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Soil-moisture dynamics and tree-water status in a Picea crassifolia forest, Qilian Mountains, China 被引量:1
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作者 Hu Liu Lin Li +2 位作者 SiJia Wang qiyue yang WenZhi Zhao 《Research in Cold and Arid Regions》 CSCD 2020年第1期34-46,共13页
Landscapes of the mountainous regions in northwestern China comprise a unique pattern of vegetation,consisting of a mosaic of grassland and shrub-forest.Forests generally self-organize into ordered structures and coal... Landscapes of the mountainous regions in northwestern China comprise a unique pattern of vegetation,consisting of a mosaic of grassland and shrub-forest.Forests generally self-organize into ordered structures and coalesce into blocks on north-facing slopes or stripes along southeast-facing slopes,with Picea crassifolia being the most representative and dominant tree species.We investigated the tree-water status and soil-moisture dynamics at a forest site(Guantan)of the Qilian Mountains in northwest China.The 30-minute-interval measurements of tree-sap flow during the growing season of 2008 are presented,and the potential functional relations between tree transpiration and environmental factors are evaluated.Soil moisture and solar energy were identified as the most influential factors,explaining more than 70%of the variance in sap flow.Based on field measurements obtained at the forest site,a stochastic model of soil-moisture dynamics was tested;and the steady-state probability density functions(PDFs)of the long-term soil-moisture dynamics and static tree-water stress were estimated using the validated model and parameters.We found that the model reproduced measured soil moisture well,despite all the simplifying assumptions.The generated PDF of long-term soil moisture was relatively open,with middle to low average values;and the calculated density of the static tree-water stress at the forest site was largely concentrated between 0 and 0.6,suggesting a moderate water-stress situation in most cases.We argue that both water and energy are limiting factors for vegetation at the forest site.In addition,the tradeoff between reduced evapotranspiration(ET)from limited solar energy and increased soil-moisture availability may create a stressed but tolerable environment and,in turn,produce a relatively constant ecological niche favorable to Picea crassifolia growth. 展开更多
关键词 sap flow soil moisture stochastic modeling semiarid alpine ecosystem
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纤维素基生物质催化转化制备二醇 被引量:4
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作者 吴巧妹 杨启悦 +3 位作者 曾宪海 邓佳慧 张良清 邱佳容 《化学进展》 SCIE CAS CSCD 北大核心 2022年第10期2173-2189,共17页
生物质作为最有潜力替代化石能源的可再生资源之一,受到日益广泛的重视。纤维素基生物质是催化转化为各种燃料和化学品的重要原料。近年来,二醇(包括乙二醇、丙二醇和丁二醇等)作为燃料和化学品广泛应用于各个领域,市场需求很大。传统... 生物质作为最有潜力替代化石能源的可再生资源之一,受到日益广泛的重视。纤维素基生物质是催化转化为各种燃料和化学品的重要原料。近年来,二醇(包括乙二醇、丙二醇和丁二醇等)作为燃料和化学品广泛应用于各个领域,市场需求很大。传统制备二醇是以化石能源为原料,存在原料不可再生和环境污染大等缺点。因此采用非化石原料途径制备二醇受到越来越多的关注,其中以纤维素基生物质催化制备二醇是克服化石燃料短缺和减少环境污染的重要途径之一。本文系统总结了近年来以纤维素基生物质(纤维素、葡萄糖、果糖和山梨醇)为原料催化转化制备二醇的研究现状,对反应途径、反应机理、催化剂稳定性和反应溶剂类型等进行了详细介绍,在此基础上对利用纤维素基生物质原料催化制备二醇的发展趋势进行展望,以期为相关研究者提供参考。 展开更多
关键词 纤维素 C_(6)碳水化合物 催化剂 二醇
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生物基平台化合物催化转化制备糠醇 被引量:2
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作者 杨启悦 吴巧妹 +3 位作者 邱佳容 曾宪海 唐兴 张良清 《化学进展》 SCIE CAS CSCD 北大核心 2022年第8期1748-1759,共12页
糠醇(FOL)作为一种重要且多用途的有机化工原料,可以有效地转化为各种高价值的化学品,如糠醛树脂、脲醛树脂、酚醛树脂、果酸、增塑剂和火箭燃料等。以糠醛(FAL)、木糖和果糖为原料经催化加氢制备FOL的绿色生产工艺,具有良好的应用前景... 糠醇(FOL)作为一种重要且多用途的有机化工原料,可以有效地转化为各种高价值的化学品,如糠醛树脂、脲醛树脂、酚醛树脂、果酸、增塑剂和火箭燃料等。以糠醛(FAL)、木糖和果糖为原料经催化加氢制备FOL的绿色生产工艺,具有良好的应用前景和研究价值。本文系统总结了近年来国内外以FAL、木糖、果糖为原料制备FOL的研究现状,从催化剂类型、催化效率和催化机理等方面对制备FOL的催化剂进行了总结,并在此基础上对催化加氢制备FOL的发展趋势进行了展望,为开发更为新型、高效、绿色、稳定的催化剂体系提供理论指导和有益借鉴。 展开更多
关键词 糠醇 催化剂 糠醛 木糖 果糖
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