We present our results from the measurements of third-order optical nonlinearity in DNA doped Rhodamine 6G/PVA films achieved through Z-scan measurements using ~2 picosecond (ps) pulses at a wavelength of 800 nm. The ...We present our results from the measurements of third-order optical nonlinearity in DNA doped Rhodamine 6G/PVA films achieved through Z-scan measurements using ~2 picosecond (ps) pulses at a wavelength of 800 nm. The films demonstrated negative nonlinear refractive index (n2) with magnitudes of (0.065 - 2.89) × 10–14 cm2/W with varying concentration of DNA. Open aperture data demonstrated strong two-photon absorption with a magnitude of ~1.6 cm/GW for films doped with 2 wt% of DNA. The recovery time of excited state population, retrieved from the degenerate pump-probe experimental data, was <4 ps. These data suggests that DNA is promising material for applications such as optical switching.展开更多
文摘We present our results from the measurements of third-order optical nonlinearity in DNA doped Rhodamine 6G/PVA films achieved through Z-scan measurements using ~2 picosecond (ps) pulses at a wavelength of 800 nm. The films demonstrated negative nonlinear refractive index (n2) with magnitudes of (0.065 - 2.89) × 10–14 cm2/W with varying concentration of DNA. Open aperture data demonstrated strong two-photon absorption with a magnitude of ~1.6 cm/GW for films doped with 2 wt% of DNA. The recovery time of excited state population, retrieved from the degenerate pump-probe experimental data, was <4 ps. These data suggests that DNA is promising material for applications such as optical switching.