利用格点化降水观测数据集(CN05.1)以及ECMWF再分析资料(ERA5),分析1961—2020年夏季西南地区东部(Eastern Southwest China,ESWC)的降水、水汽含量及降水转化率特征,并利用天气学分析方法初步探究地形分布对降水转化率空间分布差异的影...利用格点化降水观测数据集(CN05.1)以及ECMWF再分析资料(ERA5),分析1961—2020年夏季西南地区东部(Eastern Southwest China,ESWC)的降水、水汽含量及降水转化率特征,并利用天气学分析方法初步探究地形分布对降水转化率空间分布差异的影响,最后利用中尺度数值模式WRF4.0(Weather Research and Forecasting Model)设计地形敏感性试验验证地形对西南地区东部夏季降水的作用。结果表明:(1)1961—2020年夏季西南地区东部的降水呈现东多西少的分布特征,但水汽含量却在其东南部和西北部存在两个大值区,水汽大值区降水转化率偏低,强降水区与水汽含量大值区分布存在明显差异,通过分析强降水区与水平风场及垂直速度场的形势配合发现地形是导致此差异的重要因素。(2)WRF模式能较好地模拟出西南地区东部夏季降水的空间分布特征,通过地形敏感性试验发现,区域内大娄山、方斗山及大巴山组成的西南-东北向山地地形分布对降水强度有显著影响,地形高度的降低将导致区域东南部降水量显著减少。(3)敏感性试验中将区域地形高度分别降低一半和去除地形后,区域东南部的降水在月时间尺度中将分别减少9.89%和19.90%。地形高度的改变也会引起区域垂直速度、水平风场、水汽输送及水汽辐合量发生改变,当地形高度降低后,上升运动及西南风明显减弱,水汽输送强度降低,水汽辐合量减少,不利于降水形成。展开更多
Using the daily and monthly data of surface air pressure, meridional wind, radiation and water vapor from NCEP/NCAR reanalysis for the period of 1979―2006, we have examined the seasonal variations of the interhemisph...Using the daily and monthly data of surface air pressure, meridional wind, radiation and water vapor from NCEP/NCAR reanalysis for the period of 1979―2006, we have examined the seasonal variations of the interhemispheric oscillations (IHO) in mass field of the global atmosphere. Our results have demonstrated that IHO as observed in surface air pressure field shows the distinct seasonal cycle. This seasonal cycle has an interhemispheric seesaw structure with comparable annual ranges of surface air pressure in the Southern and Northern Hemispheres. Mass of water vapor changes out-of-phase between the Southern and Northern Hemispheres, showing clearly a seasonal cycle with its annual range almost equivalent to annual range of the IHO seasonal cycle. Amazingly, the cross-equatorial flow is found to be induced by annual changes in water vapor mass as a response of the atmosphere to seasonal cycle of forcing from hemispheric net surface short- and long-wave radiations. The IHO seasonality exhibits its larger variations in magnitude in mid-latitudes other than in other regions of the globe. Additionally, our results also show that the global air mass is redistributed seasonally not only between the Northern and Southern Hemispheres but also between land and sea. This land-sea air mass redis- tribution induces a zonal pattern of surface air pressure in the Northern Hemisphere but the meridional pattern in the Southern Hemisphere.展开更多
Fluoran salicylaldehyde hydrazone metal complex(FSHMC)is a kind of recently reported photo-responsive system,which has the advantages of simple synthesis,multiple colors as well as distinct color change before and aft...Fluoran salicylaldehyde hydrazone metal complex(FSHMC)is a kind of recently reported photo-responsive system,which has the advantages of simple synthesis,multiple colors as well as distinct color change before and after UV light irradiation.However,the emission property of FSHMC is relatively unitary.In solid state,especially,only fluorescence quench is induced after UV light irradiation,which limits their applications.In this work,a typical aggregation-induced emission(AIE)moiety of tetraphenylethene(TPE)was introduced to the design of FSHMC.The obtained FSHMC,2-Zn,exhibited reversible color and fluorescence changes upon UV light irradiation.Due to the AIE feature of compound 2,2-Zn exhibited different emission changes upon UV light irradiation in THF and in solid matrix,because of the fluorescence resonance energy transfer(FRET)process from TPE moiety to rhodamine B moiety.展开更多
文摘利用格点化降水观测数据集(CN05.1)以及ECMWF再分析资料(ERA5),分析1961—2020年夏季西南地区东部(Eastern Southwest China,ESWC)的降水、水汽含量及降水转化率特征,并利用天气学分析方法初步探究地形分布对降水转化率空间分布差异的影响,最后利用中尺度数值模式WRF4.0(Weather Research and Forecasting Model)设计地形敏感性试验验证地形对西南地区东部夏季降水的作用。结果表明:(1)1961—2020年夏季西南地区东部的降水呈现东多西少的分布特征,但水汽含量却在其东南部和西北部存在两个大值区,水汽大值区降水转化率偏低,强降水区与水汽含量大值区分布存在明显差异,通过分析强降水区与水平风场及垂直速度场的形势配合发现地形是导致此差异的重要因素。(2)WRF模式能较好地模拟出西南地区东部夏季降水的空间分布特征,通过地形敏感性试验发现,区域内大娄山、方斗山及大巴山组成的西南-东北向山地地形分布对降水强度有显著影响,地形高度的降低将导致区域东南部降水量显著减少。(3)敏感性试验中将区域地形高度分别降低一半和去除地形后,区域东南部的降水在月时间尺度中将分别减少9.89%和19.90%。地形高度的改变也会引起区域垂直速度、水平风场、水汽输送及水汽辐合量发生改变,当地形高度降低后,上升运动及西南风明显减弱,水汽输送强度降低,水汽辐合量减少,不利于降水形成。
基金the National Natural Science Foundation of China (Grant No. 40675025)the Project of National Key Basic Research Development (Grant No. 2004CB418302)the Key Lab of Meteorological Disasters (KLME) of Nanjing University of Information Science and Technology (NUIST) (Grant No. KLME060101)
文摘Using the daily and monthly data of surface air pressure, meridional wind, radiation and water vapor from NCEP/NCAR reanalysis for the period of 1979―2006, we have examined the seasonal variations of the interhemispheric oscillations (IHO) in mass field of the global atmosphere. Our results have demonstrated that IHO as observed in surface air pressure field shows the distinct seasonal cycle. This seasonal cycle has an interhemispheric seesaw structure with comparable annual ranges of surface air pressure in the Southern and Northern Hemispheres. Mass of water vapor changes out-of-phase between the Southern and Northern Hemispheres, showing clearly a seasonal cycle with its annual range almost equivalent to annual range of the IHO seasonal cycle. Amazingly, the cross-equatorial flow is found to be induced by annual changes in water vapor mass as a response of the atmosphere to seasonal cycle of forcing from hemispheric net surface short- and long-wave radiations. The IHO seasonality exhibits its larger variations in magnitude in mid-latitudes other than in other regions of the globe. Additionally, our results also show that the global air mass is redistributed seasonally not only between the Northern and Southern Hemispheres but also between land and sea. This land-sea air mass redis- tribution induces a zonal pattern of surface air pressure in the Northern Hemisphere but the meridional pattern in the Southern Hemisphere.
基金This work was supported by the National Science Fund for Distinguished Young Scholars of China(No.21825106)the National Natural Science Foundation of China(Nos.21671175,U1904172)+2 种基金the Program for Science&Technology Innovation Talents in Universities of Henan Province,China(No.164100510005)the Program for Innovative Research Team(in Science and Technology)in Universities of Henan Province,China(No.19IRTSTHN022)the Undergraduate Innovation and Entrepreneurship Training Program of Zhengzhou University,China(No.202010459003).
文摘Fluoran salicylaldehyde hydrazone metal complex(FSHMC)is a kind of recently reported photo-responsive system,which has the advantages of simple synthesis,multiple colors as well as distinct color change before and after UV light irradiation.However,the emission property of FSHMC is relatively unitary.In solid state,especially,only fluorescence quench is induced after UV light irradiation,which limits their applications.In this work,a typical aggregation-induced emission(AIE)moiety of tetraphenylethene(TPE)was introduced to the design of FSHMC.The obtained FSHMC,2-Zn,exhibited reversible color and fluorescence changes upon UV light irradiation.Due to the AIE feature of compound 2,2-Zn exhibited different emission changes upon UV light irradiation in THF and in solid matrix,because of the fluorescence resonance energy transfer(FRET)process from TPE moiety to rhodamine B moiety.