Intensive farming is a primary cause of increased sediment and associated nitrogen(N)and phosphorus(P)loads in surface water systems.Determining their contributing sources,pathways and loads present major challenges i...Intensive farming is a primary cause of increased sediment and associated nitrogen(N)and phosphorus(P)loads in surface water systems.Determining their contributing sources,pathways and loads present major challenges in the high-intensity agricultural catchments.Herein,we quantify the sediment sources and magnitude of sediment total N and total P from different sources using a novel application of compound-specific stable isotope(CSSI)and fallout radionuclides(FRNs)of^(137)cs and^(210)pbex in an intensive agricultural catchment in North China.Sediment sources from surface and sub-surface soils were estimated from FRNs fingerprint and accounted for 62±7%and 38±7%respectively,while surface soil from land uses that originated from hillslope were identified by CssI fingerprint.Using a novel application of FRNs and CSSI sediment fingerprinting techniques,the dominant sediment source was derived from maize farmland(44±0.1%),followed by channel bank(38±7%).The sedimentation rate(13.55±0.30 t ha^(-1)yr^(-1))was quantifed by the^(137)cs cores(0-60 cm)at the outlet of this catchment.The total N and total P in sediment were both mostly derived from maize farmland and least from channel banks.The channel banks are significant sediment sources but contribute little to the input of sediment N and P for eutrophication.It implies that chemically-applied farmlands are the main hotspots for catchment erosion control and pollution prevention.The novel application of FRNs and CSSI techniques cost-effectively quantified sediment N and P loads from different sources with a single visit to the catchment,enabling rapid assessment for optimizing soil conservation strategies and land management practices.展开更多
One of the main challenges facing humankind is ensuring food security for a rapidly growing population with lower environmental footprints under changing climate. Environmental unsustainability of agro-food systems is...One of the main challenges facing humankind is ensuring food security for a rapidly growing population with lower environmental footprints under changing climate. Environmental unsustainability of agro-food systems is multi-faced,but alteration of biogeochemical cycles (e.g., nitrogen (N)and phosphorus (P) cycles) and emissions of greenhouse gases (GHGs) to the atmosphere have been reported as one of the main disruptive forces over safe-operating space of planetary boundaries (Springmann et al., 2018).展开更多
基金supported by the International Atomic Energy Agency through coordination research projects(CRP)under Research Contract No.23008 and technical cooperation project(TCP)RAS 5084,and the Central Public-interest Scientific Institution Basal Research Fund(No.BSRF202004)Funding for AC to collaborate on this work was provided by the High-end Foreign Experts Recruitment Program from State of Administration of Foreign Experts Affairs of ChinaThis work was partly supported by the Science and Technology Major Project of Guangxi(Guike AA17204078).
文摘Intensive farming is a primary cause of increased sediment and associated nitrogen(N)and phosphorus(P)loads in surface water systems.Determining their contributing sources,pathways and loads present major challenges in the high-intensity agricultural catchments.Herein,we quantify the sediment sources and magnitude of sediment total N and total P from different sources using a novel application of compound-specific stable isotope(CSSI)and fallout radionuclides(FRNs)of^(137)cs and^(210)pbex in an intensive agricultural catchment in North China.Sediment sources from surface and sub-surface soils were estimated from FRNs fingerprint and accounted for 62±7%and 38±7%respectively,while surface soil from land uses that originated from hillslope were identified by CssI fingerprint.Using a novel application of FRNs and CSSI sediment fingerprinting techniques,the dominant sediment source was derived from maize farmland(44±0.1%),followed by channel bank(38±7%).The sedimentation rate(13.55±0.30 t ha^(-1)yr^(-1))was quantifed by the^(137)cs cores(0-60 cm)at the outlet of this catchment.The total N and total P in sediment were both mostly derived from maize farmland and least from channel banks.The channel banks are significant sediment sources but contribute little to the input of sediment N and P for eutrophication.It implies that chemically-applied farmlands are the main hotspots for catchment erosion control and pollution prevention.The novel application of FRNs and CSSI techniques cost-effectively quantified sediment N and P loads from different sources with a single visit to the catchment,enabling rapid assessment for optimizing soil conservation strategies and land management practices.
文摘One of the main challenges facing humankind is ensuring food security for a rapidly growing population with lower environmental footprints under changing climate. Environmental unsustainability of agro-food systems is multi-faced,but alteration of biogeochemical cycles (e.g., nitrogen (N)and phosphorus (P) cycles) and emissions of greenhouse gases (GHGs) to the atmosphere have been reported as one of the main disruptive forces over safe-operating space of planetary boundaries (Springmann et al., 2018).
