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Coherent and incoherent theories for photosynthetic energy transfer 被引量:1
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作者 ming-jie tao Na-Na Zhang +3 位作者 Peng-Yu Wen Fu-Guo Deng Qing Ai Gui-Lu Long 《Science Bulletin》 SCIE EI CAS CSCD 2020年第4期318-328,共11页
自然界的光合作用有一个显著的特点,即能量传递效率近乎100%.近年来,由于光合作用实验技术的飞速发展,譬如二维光谱实验和单分子泵浦探测实验,其能量传输过程中的量子相干效应已经在实验上得到了证实.传统的非相干理论能够有效计算能量... 自然界的光合作用有一个显著的特点,即能量传递效率近乎100%.近年来,由于光合作用实验技术的飞速发展,譬如二维光谱实验和单分子泵浦探测实验,其能量传输过程中的量子相干效应已经在实验上得到了证实.传统的非相干理论能够有效计算能量转移效率,如广义的F?rster理论和修正的Redfield理论.然而,为了描述光合作用中的量子相干效应,人们必须利用量子相干理论.例如,除了传统的Redfield理论之外,还有级联运动方程、量子路径积分、相干修正的Redfield理论、小极化子量子主方程、广义Bloch-Redfield理论等.本文综述了上述方法的主要内容,不仅有助于对自然界光合作用中激子能量转移的量子动力学进行有效的量子模拟,并对人工太阳能收集装置的设计提供了一定的指导作用. 展开更多
关键词 Forster theory Modified Redfield theory Hierarchical equation of motion Coherent modified Redfield theory Small-polaron quantum master equation General Bloch-Redfield theory
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Efficient quantum simulation of open quantum dynamics at various Hamiltonians and spectral densities 被引量:1
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作者 张娜娜 陶明杰 +5 位作者 何宛亭 陈鑫宇 孔祥宇 邓富国 Neill Lambert 艾清 《Frontiers of physics》 SCIE CSCD 2021年第5期47-60,共14页
Simulation of open quantum dynamics for various Hamiltonians and spectral densities are ubiquitous for studying various quantum systems.On a quantum computer,only log2N qubits are required for the simulation of an N-d... Simulation of open quantum dynamics for various Hamiltonians and spectral densities are ubiquitous for studying various quantum systems.On a quantum computer,only log2N qubits are required for the simulation of an N-dimensional quantum system,hence simulation in a quantum computer can greatly reduce the computational complexity compared with classical methods.Recently,a quantum simulation approach was proposed for studying photosynthetic light harvesting[npj Quantum Inf.4,52(2018)].In this paper,we apply the approach to simulate the open quantum dynamics of various photosynthetic systems.We show that for Drude—Lorentz spectral density,the dimerized geometries with strong couplings within the donor and acceptor clusters respectively exhibit significantly improved efficiency.We also demonstrate that the overall energy transfer can be optimized when the energy gap between the donor and acceptor clusters matches the optimum of the spectral density.The effects of different types of baths,e.g.,Ohmic,sub-Ohmic,and super-Ohmic spectral densities are also studied.The present investigations demonstrate that the proposed approach is universal for simulating the exact quantum dynamics of photosynthetic systems. 展开更多
关键词 nuclear magnetic resonance quantum simulation open quantum system
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Efficient generation of NOON states on two microwave-photon resonators
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作者 Ming Hua ming-jie tao Fu-Guo Deng 《Chinese Science Bulletin》 SCIE EI CAS 2014年第23期2829-2834,共6页
We present an efficient scheme for the generation of NOON states of photons in circuit QED assisted by a superconducting charge qutrit.It is completed with two kinds of manipulations,that is,the resonant operation on ... We present an efficient scheme for the generation of NOON states of photons in circuit QED assisted by a superconducting charge qutrit.It is completed with two kinds of manipulations,that is,the resonant operation on the qutrit and the resonator,and the single-qubit operation on the qutrit,and they both are high-fidelity operations.Compared with the one by a superconducting transmon qutrit proposed by Su et al.(Sci Rep 4:3898,2014),our scheme does not require to maintain the qutrit in the third excited state with a long time,which relaxes the difficulty of its implementation in experiment.Moreover,the level anharmonicity of a charge qutrit is larger and it is better for us to tune the different transitions of the charge qutrit resonant to the resonator,which makes our scheme faster than others. 展开更多
关键词 微波光子 状态 共振器 谐振器 三激发态 QED 操作 SCI
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