Recent advances in two-dimensional (2D) materials following the successful fabrication of graphene in 2004 by Novoselov and Geim is expected to grow into the new silicon, offering a lifeline for Moore’s law. With the...Recent advances in two-dimensional (2D) materials following the successful fabrication of graphene in 2004 by Novoselov and Geim is expected to grow into the new silicon, offering a lifeline for Moore’s law. With the rapid development of the synthesis methods, more and more 2D materials, such as transition metal dichalcogenides (TMDs, MX2), black phosphorus (BP) and InSe with a finite gap are reported to be more promising for achieving this dream since they often offer alternative solutions to compensate for the gapless graphene’s weaknesses.展开更多
Ferroelectric materials, with spontaneous electric polarization that can be reversed by an external electric field, have many technological applications, such as non-volatile memories, field-effect transistors, and se...Ferroelectric materials, with spontaneous electric polarization that can be reversed by an external electric field, have many technological applications, such as non-volatile memories, field-effect transistors, and sensors. Ferroelectric polarization originates from an asymmetric distribution of atoms in a material’s crystal structure, requiring the material to have two energetically degenerate ground state structures (two stable spontaneous polarization states) with inversion symmetry breaking[1].展开更多
Solid-state perovskite nanocrystals are promising coherent light sources, as there is optical feedback within the crystal structure. In order to utilize the high performance of perovskites for on-chip applications, or...Solid-state perovskite nanocrystals are promising coherent light sources, as there is optical feedback within the crystal structure. In order to utilize the high performance of perovskites for on-chip applications, or observe new physical phenomena, these crystals must be integrated with pre-fabricated electronic or photonic structures. However, the material's fragility has made the deterministic transfer a great challenge thus far. Here, we report the first deterministic transfer of perovskite nanocrystals with sub-micron accuracy. Cesium lead halide(CsPbI_3) nanocrystals were directly synthesized on flexible polydimethylsiloxane(PDMS) stamps via chemical vapor deposition(CVD) and subsequently transferred onto arbitrary substrates/structures. We demonstrated the transfer of a CsPbI_3 crystalline nanoplate(NP)onto an 8 mm fiber core and achieved single-mode whispering gallery mode lasing. Our method can be extended to a variety of other arbitrary substrates(e.g., electrodes, photonic structures, micromechanical systems), laying the foundations for previously unattainable opportunities in perovskites-based devices.展开更多
文摘Recent advances in two-dimensional (2D) materials following the successful fabrication of graphene in 2004 by Novoselov and Geim is expected to grow into the new silicon, offering a lifeline for Moore’s law. With the rapid development of the synthesis methods, more and more 2D materials, such as transition metal dichalcogenides (TMDs, MX2), black phosphorus (BP) and InSe with a finite gap are reported to be more promising for achieving this dream since they often offer alternative solutions to compensate for the gapless graphene’s weaknesses.
文摘Ferroelectric materials, with spontaneous electric polarization that can be reversed by an external electric field, have many technological applications, such as non-volatile memories, field-effect transistors, and sensors. Ferroelectric polarization originates from an asymmetric distribution of atoms in a material’s crystal structure, requiring the material to have two energetically degenerate ground state structures (two stable spontaneous polarization states) with inversion symmetry breaking[1].
基金supported by the National Natural Science Foundation of China (61875001, 61521004, 61874003, and 11474007)the National Key Research and Development Program of China (2018YFA0306900 and 2017YFA0206301)+1 种基金Beijing Natural Science Foundation (4182028), the National Basic Research Program of China (2013CB921901)and the ‘‘1000 Youth Talent Plan” Fund
文摘Solid-state perovskite nanocrystals are promising coherent light sources, as there is optical feedback within the crystal structure. In order to utilize the high performance of perovskites for on-chip applications, or observe new physical phenomena, these crystals must be integrated with pre-fabricated electronic or photonic structures. However, the material's fragility has made the deterministic transfer a great challenge thus far. Here, we report the first deterministic transfer of perovskite nanocrystals with sub-micron accuracy. Cesium lead halide(CsPbI_3) nanocrystals were directly synthesized on flexible polydimethylsiloxane(PDMS) stamps via chemical vapor deposition(CVD) and subsequently transferred onto arbitrary substrates/structures. We demonstrated the transfer of a CsPbI_3 crystalline nanoplate(NP)onto an 8 mm fiber core and achieved single-mode whispering gallery mode lasing. Our method can be extended to a variety of other arbitrary substrates(e.g., electrodes, photonic structures, micromechanical systems), laying the foundations for previously unattainable opportunities in perovskites-based devices.
