Functionalized graphene oxide （FGO） was prepared by treating graphene oxide with y-aminopropyl triethoxysilane （KH-550） before the mixture was dispersed into a, ω-dihydroxy polydimethylsiloxane to get room temper...Functionalized graphene oxide （FGO） was prepared by treating graphene oxide with y-aminopropyl triethoxysilane （KH-550） before the mixture was dispersed into a, ω-dihydroxy polydimethylsiloxane to get room temperature vulcanized （RTV） silicone rubber composites by solution casting. The cured composites were then reduced with hydrazine hydrate to obtain functionalized graphene （FG）/RTV silicone rubber composites. The structures of FGO and the resultant composites were characterized by atomic force microscopy, FT-IR spectra and X-ray diffraction. KH-550 was found to be grafted onto graphene sheets, leading to an increased interlayer spacing. Significant improvements in thermal and mechanical properties were obtained. Both the FGO/RTV silicone rubber composite contain 1.0 wt% of FGO, and its reduced product showed an increase of one-step weight loss temperature with 61 ℃ and 133 ℃ higher than that of pure silicone rubber. Tensile strength and elongation at break of FG/RTV silicone rubber composite （with 0.5 wt% FGO content） increased by 175% and 67%, respectively, compared with those of pure silicone rubber.展开更多
This paper is concerned with certain multilinear commutators of BMO functions and multilinear singular integral operators with non-smooth kernels. By the sharp maximal functions estimates, the weighted norm inequaliti...This paper is concerned with certain multilinear commutators of BMO functions and multilinear singular integral operators with non-smooth kernels. By the sharp maximal functions estimates, the weighted norm inequalities for this kind of commutators are established.展开更多
Carbon materials have taken an important role in supercapacitor applications due to their outstanding features of large surface area,low price,and stable physicochemical properties.Considerable research efforts have b...Carbon materials have taken an important role in supercapacitor applications due to their outstanding features of large surface area,low price,and stable physicochemical properties.Considerable research efforts have been devoted to the development of novel synthesis strategy for the preparation of porous carbon materials in recent years.In particular,molten salt strategy represents an emerging and promising method,whereby it has shown great potential in achieving tailored production of porous carbon.It has been proved that the molten salt-assisted production of carbon via the direct carbonization of carbonaceous precursors is an effective approach.Furthermore,with the incorporation of electrochemical technology,molten salt synthesis of porous carbon has become flexible and diversiform.Here,this review focuses on the mainstream molten salt synthesis strategies for the production of porous carbon materials,which includes direct molten salt carbonization process,capture and electrochemical conversion of CO_(2)to value-added carbon,electrochemical exfoliation of graphite to graphene-based materials,and electrochemical etching of carbides to new-type carbide-derived carbon materials.The reaction mechanisms and recent advances for these strategies are reviewed and discussed systematically.The morphological and structural properties and capacitive performances of the obtained carbon materials are summarized to reveal their appealing points for supercapacitor applications.Moreover,the opportunities and challenges of the molten salt synthesis strategy for the preparation of carbon materials are also discussed in this review to provide inspiration to the future researches.展开更多
By using,summer temperature data in 26 stations from 1951 to 2003, the variation characteristics of summer temperature in Northeast China （NET） were analyzed based on the background of climate wanning. The results s...By using,summer temperature data in 26 stations from 1951 to 2003, the variation characteristics of summer temperature in Northeast China （NET） were analyzed based on the background of climate wanning. The results showed that the warming in summer was 0.15~C/10a in Northeast China, which was higher than that on the global, Northern Hemisphere or Northeast Asia scale in the recent 50 years. The responses of NET to global warming were shown in 3 aspects mainly. Firstly, it became warm and the average temperature increased in summer; secondly, the temperature variability increased, which displayed the increase of climatic instability; thirdly, the disaster of low temperature decreased and high temperature damage increased obviously, but the disaster of low temperature still existed in some areas under global warming background, which would be worthy of notice further.展开更多
In recent years,silicon(Si)and germanium(Ge)materials have been considered as promising highperformance anode materials for lithium-ion batteries due to their high theoretical capacities.It is of great importance to d...In recent years,silicon(Si)and germanium(Ge)materials have been considered as promising highperformance anode materials for lithium-ion batteries due to their high theoretical capacities.It is of great importance to design and synthesize micro/nanostructured Si and Ge materials.In this work,we demonstrated that Si,Ge and SiGe micro/nanowires can be continuously synthesized from their oxides precursors through molten salt electrodeposition.The electrochemical synthesis processes have been investigated systematically,and the deposited Si,Ge and SiGe micro/nanowires have been characterized and compared.The results show that the micro/nanostructured Si and Ge materials with tunable morphology can be facilely and continuously produced via molten salt electrodeposition.The electrodeposition process generally includes calcium oxide-assisted dissolution and electrodeposition processes,and the morphologies of the deposited Si and Ge products can be controlled by varying conditions.Si micro/nanowires,Si films,Ge micro/nanowires,and Ge particles can be continuously synthesized in a controlled manner.展开更多
【目的】现有的混合储能系统控制策略难以在保持荷电状态(state of charge,SOC)处于合理范围的同时,满足未来时刻风电波动造成的混合储能系统超前充放电需求,因此提出一种考虑平抑未来时刻风电功率波动的混合储能系统超前模糊控制策略...【目的】现有的混合储能系统控制策略难以在保持荷电状态(state of charge,SOC)处于合理范围的同时,满足未来时刻风电波动造成的混合储能系统超前充放电需求,因此提出一种考虑平抑未来时刻风电功率波动的混合储能系统超前模糊控制策略。【方法】首先,通过采用集合经验模态分解(ensemble empirical mode decomposition,EEMD)方法分解得到不同类型储能设备需要平抑的风电功率;其次,根据混合储能系统SOC和功率饱和程度整定功率修正参数,对混合储能系统输出功率进行修正;再次,由风电预测算法得到前瞻周期内风电功率预测值,根据前瞻周期内风电功率波动情况和超前控制理论整定提前充放电参数,校正储能系统输出功率;最后,以某风电场的实际数据为例,通过仿真验证了所提超前模糊控制策略的有效性。【结果】提出的控制策略不仅能够降低风电并网波动越限概率,显著减少总输出功率与目标功率偏差值,而且能够使混合储能系统的SOC控制在合理范围内。【结论】该策略可以为平抑风电波动的相关研究提供有益参考。展开更多
Remote sensing image analysis is a basic and practical research hotspot in remote sensing science.Remote sensing images contain abundant ground object information and it can be used in urban planning,agricultural moni...Remote sensing image analysis is a basic and practical research hotspot in remote sensing science.Remote sensing images contain abundant ground object information and it can be used in urban planning,agricultural monitoring,ecological services,geological exploration and other aspects.In this paper,we propose a lightweight model combining vgg-16 and u-net network.By combining two convolutional neural networks,we classify scenes of remote sensing images.While ensuring the accuracy of the model,try to reduce the memory of themodel.According to the experimental results of this paper,we have improved the accuracy of the model to 98%.The memory size of the model is 3.4 MB.At the same time,The classification and convergence speed of the model are greatly improved.We simultaneously take the remote sensing scene image of 64×64 as input into the designed model.As the accuracy of the model is 97%,it is proved that the model designed in this paper is also suitable for remote sensing images with few target feature points and low accuracy.Therefore,the model has a good application prospect in the classification of remote sensing images with few target feature points and low pixels.展开更多
Harnessing the rhizospheric microbiome,including phosphorus mineralizing bacteria(PMB),is a promising technique for maintaining sustainability and productivity in intensive agricultural systems.However,it is unclear a...Harnessing the rhizospheric microbiome,including phosphorus mineralizing bacteria(PMB),is a promising technique for maintaining sustainability and productivity in intensive agricultural systems.However,it is unclear as to which beneficial taxonomic group populations in the rhizosphere are potentially associated with the changes in soil microbiomes shifted by fertilization regimes.Herein,we analyzed the diversity and community structure of total bacteria and PMB in the rhizosphere of maize(Zea mays L.)grown in soils under 25 years of four fertilization regimes(compost,biocompost,chemical,or nonfertilized)via selective culture and Illumina sequencing of the 16S rRNA genes.Plant development explained more variations(29 and 13%,respectively)in the composition of total bacteria and PMB in the rhizosphere of maize than the different fertilization regimes.Among those genera enriched in the rhizosphere of maize,the relative abundances of Oceanobacillus,Bacillus,Achromobacter,Ensifer,Paracoccus,Ramlibacter,and Luteimonas were positively correlated with those in the bulk soil.The relative abundance of Paracoccus was significantly higher in soils fertilized by compost or biocompost than the other soils.Similar results were also observed for PMB affiliated with Ensifer,Bacillus,and Streptomyces.Although plant development was the major factor in shaping the rhizospheric microbiome of maize,fertilization regimes might have modified beneficial rhizospheric microbial taxa such as Bacillus and Ensifer.展开更多
Objective:To evaluate the compliance with lower extremity exercise and blood circulation in the feet of elderly diabetics following a combination of music media therapy and a lower extremity exercise regimen.Method:Th...Objective:To evaluate the compliance with lower extremity exercise and blood circulation in the feet of elderly diabetics following a combination of music media therapy and a lower extremity exercise regimen.Method:The 72 elderly diabetic patient subjects were divided into two groups:control group(n=38)and intervention group(n=34).Both groups were exposed to the same comprehensive therapy to control glucose levels.While the control group was given the lower extremity exercise,the intervention group received the extremity exercise in addition to the music media.Result:After three months of intervention,the adherence to the lower extremity exercise regimen in the intervention group was significantly higher than that of the control group(p<0.05).Additionally,following six months of treatment,both the dorsal artery peak values and ankle-brachial indices(ABIs)showed significant differences between the control and intervention groups(p<0.05).Conclusion:Music media treatment combined with lower extremity exercise can both significantly increase the extent of exercise compliance of elderly patients suffering from diabetes mellitus,as well as improve blood circulation in their feet.展开更多
基金Funded by the National Natural Science Foundation of China (No.51072059)
文摘Functionalized graphene oxide （FGO） was prepared by treating graphene oxide with y-aminopropyl triethoxysilane （KH-550） before the mixture was dispersed into a, ω-dihydroxy polydimethylsiloxane to get room temperature vulcanized （RTV） silicone rubber composites by solution casting. The cured composites were then reduced with hydrazine hydrate to obtain functionalized graphene （FG）/RTV silicone rubber composites. The structures of FGO and the resultant composites were characterized by atomic force microscopy, FT-IR spectra and X-ray diffraction. KH-550 was found to be grafted onto graphene sheets, leading to an increased interlayer spacing. Significant improvements in thermal and mechanical properties were obtained. Both the FGO/RTV silicone rubber composite contain 1.0 wt% of FGO, and its reduced product showed an increase of one-step weight loss temperature with 61 ℃ and 133 ℃ higher than that of pure silicone rubber. Tensile strength and elongation at break of FG/RTV silicone rubber composite （with 0.5 wt% FGO content） increased by 175% and 67%, respectively, compared with those of pure silicone rubber.
基金Supported by the National Natural Science Foundation of China (10771054, 10771221, 11071200)the Youth Foundation of Wuyi University (No. xq0930)
文摘This paper is concerned with certain multilinear commutators of BMO functions and multilinear singular integral operators with non-smooth kernels. By the sharp maximal functions estimates, the weighted norm inequalities for this kind of commutators are established.
基金financially supported by the National Natural Science Foundation of China(Nos.5202205451974181+4 种基金5200415)the Shanghai Rising-Star Program(19QA1403600)the Iron and Steel Joint Research Found of National Natural Science Foundation and China Baowu Steel Group Corporation Limited(U1860203)the Program for Professor of Special Appointment(Eastern Scholar)at Shanghai Institutions of Higher Learning(TP2019041)the CAS Interdisciplinary Innovation Team for financial support。
文摘Carbon materials have taken an important role in supercapacitor applications due to their outstanding features of large surface area,low price,and stable physicochemical properties.Considerable research efforts have been devoted to the development of novel synthesis strategy for the preparation of porous carbon materials in recent years.In particular,molten salt strategy represents an emerging and promising method,whereby it has shown great potential in achieving tailored production of porous carbon.It has been proved that the molten salt-assisted production of carbon via the direct carbonization of carbonaceous precursors is an effective approach.Furthermore,with the incorporation of electrochemical technology,molten salt synthesis of porous carbon has become flexible and diversiform.Here,this review focuses on the mainstream molten salt synthesis strategies for the production of porous carbon materials,which includes direct molten salt carbonization process,capture and electrochemical conversion of CO_(2)to value-added carbon,electrochemical exfoliation of graphite to graphene-based materials,and electrochemical etching of carbides to new-type carbide-derived carbon materials.The reaction mechanisms and recent advances for these strategies are reviewed and discussed systematically.The morphological and structural properties and capacitive performances of the obtained carbon materials are summarized to reveal their appealing points for supercapacitor applications.Moreover,the opportunities and challenges of the molten salt synthesis strategy for the preparation of carbon materials are also discussed in this review to provide inspiration to the future researches.
基金U nder the auspices of A pplication Fund of A griculture Science and Technology Fruits of M inistry of Science andTechnology ofChina (N o.04EFN 217400411)
文摘By using,summer temperature data in 26 stations from 1951 to 2003, the variation characteristics of summer temperature in Northeast China （NET） were analyzed based on the background of climate wanning. The results showed that the warming in summer was 0.15~C/10a in Northeast China, which was higher than that on the global, Northern Hemisphere or Northeast Asia scale in the recent 50 years. The responses of NET to global warming were shown in 3 aspects mainly. Firstly, it became warm and the average temperature increased in summer; secondly, the temperature variability increased, which displayed the increase of climatic instability; thirdly, the disaster of low temperature decreased and high temperature damage increased obviously, but the disaster of low temperature still existed in some areas under global warming background, which would be worthy of notice further.
基金the Shanghai Rising-Star Program(19QA1403600)the National Natural Science Foundation of China(Nos.51974181+2 种基金51574164)the Iron and Steel Joint Research Found of National Natural Science Foundation and China Baowu Steel Group Corporation Limited(U1860203)the authors also thank the CAS Interdisciplinary In novation Team for financial support.
文摘In recent years,silicon(Si)and germanium(Ge)materials have been considered as promising highperformance anode materials for lithium-ion batteries due to their high theoretical capacities.It is of great importance to design and synthesize micro/nanostructured Si and Ge materials.In this work,we demonstrated that Si,Ge and SiGe micro/nanowires can be continuously synthesized from their oxides precursors through molten salt electrodeposition.The electrochemical synthesis processes have been investigated systematically,and the deposited Si,Ge and SiGe micro/nanowires have been characterized and compared.The results show that the micro/nanostructured Si and Ge materials with tunable morphology can be facilely and continuously produced via molten salt electrodeposition.The electrodeposition process generally includes calcium oxide-assisted dissolution and electrodeposition processes,and the morphologies of the deposited Si and Ge products can be controlled by varying conditions.Si micro/nanowires,Si films,Ge micro/nanowires,and Ge particles can be continuously synthesized in a controlled manner.
基金This researchwas supported byNationalKeyResearch andDevelopment Program sub-topics[2018YFF0213606-03(Mu Y.,Hu T.L.,Gong H.,Li S.J.and Sun Y.H.)http://www.most.gov.cn]Jilin Province Science and Technology Development Plan(focuses on research and development projects)[20200402006NC(Mu Y.,Hu T.L.,Gong H.and Li S.J.)http://kjt.jl.gov.cn]+1 种基金Science and Technology Support Project for Key Industries in Southern Xinjiang[2018DB001(Gong H.,and Li S.J.)http://kjj.xjbt.gov.cn]Key technology R&D project of Changchun Science and Technology Bureau of Jilin Province[21ZGN29(Mu Y.,Bao H.P.,Wang X.B.)http://kjj.changchun.gov.cn].
文摘Remote sensing image analysis is a basic and practical research hotspot in remote sensing science.Remote sensing images contain abundant ground object information and it can be used in urban planning,agricultural monitoring,ecological services,geological exploration and other aspects.In this paper,we propose a lightweight model combining vgg-16 and u-net network.By combining two convolutional neural networks,we classify scenes of remote sensing images.While ensuring the accuracy of the model,try to reduce the memory of themodel.According to the experimental results of this paper,we have improved the accuracy of the model to 98%.The memory size of the model is 3.4 MB.At the same time,The classification and convergence speed of the model are greatly improved.We simultaneously take the remote sensing scene image of 64×64 as input into the designed model.As the accuracy of the model is 97%,it is proved that the model designed in this paper is also suitable for remote sensing images with few target feature points and low accuracy.Therefore,the model has a good application prospect in the classification of remote sensing images with few target feature points and low pixels.
基金supported by the National Key R&D Program of China(2019YFD1002000,2016YFD0800602 and 2016YFD0501404)。
文摘Harnessing the rhizospheric microbiome,including phosphorus mineralizing bacteria(PMB),is a promising technique for maintaining sustainability and productivity in intensive agricultural systems.However,it is unclear as to which beneficial taxonomic group populations in the rhizosphere are potentially associated with the changes in soil microbiomes shifted by fertilization regimes.Herein,we analyzed the diversity and community structure of total bacteria and PMB in the rhizosphere of maize(Zea mays L.)grown in soils under 25 years of four fertilization regimes(compost,biocompost,chemical,or nonfertilized)via selective culture and Illumina sequencing of the 16S rRNA genes.Plant development explained more variations(29 and 13%,respectively)in the composition of total bacteria and PMB in the rhizosphere of maize than the different fertilization regimes.Among those genera enriched in the rhizosphere of maize,the relative abundances of Oceanobacillus,Bacillus,Achromobacter,Ensifer,Paracoccus,Ramlibacter,and Luteimonas were positively correlated with those in the bulk soil.The relative abundance of Paracoccus was significantly higher in soils fertilized by compost or biocompost than the other soils.Similar results were also observed for PMB affiliated with Ensifer,Bacillus,and Streptomyces.Although plant development was the major factor in shaping the rhizospheric microbiome of maize,fertilization regimes might have modified beneficial rhizospheric microbial taxa such as Bacillus and Ensifer.
基金This study is a program,named Shanghai Geriatrics Clinical Trials Registry.Its number is 13DZ2260700financially supported by both the Nursing Research Foundation(FNF201223)of Fudan Universitythe Hua Dong Hospital,which is affiliated with Fudan University.
文摘Objective:To evaluate the compliance with lower extremity exercise and blood circulation in the feet of elderly diabetics following a combination of music media therapy and a lower extremity exercise regimen.Method:The 72 elderly diabetic patient subjects were divided into two groups:control group(n=38)and intervention group(n=34).Both groups were exposed to the same comprehensive therapy to control glucose levels.While the control group was given the lower extremity exercise,the intervention group received the extremity exercise in addition to the music media.Result:After three months of intervention,the adherence to the lower extremity exercise regimen in the intervention group was significantly higher than that of the control group(p<0.05).Additionally,following six months of treatment,both the dorsal artery peak values and ankle-brachial indices(ABIs)showed significant differences between the control and intervention groups(p<0.05).Conclusion:Music media treatment combined with lower extremity exercise can both significantly increase the extent of exercise compliance of elderly patients suffering from diabetes mellitus,as well as improve blood circulation in their feet.
