The light-matter interaction between plasmonic nanocavity and exciton at the sub-diffraction limit is a central research field in nanophotonics.Here,we demonstrated the vertical distribution of the light-matter intera...The light-matter interaction between plasmonic nanocavity and exciton at the sub-diffraction limit is a central research field in nanophotonics.Here,we demonstrated the vertical distribution of the light-matter interactions at~1 nm spatial resolution by coupling A excitons of MoS2 and gap-mode plasmonic nanocavities.Moreover,we observed the significant photoluminescence(PL)enhancement factor reaching up to 2800 times,which is attributed to the Purcell effect and large local density of states in gap-mode plasmonic nanocavities.Meanwhile,the theoretical calculations are well reproduced and support the experimental results.展开更多
基金supported by the National Key Research and Development Program of China(2019YFA0705400,2020YFB1505800,2019YFD0901100.and 2021YFA12015021.the National Natural Science Foundation of China(21925404,22021001,22002128,21991151,and 92161118).the Science and Technology Planning Project of Fujian Province(2021Y0104).the State Key Laboratory of Fine Chemicals Dalian University of Technology(KF2002 and the“111”Project(B17027).
文摘The light-matter interaction between plasmonic nanocavity and exciton at the sub-diffraction limit is a central research field in nanophotonics.Here,we demonstrated the vertical distribution of the light-matter interactions at~1 nm spatial resolution by coupling A excitons of MoS2 and gap-mode plasmonic nanocavities.Moreover,we observed the significant photoluminescence(PL)enhancement factor reaching up to 2800 times,which is attributed to the Purcell effect and large local density of states in gap-mode plasmonic nanocavities.Meanwhile,the theoretical calculations are well reproduced and support the experimental results.
