Single zinc oxide nanowires(ZnO NWs)are promising for nanogenerators because of their excellent semiconducting and piezoelectric properties,but characterizing the latter efficiently is challenging.As reported here,an ...Single zinc oxide nanowires(ZnO NWs)are promising for nanogenerators because of their excellent semiconducting and piezoelectric properties,but characterizing the latter efficiently is challenging.As reported here,an electrical breakdown strategy was used to construct single ZnO NWs with a specific length.With the high operability of a nanomanipulator in a scanning electron microscope,ZnO-NW-based twoprobe and three-probe structures were constructed for fabricating AC/DC nanogenerators,respectively.For a ZnO NW,an AC output of between−15.31 mV and 5.82 mV was achieved,while for a DC nanogenerator,an output of24.3 mV was realized.Also,the three-probe structure’s output method was changed to verify the distribution of piezoelectric charges when a single ZnO NW is bent by a probe,and DC outputs of different amplitudes were achieved.This study provides a low-cost,highly convenient,and operational method for studying the AC/DC output characteristics of single NWs,which is beneficial for the further development of nanogenerators.展开更多
Because of their unique mechanical and electrical properties,zinc oxide(ZnO)nanowires are used widely in microscopic and nanoscopic devices and structures,but characterizing them remains challenging.In this paper,two ...Because of their unique mechanical and electrical properties,zinc oxide(ZnO)nanowires are used widely in microscopic and nanoscopic devices and structures,but characterizing them remains challenging.In this paper,two pick-up strategies are proposed for characterizing the electrical properties of ZnO nanowires using SEM equipped with a nanomanipulator.To pick up nanowires efficiently,direct sampling is compared with electrification fusing,and experiments show that direct sampling is more stable while electrification fusing is more efficient.ZnO nanowires have cut-off properties,and good Schottky contact with the tungsten probes was established.In piezoelectric experiments,the maximum piezoelectric voltage generated by an individual ZnO nanowire was 0.07 V,and its impedance decreased with increasing input signal frequency until it became stable.This work offers a technical reference for the pick-up and construction of nanomaterials and nanogeneration technology.展开更多
Dissipative solitons emerge as stable pulse solutions of nonintegrable and nonconservative nonlinear physical systems, owing to a balance of nonlinearity, dispersion, and loss/gain. A considerable research effort has ...Dissipative solitons emerge as stable pulse solutions of nonintegrable and nonconservative nonlinear physical systems, owing to a balance of nonlinearity, dispersion, and loss/gain. A considerable research effort has been dedicated to characterizing amplitude and phase evolutions in the spatiotemporal dynamics of dissipative solitons emerging from fiber lasers. Yet, the picture of the buildup process of dissipative solitons in fiber lasers is incomplete in the absence of corresponding information about the polarization evolution. Here, we characterize probabilistic polarization distributions in the buildup of dissipative solitons in a net-normal dispersion fiber laser system, mode-locked by single-wall carbon nanotubes. The output optical spectra under different pump powers are filtered by a tunable filter, and are detected by a polarization state analyzer. The laser system operates from random amplified spontaneous emission into a stable dissipative soliton state as the cavity gain is progressively increased. Correspondingly, the state of polarization of each spectral wavelength converges towards a fixed point.To reveal the invariant polarization relationship among the various wavelength components of the laser output field, the phase diagram of the ellipticity angle and the spherical orientation angle is introduced. We find that,within the central spectral region of the dissipative soliton, the state of polarization evolves with frequency by tracing a uniform arc on the Poincaré sphere, whereas in the edges of the dissipative soliton spectrum, the state of polarization abruptly changes its path. Increasing cavity gain leads to spectral broadening, accompanied by a random scattering of the state of polarization of newly generated frequencies. Further increases of pump power result in dissipative soliton explosions, accompanied by the emergence of a new type of optical polarization rogue waves. These experimental results provide a deeper insight into the transient dynamics of dissipative soliton fiber lasers.展开更多
基金supported by the Research Fund Program of the Guangdong Provincial Key Laboratory of Fuel Cell Technology (Grant No.FC202204).
文摘Single zinc oxide nanowires(ZnO NWs)are promising for nanogenerators because of their excellent semiconducting and piezoelectric properties,but characterizing the latter efficiently is challenging.As reported here,an electrical breakdown strategy was used to construct single ZnO NWs with a specific length.With the high operability of a nanomanipulator in a scanning electron microscope,ZnO-NW-based twoprobe and three-probe structures were constructed for fabricating AC/DC nanogenerators,respectively.For a ZnO NW,an AC output of between−15.31 mV and 5.82 mV was achieved,while for a DC nanogenerator,an output of24.3 mV was realized.Also,the three-probe structure’s output method was changed to verify the distribution of piezoelectric charges when a single ZnO NW is bent by a probe,and DC outputs of different amplitudes were achieved.This study provides a low-cost,highly convenient,and operational method for studying the AC/DC output characteristics of single NWs,which is beneficial for the further development of nanogenerators.
基金supported by the Research Fund Program of the Guangdong Provincial Key Laboratory of Fuel Cell Technology。
文摘Because of their unique mechanical and electrical properties,zinc oxide(ZnO)nanowires are used widely in microscopic and nanoscopic devices and structures,but characterizing them remains challenging.In this paper,two pick-up strategies are proposed for characterizing the electrical properties of ZnO nanowires using SEM equipped with a nanomanipulator.To pick up nanowires efficiently,direct sampling is compared with electrification fusing,and experiments show that direct sampling is more stable while electrification fusing is more efficient.ZnO nanowires have cut-off properties,and good Schottky contact with the tungsten probes was established.In piezoelectric experiments,the maximum piezoelectric voltage generated by an individual ZnO nanowire was 0.07 V,and its impedance decreased with increasing input signal frequency until it became stable.This work offers a technical reference for the pick-up and construction of nanomaterials and nanogeneration technology.
基金National Natural Science Foundation of China(61405023,61635004)National Postdoctoral Program for Innovative Talents(BX201600200)+6 种基金Postdoctoral Science Foundation of China(2017M610589)Postdoctoral Science Foundation of Chongqing(Xm2017047)Science Foundation of Chongqing(CSTC2017JCYJA0651)Fundamental Research Funds for the Central Universities(106112017CDJXY120004)National Science Fund for Distinguished Young Scholars(61825501)H2020 Marie Sklodowska-Curie Actions(691051)Russian Ministry of Science and Education(14.Y26.31.0017)
文摘Dissipative solitons emerge as stable pulse solutions of nonintegrable and nonconservative nonlinear physical systems, owing to a balance of nonlinearity, dispersion, and loss/gain. A considerable research effort has been dedicated to characterizing amplitude and phase evolutions in the spatiotemporal dynamics of dissipative solitons emerging from fiber lasers. Yet, the picture of the buildup process of dissipative solitons in fiber lasers is incomplete in the absence of corresponding information about the polarization evolution. Here, we characterize probabilistic polarization distributions in the buildup of dissipative solitons in a net-normal dispersion fiber laser system, mode-locked by single-wall carbon nanotubes. The output optical spectra under different pump powers are filtered by a tunable filter, and are detected by a polarization state analyzer. The laser system operates from random amplified spontaneous emission into a stable dissipative soliton state as the cavity gain is progressively increased. Correspondingly, the state of polarization of each spectral wavelength converges towards a fixed point.To reveal the invariant polarization relationship among the various wavelength components of the laser output field, the phase diagram of the ellipticity angle and the spherical orientation angle is introduced. We find that,within the central spectral region of the dissipative soliton, the state of polarization evolves with frequency by tracing a uniform arc on the Poincaré sphere, whereas in the edges of the dissipative soliton spectrum, the state of polarization abruptly changes its path. Increasing cavity gain leads to spectral broadening, accompanied by a random scattering of the state of polarization of newly generated frequencies. Further increases of pump power result in dissipative soliton explosions, accompanied by the emergence of a new type of optical polarization rogue waves. These experimental results provide a deeper insight into the transient dynamics of dissipative soliton fiber lasers.