In traditional system identification (SI), actual values of system parameters are concealed in the input and output data;hence, it is necessary to apply estimation methods to determine the parameters. In signal proces...In traditional system identification (SI), actual values of system parameters are concealed in the input and output data;hence, it is necessary to apply estimation methods to determine the parameters. In signal processing, a signal with N elements must be sampled at least N times. Thus, most SI methods use N or more sample data to identify a model with N parameters;however, this can be improved by a new sampling theory called compressive sensing (CS). Based on CS, an SI method called compressive measurement identification (CMI) is proposed for reducing the data needed for estimation, by measuring the parameters using a series of linear measurements, rather than the measurements in sequence. In addition, the accuracy of the measurement process is guaranteed by a criterion called the restrict isometric principle. Simulations demonstrate the accuracy and robustness of CMI in an underdetermined case. Further, the dynamic process of a DC motor is identified experimentally, establishing that CMI can shorten the identification process and increase the prediction accuracy.展开更多
A low-carbon future demands more affordable batteries utilizing abundant elements with sustainable end-of-life battery management.Despite the economic and environmental advantages of Li-MnO_(2)batteries,their applica-...A low-carbon future demands more affordable batteries utilizing abundant elements with sustainable end-of-life battery management.Despite the economic and environmental advantages of Li-MnO_(2)batteries,their applica-tion so far has been largely constrained to primary batteries.Here,we demonstrate that one of the major limiting factors preventing the stable cycling of Li-MnO_(2)batteries,Mn dissolution,can be effectively mitigated by employing a common ether electrolyte,1 mol/L lithium bis(trifluorometha-nesulfonyl)imide(LiTFSI)in 1,3-dioxane(DOL)/1,2-dimethoxyethane(DME).We discover that the suppression of this dissolution enables highly reversible cycling of the MnO_(2)cathode regardless of the synthesized phase and morphology.Moreover,we find that both the LiPF_(6)salt and carbonate solvents present in conventional electrolytes are responsible for previous cycling challenges.The ether electrolyte,paired with MnO_(2)cathodes is able to demonstrate stable cycling performance at various rates,even at elevated temperature such as 60℃.Our discovery not only represents a defining step in Li-MnO_(2)batteries with extended life but provides design criteria of electrolytes for vast manganese-based cathodes in rechargeable batteries.展开更多
Intercultural trust in global contexts plays a central role in helping people from different cultures to communicate comfortably,which is essential for cooperation.Attempting to construct a framework that might foster...Intercultural trust in global contexts plays a central role in helping people from different cultures to communicate comfortably,which is essential for cooperation.Attempting to construct a framework that might foster international cooperation,and thus be helpful for coping with global emergencies,we relate a Western nomological approach to an Eastern systems approach to analyse intercultural trust in global contexts.Considering cultural impacts on intercultural trust and the nomological framework of cultural differences,we propose an intercultural trust model to interpret how cultural differences influence trust.A qualitative study of Chinese-Irish interactions was conducted to interpret this model.We organized 10 seminars on intercultural trust,and interviewed 16 people to further explore the respondents'deeper feelings and experiences about intercultural trust in global contexts.Through this study,we have identified factors impacting on intercultural trust,and found that intercultural trust can be developed and improved in various ways.To llustrate these ways,we have provided tactics and methods for building intercultural trust in global contexts.Implications are highlighted for organizations to avoid cultural clashes and relevant political or economic risks.展开更多
The many-banded krait,Bungarus multicinctus,has been recorded as the animal resource of JinQianBaiHuaShe in the Chinese Pharmacopoeia.Characterization of its venoms classified chief phyla of modern animal neurotoxins....The many-banded krait,Bungarus multicinctus,has been recorded as the animal resource of JinQianBaiHuaShe in the Chinese Pharmacopoeia.Characterization of its venoms classified chief phyla of modern animal neurotoxins.However,the evolutionary origin and diversification of its neurotoxins as well as biosynthesis of its active compounds remain largely unknown due to the lack of its high-quality genome.Here,we present the 1.58 Gbp genome of B.multicinctus assembled into 18 chromosomes with contig/scaffold N50 of 7.53 Mbp/149.8 Mbp.Major bungarotoxin-coding genes were clustered within genome by family and found to be associated with ancient local duplications.The truncation of glycosylphosphatidylinositol anchor in the 3'-terminal of a LY6E paralog released modern three-finger toxins(3FTxs)from membrane tethering before the Colubroidea divergence.Subsequent expansion and mutations diversified and recruited these 3FTxs.After the cobra/krait divergence,the modern unit-B ofβ-bungarotoxin emerged with an extra cysteine residue.A subsequent point substitution in unit-A enabled theβ-bungarotoxin covalent linkage.The B.multicinctus gene expression,chromatin topological organization,and histone modification characteristics were featured by transcriptome,proteome,chromatin conformation capture sequencing,and ChIP-seq.The results highlighted that venom production was under a sophisticated regulation.Our findings provide new insights into snake neurotoxin research,meanwhile will facilitate antivenom development,toxin-driven drug discovery and the quality control of JinQianBaiHuaShe.展开更多
Molecular dynamics(MD)simulation and orthotropic continuum model that considers interlayer shear are used to investigate the transverse deformation and free transverse vibration of multilayered rectangular molybdenum ...Molecular dynamics(MD)simulation and orthotropic continuum model that considers interlayer shear are used to investigate the transverse deformation and free transverse vibration of multilayered rectangular molybdenum disulfide(MoS2).The interlayer shear effect is considered in the continuum model by considering the multilayered MoS_(2) as a continuous uniform orthotropic material.A method for obtaining mode shapes using a single thermal vibration MD simulation is proposed.The frequencies and mode shapes predicted using the orthotropic continuum model and MD simulation agree well.The mechanical problem of multilayered two‐dimensional material plate resonator can be solved easily and efficiently by using the finite element method for the orthotropic continuum model.展开更多
The two leading modes of winter surface air temperature(SAT) over China during 1961–2017 are a spatially consistent pattern and a north-south dipole pattern. Based on the two leading modes, the characteristics of the...The two leading modes of winter surface air temperature(SAT) over China during 1961–2017 are a spatially consistent pattern and a north-south dipole pattern. Based on the two leading modes, the characteristics of the extreme cold and warm days in the two patterns, defined by the standard deviation larger than 1.28 or smaller than-1.28 in the time series of the two leading modes, are analyzed. With the increase of winter SAT during 1961–2017, the number of spatially consistent extreme cold days decreased and their occurrence was restricted to late December to early January, whereas the number of spatially consistent extreme warm days increased significantly in January and February. Global warming is associated with an increase in the spatially consistent extreme warm days and a decrease in spatially consistent extreme cold days, but has little relation to the sum of extreme cold and warm days of either the spatially consistent or north-south dipole pattern. The Siberian High(SH) is the main factor controlling the sum of spatially consistent extreme warm and cold days. The strong(weak) SH before(after) the1990 s corresponds to an increase(decrease) in the sum of the spatially consistent extreme warm and cold days. The occurrences of extreme south-cold-north-warm and extreme south-warm-north-cold days are related to the north-south difference of the SH.When the center of the SH is in mid-high latitudes, the extreme south-warm-north-cold(south-cold-north-warm) days occur more(less) often. During the winters of 1961–2017, the total number of extreme cold and warm days of the north-south dipole pattern changes negligibly. The North Atlantic meridional overturning circulation(AMOC) may be the main factor affecting the sum of the extreme cold and warm days of the two types of SAT pattern in China.展开更多
基金Supported by the National Natural Science Foundation of China(61605218)National Defense Science and Technology Innovation Foundation of Chinese Academy of Sciences(CXJJ-17S023)
文摘In traditional system identification (SI), actual values of system parameters are concealed in the input and output data;hence, it is necessary to apply estimation methods to determine the parameters. In signal processing, a signal with N elements must be sampled at least N times. Thus, most SI methods use N or more sample data to identify a model with N parameters;however, this can be improved by a new sampling theory called compressive sensing (CS). Based on CS, an SI method called compressive measurement identification (CMI) is proposed for reducing the data needed for estimation, by measuring the parameters using a series of linear measurements, rather than the measurements in sequence. In addition, the accuracy of the measurement process is guaranteed by a criterion called the restrict isometric principle. Simulations demonstrate the accuracy and robustness of CMI in an underdetermined case. Further, the dynamic process of a DC motor is identified experimentally, establishing that CMI can shorten the identification process and increase the prediction accuracy.
基金supported by NSF through the UC San Diego Materials Research Science and Engineering Center(UCSD MRSEC)DMR-2011924Part of the work used the UCSD-MTI Battery Fabrication Facility and the UCSDArbin Battery Testing Facility.Electron microscopic characterization was performed at the San Diego Nanotechnology Infrastructure(SDNI)of UCSD,a member of the National Nanotechnology Coordinated Infrastructure,which is supported by the National Science Foundation(Grant No.ECCS-1542148)Use of the Stanford Synchrotron Radiation Light source,SLAC National Accelerator Laboratory,is supported by the U.S.Department of Energy,Office of Science,Office of Basic Energy Sciences,under Contract No.DE-AC02-76SF00515.
文摘A low-carbon future demands more affordable batteries utilizing abundant elements with sustainable end-of-life battery management.Despite the economic and environmental advantages of Li-MnO_(2)batteries,their applica-tion so far has been largely constrained to primary batteries.Here,we demonstrate that one of the major limiting factors preventing the stable cycling of Li-MnO_(2)batteries,Mn dissolution,can be effectively mitigated by employing a common ether electrolyte,1 mol/L lithium bis(trifluorometha-nesulfonyl)imide(LiTFSI)in 1,3-dioxane(DOL)/1,2-dimethoxyethane(DME).We discover that the suppression of this dissolution enables highly reversible cycling of the MnO_(2)cathode regardless of the synthesized phase and morphology.Moreover,we find that both the LiPF_(6)salt and carbonate solvents present in conventional electrolytes are responsible for previous cycling challenges.The ether electrolyte,paired with MnO_(2)cathodes is able to demonstrate stable cycling performance at various rates,even at elevated temperature such as 60℃.Our discovery not only represents a defining step in Li-MnO_(2)batteries with extended life but provides design criteria of electrolytes for vast manganese-based cathodes in rechargeable batteries.
基金supported by the National Natural Science Foundation of China under Grant No.72171187the International Cooperation Project of Shaanxi Science and Technology under Grant No.2022WGZJ-15.
文摘Intercultural trust in global contexts plays a central role in helping people from different cultures to communicate comfortably,which is essential for cooperation.Attempting to construct a framework that might foster international cooperation,and thus be helpful for coping with global emergencies,we relate a Western nomological approach to an Eastern systems approach to analyse intercultural trust in global contexts.Considering cultural impacts on intercultural trust and the nomological framework of cultural differences,we propose an intercultural trust model to interpret how cultural differences influence trust.A qualitative study of Chinese-Irish interactions was conducted to interpret this model.We organized 10 seminars on intercultural trust,and interviewed 16 people to further explore the respondents'deeper feelings and experiences about intercultural trust in global contexts.Through this study,we have identified factors impacting on intercultural trust,and found that intercultural trust can be developed and improved in various ways.To llustrate these ways,we have provided tactics and methods for building intercultural trust in global contexts.Implications are highlighted for organizations to avoid cultural clashes and relevant political or economic risks.
基金the Fundamental Research Funds for the Central Public Welfare Research Institutes(ZZ13-YQ-047,ZXKT22006,China)quality standard system construction for the whole industry chain of Chinese medicine from Guangdong Provincial Drug Administration of China(002009/2019KT1261/2020ZDB25)+2 种基金the National Major Science and Technology Projects(2019ZX09201005,China)the Open Research Fund of Chengdu University of Traditional Chinese Medicino state Key Laboratory scluthwestern Chinese Medicine Resources(2022ZYXK2011006,China)the National Key R&D Program of China(2019YFC1711100)。
文摘The many-banded krait,Bungarus multicinctus,has been recorded as the animal resource of JinQianBaiHuaShe in the Chinese Pharmacopoeia.Characterization of its venoms classified chief phyla of modern animal neurotoxins.However,the evolutionary origin and diversification of its neurotoxins as well as biosynthesis of its active compounds remain largely unknown due to the lack of its high-quality genome.Here,we present the 1.58 Gbp genome of B.multicinctus assembled into 18 chromosomes with contig/scaffold N50 of 7.53 Mbp/149.8 Mbp.Major bungarotoxin-coding genes were clustered within genome by family and found to be associated with ancient local duplications.The truncation of glycosylphosphatidylinositol anchor in the 3'-terminal of a LY6E paralog released modern three-finger toxins(3FTxs)from membrane tethering before the Colubroidea divergence.Subsequent expansion and mutations diversified and recruited these 3FTxs.After the cobra/krait divergence,the modern unit-B ofβ-bungarotoxin emerged with an extra cysteine residue.A subsequent point substitution in unit-A enabled theβ-bungarotoxin covalent linkage.The B.multicinctus gene expression,chromatin topological organization,and histone modification characteristics were featured by transcriptome,proteome,chromatin conformation capture sequencing,and ChIP-seq.The results highlighted that venom production was under a sophisticated regulation.Our findings provide new insights into snake neurotoxin research,meanwhile will facilitate antivenom development,toxin-driven drug discovery and the quality control of JinQianBaiHuaShe.
基金National Science Fund for Distinguished Young Scholars,Grant/Award Number:11925205National Natural Science Foundation of China,Grant/Award Number:51921003。
文摘Molecular dynamics(MD)simulation and orthotropic continuum model that considers interlayer shear are used to investigate the transverse deformation and free transverse vibration of multilayered rectangular molybdenum disulfide(MoS2).The interlayer shear effect is considered in the continuum model by considering the multilayered MoS_(2) as a continuous uniform orthotropic material.A method for obtaining mode shapes using a single thermal vibration MD simulation is proposed.The frequencies and mode shapes predicted using the orthotropic continuum model and MD simulation agree well.The mechanical problem of multilayered two‐dimensional material plate resonator can be solved easily and efficiently by using the finite element method for the orthotropic continuum model.
基金This work was supported by the National Key R&D Program(Grant No.2016YFA0601502)the National Natural Science Foundation of China(Grant Nos.41822503&41375092).
文摘The two leading modes of winter surface air temperature(SAT) over China during 1961–2017 are a spatially consistent pattern and a north-south dipole pattern. Based on the two leading modes, the characteristics of the extreme cold and warm days in the two patterns, defined by the standard deviation larger than 1.28 or smaller than-1.28 in the time series of the two leading modes, are analyzed. With the increase of winter SAT during 1961–2017, the number of spatially consistent extreme cold days decreased and their occurrence was restricted to late December to early January, whereas the number of spatially consistent extreme warm days increased significantly in January and February. Global warming is associated with an increase in the spatially consistent extreme warm days and a decrease in spatially consistent extreme cold days, but has little relation to the sum of extreme cold and warm days of either the spatially consistent or north-south dipole pattern. The Siberian High(SH) is the main factor controlling the sum of spatially consistent extreme warm and cold days. The strong(weak) SH before(after) the1990 s corresponds to an increase(decrease) in the sum of the spatially consistent extreme warm and cold days. The occurrences of extreme south-cold-north-warm and extreme south-warm-north-cold days are related to the north-south difference of the SH.When the center of the SH is in mid-high latitudes, the extreme south-warm-north-cold(south-cold-north-warm) days occur more(less) often. During the winters of 1961–2017, the total number of extreme cold and warm days of the north-south dipole pattern changes negligibly. The North Atlantic meridional overturning circulation(AMOC) may be the main factor affecting the sum of the extreme cold and warm days of the two types of SAT pattern in China.