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Radiative suppression of exciton-exciton annihilation in a two-dimensional semiconductor
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作者 luca sortino Merve Gülmüs +2 位作者 Benjamin Tilmann Leonardo de S.Menezes Stefan A.Maier 《Light(Science & Applications)》 SCIE EI CSCD 2023年第9期1911-1920,共10页
Two-dimensional(2D)semiconductors possess strongly bound excitons,opening novel opportunities for engineering light-matter interaction at the nanoscale.However,their in-plane confinement leads to large non-radiative e... Two-dimensional(2D)semiconductors possess strongly bound excitons,opening novel opportunities for engineering light-matter interaction at the nanoscale.However,their in-plane confinement leads to large non-radiative exciton–exciton annihilation(EEA)processes,setting a fundamental limit for their photonic applications.In this work,we demonstrate suppression of EEA via enhancement of light-matter interaction in hybrid 2D semiconductor-dielectric nanophotonic platforms,by coupling excitons in WS2 monolayers with optical Mie resonances in dielectric nanoantennas.The hybrid system reaches an intermediate light-matter coupling regime,with photoluminescence enhancement factors up to 102.Probing the exciton ultrafast dynamics reveal suppressed EEA for coupled excitons,even under high exciton densities>10^(12)cm^(−2).We extract EEA coefficients in the order of 10^(−3),compared to 10^(−2)for uncoupled monolayers,as well as a Purcell factor of 4.5.Our results highlight engineering the photonic environment as a route to achieve higher quantum efficiencies,for low-power hybrid devices,and larger exciton densities,towards strongly correlated excitonic phases in 2D semiconductors. 展开更多
关键词 ANNIHILATION dielectric coupling
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