-dependent p–d hybridization in the topmost and second Fe layers.Furthermore, the observed energy levels and Fermi wave numbers for the oxygen adsorbed Fe surface were deviated from the DFT calculations depending on the orbital characters and momentum directions, indicating an anisotropic interplay of the electron correlation and p–d hybridization effects in the surface region.
