Nontrivial topological behaviors in superconducting materials provide resourceful ground for the emergence and study of unconventional quantum states.Charge doping by the controlled intercalation of donor atoms is an ...Nontrivial topological behaviors in superconducting materials provide resourceful ground for the emergence and study of unconventional quantum states.Charge doping by the controlled intercalation of donor atoms is an efficient route for enhancing/inducement of superconducting and topological behaviors in layered topological insulators and semimetals.Herein,we enhanced the superconducting temperature of TaSe_(2) by 20-folds(~3 K)through Sn atoms intercalation.Using first-principles calculations,we demonstrated the existence of nontrivial topological features.Sn_(0.5)TaSe_(2) displays topological nodal lines around the K high symmetry point in the Brillouin zone,with drumhead-like shaped surface states protected by inversion symmetry.Altogether,the coexistence of these properties makes Sn_(0.5)TaSe_(2) a potential candidate for topological superconductivity.展开更多
基金the financial support in part by the National Key R&D Program of China(No.2017YFA0303500)the National Natural Science Foundation of China(NSFC)(Nos.U1932201,11574280,and 21727801)+2 种基金NSFC-MAECI(No.51861135202)International Partnership Program of CAS(No.211134KYSB20190063)CAS Collaborative Innovation Program of Hefei Science Center(No.2019HSC-CIP002).
文摘Nontrivial topological behaviors in superconducting materials provide resourceful ground for the emergence and study of unconventional quantum states.Charge doping by the controlled intercalation of donor atoms is an efficient route for enhancing/inducement of superconducting and topological behaviors in layered topological insulators and semimetals.Herein,we enhanced the superconducting temperature of TaSe_(2) by 20-folds(~3 K)through Sn atoms intercalation.Using first-principles calculations,we demonstrated the existence of nontrivial topological features.Sn_(0.5)TaSe_(2) displays topological nodal lines around the K high symmetry point in the Brillouin zone,with drumhead-like shaped surface states protected by inversion symmetry.Altogether,the coexistence of these properties makes Sn_(0.5)TaSe_(2) a potential candidate for topological superconductivity.
