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Ecological-Based Mining:A Coal-Water-Thermal Collaborative Paradigm in Ecologically Fragile Areas in Western China 被引量:2
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作者 Xiaoxiu Liu Yifan Zeng +3 位作者 qiang wu Shihao Meng Jiyue Liang Zhuping Hou 《Engineering》 SCIE EI CAS CSCD 2024年第7期209-222,共14页
A substantial reduction in groundwater level,exacerbated by coal mining activities,is intensifying water scarcity in western China’s ecologically fragile coal mining areas.China’s national strategic goal of achievin... A substantial reduction in groundwater level,exacerbated by coal mining activities,is intensifying water scarcity in western China’s ecologically fragile coal mining areas.China’s national strategic goal of achieving a carbon peak and carbon neutrality has made eco-friendly mining that prioritizes the protection and efficient use of water resources essential.Based on the resource characteristics of mine water and heat hazards,an intensive coal-water-thermal collaborative co-mining paradigm for the duration of the mining process is proposed.An integrated system for the production,supply,and storage of mining companion resources is achieved through technologies such as roof water inrush prevention and control,hydrothermal quality improvement,and deep-injection geological storage.An active preventive and control system achieved by adjusting the mining technology and a passive system centered on multiobjective drainage and grouting treatment are suggested,in accordance with the original geological characteristics and dynamic process of water inrush.By implementing advanced multi-objective drainage,specifically designed to address the“skylight-type”water inrush mode in the Yulin mining area of Shaanxi Province,a substantial reduction of 50%in water drillings and inflow was achieved,leading to stabilized water conditions that effectively ensure subsequent safe coal mining.An integrated-energy complementary model that incorporates the clean production concept of heat utilization is also proposed.The findings indicate a potential saving of 8419 t of standard coal by using water and air heat as an alternative heating source for the Xiaojihan coalmine,resulting in an impressive energy conservation of 50.2%and a notable 24.2%reduction in carbon emissions.The ultra-deep sustained water injection of 100 m^(3)·h^(-1)in a single well would not rupture the formation or cause water leakage,and 7.87×10^(5)t of mine water could be effectively stored in the Liujiagou Formation,presenting a viable method for mine-water management in the Ordos Basin and providing insights for green and low-carbon mining. 展开更多
关键词 Dual carbon targets Coal-water-thermal co-mining Ecologically fragile areas Mine-water control Resource utilization
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Role of gut microbiota in Crohn’s disease pathogenesis:Insights from fecal microbiota transplantation in mouse model 被引量:2
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作者 qiang wu Lian-Wen Yuan +5 位作者 Li-Chao Yang Ya-Wei Zhang Heng-Chang Yao Liang-Xin Peng Bao-Jia Yao Zhi-Xian Jiang 《World Journal of Gastroenterology》 SCIE CAS 2024年第31期3689-3704,共16页
BACKGROUND Inflammatory bowel disease,particularly Crohn’s disease(CD),has been associated with alterations in mesenteric adipose tissue(MAT)and the phenomenon termed“creeping fat”.Histopathological evaluations sho... BACKGROUND Inflammatory bowel disease,particularly Crohn’s disease(CD),has been associated with alterations in mesenteric adipose tissue(MAT)and the phenomenon termed“creeping fat”.Histopathological evaluations showed that MAT and intestinal tissues were significantly altered in patients with CD,with these tissues characterized by inflammation and fibrosis.AIM To evaluate the complex interplay among MAT,creeping fat,inflammation,and gut microbiota in CD.METHODS Intestinal tissue and MAT were collected from 12 patients with CD.Histological manifestations and protein expression levels were analyzed to determine lesion characteristics.Fecal samples were collected from five recently treated CD patients and five control subjects and transplanted into mice.The intestinal and mesenteric lesions in these mice,as well as their systemic inflammatory status,were assessed and compared in mice transplanted with fecal samples from CD patients and control subjects.RESULTS Pathological examination of MAT showed significant differences between CDaffected and unaffected colons,including significant differences in gut microbiota structure.Fetal microbiota transplantation(FMT)from clinically healthy donors into mice with 2,4,6-trinitrobenzene sulfonic acid(TNBS)-induced CD ameliorated CD symptoms,whereas FMT from CD patients into these mice exacerbated CD symptoms.Notably,FMT influenced intestinal permeability,barrier function,and levels of proinflammatory factors and adipokines.Furthermore,FMT from CD patients intensified fibrotic changes in the colon tissues of mice with TNBS-induced CD.CONCLUSION Gut microbiota play a critical role in the histopathology of CD.Targeting MAT and creeping fat may therefore have potential in the treatment of patients with CD. 展开更多
关键词 Mesenteric adipose tissue Crohn’s disease Fecal microbiota transplantation Intestinal fibrosis Intestinal barrier
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A mixed-coordination electron trapping-enabled high-precision touch-sensitive screen for wearable devices 被引量:1
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作者 Xi Zhang Junchi Ma +5 位作者 Hualin Deng Jinming Zhong Kaichen Xu qiang wu Bo Wen Dongfeng Diao 《Bio-Design and Manufacturing》 SCIE EI CAS CSCD 2024年第4期413-427,共15页
Touch-sensitive screens are crucial components of wearable devices.Materials such as reduced graphene oxide(rGO),carbon nanotubes(CNTs),and graphene offer promising solutions for flexible touch-sensitive screens.Howev... Touch-sensitive screens are crucial components of wearable devices.Materials such as reduced graphene oxide(rGO),carbon nanotubes(CNTs),and graphene offer promising solutions for flexible touch-sensitive screens.However,when stacked with flexible substrates to form multilayered capacitive touching sensors,these materials often suffer from substrate delamination in response to deformation;this is due to the materials having different Young’s modulus values.Delamination results in failure to offer accurate touch screen recognition.In this work,we demonstrate an induced charge-based mutual capacitive touching sensor capable of high-precision touch sensing.This is enabled by electron trapping and polarization effects related to mixed-coordinated bonding between copper nanoparticles and vertically grown graphene nanosheets.Here,we used an electron cyclotron resonance system to directly fabricate graphene-metal nanofilms(GMNFs)using carbon and copper,which are firmly adhered to flexible substrates.After being subjected to 3000 bending actions,we observed almost no change in touch sensitivity.The screen interaction system,which has a signal-to-noise ratio of 41.16 dB and resolution of 650 dpi,was tested using a handwritten Chinese character recognition trial and achieved an accuracy of 94.82%.Taken together,these results show the promise of touch-sensitive screens that use directly fabricated GMNFs for wearable devices. 展开更多
关键词 Flexible touch-sensitive screen Graphene-metal nanofilms Mixed coordination Wearable device
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Automatic diagnosis of diabetic retinopathy using vision transformer based on wide-field optical coherence tomography angiography
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作者 Zenan Zhou Huanhuan Yu +3 位作者 Jiaqing Zhao Xiangning Wang qiang wu Cuixia Dai 《Journal of Innovative Optical Health Sciences》 SCIE EI CSCD 2024年第2期35-44,共10页
Diabetic retinopathy(DR)is one of the major causes of visual impairment in adults with diabetes.Optical coherence tomography angiography(OCTA)is nowadays widely used as the golden criterion for diagnosing DR.Recently,... Diabetic retinopathy(DR)is one of the major causes of visual impairment in adults with diabetes.Optical coherence tomography angiography(OCTA)is nowadays widely used as the golden criterion for diagnosing DR.Recently,wide-field OCTA(WF-OCTA)provided more abundant information including that of the peripheral retinal degenerative changes and it can contribute in accurately diagnosing DR.The need for an automatic DR diagnostic system based on WF-OCTA pictures attracts more and more attention due to the large diabetic population and the prevalence of retinopathy cases.In this study,automatic diagnosis of DR using vision transformer was performed using WF-OCTA images(12 mm×12 mm single-scan)centered on the fovea as the dataset.WF-OCTA images were automatically classified into four classes:No DR,mild nonproliferative diabetic retinopathy(NPDR),moderate to severe NPDR,and proliferative diabetic retinopathy(PDR).The proposed method for detecting DR on the test set achieves accuracy of 99.55%,sensitivity of 99.49%,and specificity of 99.57%.The accuracy of the method for DR staging reaches up to 99.20%,which has been proven to be higher than that attained by classical convolutional neural network models.Results show that the automatic diagnosis of DR based on vision transformer and WF-OCTA pictures is more effective for detecting and staging DR. 展开更多
关键词 Wide field optical coherence tomography angiography diabetic retinopathy vision transformer image classification
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Three dimensional discrete element modelling of the conventional compression behavior of gas hydrate bearing coal
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作者 Xia Gao Nannan Wang +4 位作者 Baoyong Zhang Qiqi Lin qiang wu Wei Meng Xia Liu 《International Journal of Coal Science & Technology》 EI CAS CSCD 2024年第1期61-77,共17页
To analyze the relationship between macro and meso parameters of the gas hydrate bearing coal(GHBC)and to calibrate the meso-parameters,the numerical tests were conducted to simulate the laboratory triaxial compressio... To analyze the relationship between macro and meso parameters of the gas hydrate bearing coal(GHBC)and to calibrate the meso-parameters,the numerical tests were conducted to simulate the laboratory triaxial compression tests by PFC3D,with the parallel bond model employed as the particle contact constitutive model.First,twenty simulation tests were conducted to quantify the relationship between the macro–meso parameters.Then,nine orthogonal simulation tests were performed using four meso-mechanical parameters in a three-level to evaluate the sensitivity of the meso-mechanical parameters.Furthermore,the calibration method of the meso-parameters were then proposed.Finally,the contact force chain,the contact force and the contact number were examined to investigate the saturation effect on the meso-mechanical behavior of GHBC.The results show that:(1)The elastic modulus linearly increases with the bonding stiffness ratio and the friction coefficient while exponentially increasing with the normal bonding strength and the bonding radius coefficient.The failure strength increases exponentially with the increase of the friction coefficient,the normal bonding strength and the bonding radius coefficient,and remains constant with the increase of bond stiffness ratio;(2)The friction coefficient and the bond radius coefficient are most sensitive to the elastic modulus and the failure strength;(3)The number of the force chains,the contact force,and the bond strength between particles will increase with the increase of the hydrate saturation,which leads to the larger failure strength. 展开更多
关键词 Gas hydrate bearing coal Discrete element method Triaxial compression test Macro-meso mechanical propertie
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Multistage Microstructured Ionic Skin for Real-Time Vital Signs Monitoring and Human-Machine Interaction
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作者 Xueke Wang Jinyu Zi +5 位作者 Yi Chen qiang wu Zhimin Xiang Yongqiang Tu Peng Yang Yanfen Wan 《Energy & Environmental Materials》 SCIE EI CAS CSCD 2024年第6期218-229,共12页
Skin-like electronics research aiming to mimic even surpass human-like specific tactile cognition by operating perception-to-cognition-to-feedback of stimulus to build intelligent cognition systems for certain imperce... Skin-like electronics research aiming to mimic even surpass human-like specific tactile cognition by operating perception-to-cognition-to-feedback of stimulus to build intelligent cognition systems for certain imperceptible or inappreciable signals was so attractive.Herein,we constructed an all-in-one tri-modal pressure sensing wearable device to address the issue of power supply by integrating multistage microstructured ionic skin(MM i-skin)and thermoelectric self-power staffs,which exhibits high sensitivity simultaneously.The MM i-skin with multi-stage“interlocked”configurations achieved precise recognition of subtle signals,where the sensitivity reached up to 3.95 kPa^(−1),as well as response time of 46 ms,cyclic stability(over 1500 cycles),a wide detection range of 0–200 kPa.Furthermore,we developed the thermoelectricity nanogenerator,piezoelectricity nanogenerator,and piezocapacitive sensing as an integrated tri-modal pressure sensing,denoted as P-iskin,T-iskin,and C-iskin,respectively.This multifunctional ionic skin enables real-time monitoring of weak body signals,rehab guidance,and robotic motion recognition,demonstrating potential for Internet of things(IoT)applications involving the artificial intelligence-motivated sapiential healthcare Internet(SHI)and widely distributed human-machine interaction(HMI). 展开更多
关键词 bio-template method integrated device ionic skin skin-like microstructure tri-modal pressure sensing
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Loosely coordinating diluted highly concentrated electrolyte toward -60℃ Li metal batteries
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作者 Han Zhang Ziqi Zeng +5 位作者 qiang wu Xinlan Wang Mingsheng Qin Sheng Lei Shijie Cheng Jia Xie 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第3期380-387,I0009,共9页
Lithium metal batteries(LMBs) promise energy density over 400 Wh kg^(-1).However,they suffer severe electrochemical performance deterioration at sub-zero temperatures.Such failure behavior highly correlates to inferio... Lithium metal batteries(LMBs) promise energy density over 400 Wh kg^(-1).However,they suffer severe electrochemical performance deterioration at sub-zero temperatures.Such failure behavior highly correlates to inferior lithium metal anode(LMA) compatibility and sluggish Li^(+) desolvation.Here,we demonstrate that cyclopentylmethyl ether(CPME) based diluted high-concentration electrolyte(DHCE)enables-60℃ LMBs operation.By leveraging the loose coordination between Li^(+) and CPME,such developed electrolyte boosts the formation of ion clusters to derive anion-dominant interfacial chemistry for enhancing LMA compatibility and greatly accelerates Li^(+) desolvation kinetics.The resulting electrolyte demonstrates high Coulombic efficiencies(CE),providing over 99.5%,99.1%,98.5% and 95% at 25,-20,-40,and-60℃respectively.The assembled Li-S battery exhibits remarkable cyclic stability in-20,and-40℃ at 0.2 C charging and 0.5 C discharging.Even at-60℃,Li-S cell with this designed electrolyte retains> 70% of the initial capacity over 170 cycles.Besides,lithium metal coin cell and pouch cell with10 mg cm^(-2) high S cathode loading exhibit cycling stability at-20℃.This work offers an opportunity for rational designing electrolytes toward low temperature LMBs. 展开更多
关键词 Lithium metal batteries -60℃operation Lithium metal anode compatibility Li^(+) desolvation kinetics
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Effects of projectile parameters on the momentum transfer and projectile melting during hypervelocity impact
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作者 Wenjin Liu Qingming Zhang +6 位作者 Renrong Long Zizheng Gong Ren Jiankang Xin Hu Siyuan Ren qiang wu Guangming Song 《Defence Technology(防务技术)》 SCIE EI CAS CSCD 2024年第2期89-103,共15页
The effects of projectile/target impedance matching and projectile shape on energy,momentum transfer and projectile melting during collisions are investigated by numerical simulation.By comparing the computation resul... The effects of projectile/target impedance matching and projectile shape on energy,momentum transfer and projectile melting during collisions are investigated by numerical simulation.By comparing the computation results with the experimental results,the correctness of the calculation and the statistical method of momentum transfer coefficient is verified.Different shapes of aluminum,copper and heavy tungsten alloy projectiles striking aluminum,basalt,and pumice target for impacts up to 10 km/s are simulated.The influence mechanism of the shape of the projectile and projectile/target density on the momentum transfer was obtained.With an increase in projectile density and length-diameter ratio,the energy transfer time between the projectile and targets is prolonged.The projectile decelerates slowly,resulting in a larger cratering depth.The energy consumed by the projectile in the excavation stage increased,resulting in lower mass-velocity of ejecta and momentum transfer coefficient.The numerical simulation results demonstrated that for different projectile/target combinations,the higher the wave impedance of the projectile,the higher the initial phase transition velocity and the smaller the mass of phase transition.The results can provide theoretical guidance for kinetic impactor design and material selection. 展开更多
关键词 Hypervelocity impact Energy partitioning Impact melting Momentum transfer
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Plasma metabolites and risk of myocardial infarction:a bidirectional Mendelian randomization study
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作者 Dong-Hua LI qiang wu +10 位作者 Jing-Sheng LAN Shuo CHEN You-Yi HUANG Lan-Jin wu Zhi-Qing QIN Ying HUANG Wan-Zhong HUANG Ting ZENG Xin HAO Hua-Bin SU qiang SU 《Journal of Geriatric Cardiology》 SCIE CAS CSCD 2024年第2期219-231,共13页
BACKGROUND Myocardial infarction(MI)is a critical cardiovascular event with multifaceted etiology,involving several genetic and environmental factors.It is essential to understand the function of plasma metabolites in... BACKGROUND Myocardial infarction(MI)is a critical cardiovascular event with multifaceted etiology,involving several genetic and environmental factors.It is essential to understand the function of plasma metabolites in the development of MI and unravel its complex pathogenesis.METHODS This study employed a bidirectional Mendelian randomization(MR)approach to investigate the causal relationships between plasma metabolites and MI risk.We used genetic instruments as proxies for plasma metabolites and MI and conducted MR analyses in both directions to assess the impact of metabolites on MI risk and vice versa.In addition,the large-scale genome-wide association studies datasets was used to identify genetic variants associated with plasma metabolite(1400 metabolites)and MI(20,917 individuals with MI and 440,906 individuals without MI)susceptibility.Inverse variance weighted was the primary method for estimating causal effects.MR estimates are expressed as beta coefficients or odds ratio(OR)with 95%CI.RESULTS We identified 14 plasma metabolites associated with the occurrence of MI(P<0.05),among which 8 plasma metabolites[propionylglycine levels(OR=0.922,95%CI:0.881–0.965,P<0.001),gamma-glutamylglycine levels(OR=0.903,95%CI:0.861–0.948,P<0.001),hexadecanedioate(C16-DC)levels(OR=0.941,95%CI:0.911–0.973,P<0.001),pentose acid levels(OR=0.923,95%CI:0.877–0.972,P=0.002),X-24546 levels(OR=0.936,95%CI:0.902–0.971,P<0.001),glycine levels(OR=0.936,95%CI:0.909–0.964,P<0.001),glycine to serine ratio(OR=0.930,95%CI:0.888–0.974,P=0.002),and mannose to trans-4-hydroxyproline ratio(OR=0.912,95%CI:0.869–0.958,P<0.001)]were correlated with a decreased risk of MI,whereas the remaining 6 plasma metabolites[1-palmitoyl-2-arachidonoyl-GPE(16:0/20:4)levels(OR=1.051,95%CI:1.018–1.084,P=0.002),behenoyl dihydrosphingomyelin(d18:0/22:0)levels(OR=1.076,95%CI:1.027–1.128,P=0.002),1-stearoyl-2-docosahexaenoyl-GPE(18:0/22:6)levels(OR=1.067,95%CI:1.027–1.109,P=0.001),alpha-ketobutyrate levels(OR=1.108,95%CI:1.041–1.180,P=0.001),5-acetylamino-6-formylamino-3-methyluracil levels(OR=1.047,95%CI:1.019–1.076,P<0.001),and N-acetylputrescine to(N(1)+N(8))-acetylspermidine ratio(OR=1.045,95%CI:1.018–1.073,P<0.001)]were associated with an increased risk of MI.Furthermore,we also observed that the mentioned relationships were unaffected by horizontal pleiotropy(P>0.05).On the contrary,MI did not lead to significant alterations in the levels of the aforementioned 14 plasma metabolites(P>0.05 for each comparison).CONCLUSIONS Our bidirectional MR study identified 14 plasma metabolites associated with the occurrence of MI,among which 13 plasma metabolites have not been reported previously.These findings provide valuable insights for the early diagnosis of MI and potential therapeutic targets. 展开更多
关键词 INFARCTION alterations DIAGNOSIS
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Direct visualization of laser-driven dynamic fragmentation in tin by in situ x-ray diffraction
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作者 Jing Yang Xinxin Wang +9 位作者 Liang Xu Qiannan Wang Yi Sun Jiangtao Li Lin Zhang Yinghua Li Yuying Yu Pei Wang qiang wu Jianbo Hu 《Matter and Radiation at Extremes》 SCIE EI CSCD 2024年第5期109-114,共6页
We present a novel method for investigating laser-driven dynamic fragmentation in tin using in situ X-ray diffraction.Our experimental results demonstrate the feasibility of the method for simultaneously identifying t... We present a novel method for investigating laser-driven dynamic fragmentation in tin using in situ X-ray diffraction.Our experimental results demonstrate the feasibility of the method for simultaneously identifying the phase and temperature of fragments through analysis of the diffraction pattern.Surprisingly,we observe a deviation from the widely accepted isentropic release assumption,with the temperature of the fragments being found to be more than 100 K higher than expected,owing to the release of plastic work during dynamic fragmentation.Our findings are further verified through extensive large-scale molecular dynamics simulations,in which strain energies are found to be transferred into thermal energies during the nucleation and growth of voids,leading to an increase in temperature.Our findings thus provide crucial insights into the impact-driven dynamic fragmentation phenomenon and reveal the significant influence of plastic work on material response during shock release. 展开更多
关键词 DYNAMIC RELEASE DIFFRACTION
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TIL20: A review of island biogeography and habitat fragmentation studies on subtropical reservoir islands of Thousand Island Lake, China
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作者 Xingfeng Si Tinghao Jin +7 位作者 Wande Li Peng Ren qiang wu Di Zeng Xue Zhang Yuhao Zhao Chen Zhu Ping Ding 《Zoological Research(Diversity and Conservation)》 2024年第2期89-105,共17页
Reservoir islands formed by dam construction have the same history,clear boundaries,and large numbers that provide a natural platform for testing theories in ecology and biogeography.In this paper,we review studies of... Reservoir islands formed by dam construction have the same history,clear boundaries,and large numbers that provide a natural platform for testing theories in ecology and biogeography.In this paper,we review studies of multiple zoological taxa on reservoir islands of a large lake in eastern China(Thousand Island Lake).This lake,created in 1959,has 1078 artificial land-bridge islands of varying areas and isolation.Our review summarizes the decades-long studies in island biogeography and habitat fragmentation from this island system,grouped into three topics:species richness(“how many species are there”),community structure(“who are they”),and species interaction(“how they interact with each other”).Our findings support the predictions of the Equilibrium Theory of Island Biogeography and extend this theory to predict community structure of island faunas by moving beyond assumptions of species equivalency.In addition,the extensive studies on ecological networks,including mutualistic,antagonistic,and parasitic interactions,reveal the negative impacts of habitat loss on the maintenance of such networks,even as increasing forest edge enhances the robustness of pollination networks.At the end of this review,we proposed several future research directions based on current studies that are simultaneously at the frontier of ecology and biogeography. 展开更多
关键词 Biodiversity conservation Community assembly Species extinction ISLAND Species interaction
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2023年第3版《NCCN肿瘤临床实践指南:非小细胞肺癌》更新解读 被引量:9
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作者 朱玲玲 王艇 +6 位作者 伍娟 翟小倩 吴强 邓汉宇 秦昌龙 田龙 周清华 《中国肺癌杂志》 CAS CSCD 北大核心 2023年第6期407-415,共9页
肺癌是我国发病率和死亡率均居首位的恶性肿瘤,非小细胞肺癌(non-small cell lung cancer,NSCLC)是肺癌的主要病理学亚型。2023年4月13日,美国国立综合癌症网络(National Comprehensive Cancer Network,NCCN)发布了2023年第3版《NCCN肿... 肺癌是我国发病率和死亡率均居首位的恶性肿瘤,非小细胞肺癌(non-small cell lung cancer,NSCLC)是肺癌的主要病理学亚型。2023年4月13日,美国国立综合癌症网络(National Comprehensive Cancer Network,NCCN)发布了2023年第3版《NCCN肿瘤临床实践指南:非小细胞肺癌》,其反映了国际肺癌研究的最新进展。本文将对新版《指南》主要更新内容进行解读,并与2022年第3版NCCN指南相比较,旨在为我国临床医务人员诊治NSCLC提供参考。 展开更多
关键词 临床实践 肺肿瘤 NCCN指南 指南解读 循证医学证据
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1,3,5-Trifluorobenzene endorsed EC-free electrolyte for high-voltage and wide-temperature lithium-ion batteries 被引量:4
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作者 Mingsheng Qin Ziqi Zeng +4 位作者 qiang wu Xiaowei Liu Qijun Liu Shijie Cheng Jia Xie 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2023年第10期49-57,I0003,共10页
Ethylene carbonate(EC)is susceptible to the aggressive chemistry of nickel-rich cathodes,making it undesirable for high-voltage lithium-ion batteries(LIBs).The arbitrary elimination of EC leads to better oxidative tol... Ethylene carbonate(EC)is susceptible to the aggressive chemistry of nickel-rich cathodes,making it undesirable for high-voltage lithium-ion batteries(LIBs).The arbitrary elimination of EC leads to better oxidative tolerance but always incurs interfacial degradation and electrolyte decomposition.Herein,an EC-free electrolyte is deliberately developed based on gradient solvation by pairing solvation-protection agent(1,3,5-trifluorobenzene,F_(3)B)with propylene carbonate(PC)/methyl ethyl carbonate(EMC)formulation.F_(3)B keeps out of inner coordination shell but decomposes preferentially to construct robust interphase,inhibiting solvent decomposition and electrode corrosion.Thereby,the optimized electrolyte(1.1 M)with wide liquid range(-70–77℃)conveys decent interfacial compatibility and high-voltage stability(4.6 V for LiNi_(0.6)Mn_(0.2)Co_(0.2)O_(2),NCM622),qualifying reliable operation of practical NCM/graphite pouch cell(81.1%capacity retention over 600 cycles at 0.5 C).The solvation preservation and interface protection from F_(3)B blaze a new avenue for developing high-voltage electrolytes in next-generation LIBs. 展开更多
关键词 Lithium-ion batteries Solvation structure High-voltage electrolyte Wide-temperature range Interfacial chemistry
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Green‑Solvent Processed Blade‑Coating Organic Solar Cells with an Efficiency Approaching 19%Enabled by Alkyl‑Tailored Acceptors 被引量:2
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作者 Hairui Bai Ruijie Ma +23 位作者 Wenyan Su Top Archie Dela Pea Tengfei Li Lingxiao Tang Jie Yang Bin Hu Yilin Wang Zhaozhao Bi Yueling Su Qi Wei qiang wu Yuwei Duan Yuxiang Li Jiaying wu Zicheng Ding Xunfan Liao Yinjuan Huang Chao Gao Guanghao Lu Mingjie Li Weiguo Zhu Gang Li Qunping Fan Wei Ma 《Nano-Micro Letters》 SCIE EI CAS CSCD 2023年第12期449-462,共14页
Power-conversion-efficiencies(PCEs)of organic solar cells(OSCs)in laboratory,normally processed by spin-coating technology with toxic halogenated solvents,have reached over 19%.However,there is usually a marked PCE dr... Power-conversion-efficiencies(PCEs)of organic solar cells(OSCs)in laboratory,normally processed by spin-coating technology with toxic halogenated solvents,have reached over 19%.However,there is usually a marked PCE drop when the bladecoating and/or green-solvents toward large-scale printing are used instead,which hampers the practical development of OSCs.Here,a new series of N-alkyl-tailored small molecule acceptors named YR-SeNF with a same molecular main backbone are developed by combining selenium-fused central-core and naphthalene-fused endgroup.Thanks to the N-alkyl engineering,NIR-absorbing YR-SeNF series show different crystallinity,packing patterns,and miscibility with polymeric donor.The studies exhibit that the molecular packing,crystallinity,and vertical distribution of active layer morphologies are well optimized by introducing newly designed guest acceptor associated with tailored N-alkyl chains,providing the improved charge transfer dynamics and stability for the PM6:L8-BO:YRSeNF-based OSCs.As a result,a record-high PCE approaching 19%is achieved in the blade-coating OSCs fabricated from a greensolvent o-xylene with high-boiling point.Notably,ternary OSCs offer robust operating stability under maximum-power-point tracking and well-keep>80%of the initial PCEs for even over 400 h.Our alkyl-tailored guest acceptor strategy provides a unique approach to develop green-solvent and blade-coating processed high-efficiency and operating stable OSCs,which paves a way for industrial development. 展开更多
关键词 Alkyl-tailored guest acceptors Blade-coating Green solvent processing Stability Organic solar cells
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Dual-Functional Organotelluride Additive for Highly Efficient Sulfur Redox Kinetics and Lithium Regulation in Lithium–Sulfur Batteries 被引量:2
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作者 Wei Zhang Fenfen Ma +5 位作者 qiang wu Ziqi Zeng Wei Zhong Shijie Cheng Xin Chen Jia Xie 《Energy & Environmental Materials》 SCIE EI CAS CSCD 2023年第3期126-133,共8页
High energy density and low cost made lithium–sulfur(Li–S)batteries appealing for the next-generation energy storage devices.However,their commercial viability is seriously challenged by serious polysulfide shuttle ... High energy density and low cost made lithium–sulfur(Li–S)batteries appealing for the next-generation energy storage devices.However,their commercial viability is seriously challenged by serious polysulfide shuttle effect,sluggish sulfur kinetics,and uncontrollable dendritic Li growth.Herein,a dual-functional electrolyte additive,diphenyl ditelluride(DPDTe)is reported for Li–S battery.For sulfur cathodes,DPDTe works as a redox mediator to accelerate redox kinetics of sulfur,in which Te radical-mediated catalytic cycle at the solid–liquid interface contributes significantly to the whole process.For lithium anodes,DPDTe can react with lithium metal to form a smooth and stable organic–inorganic hybrid solid-electrolyte interphase(SEI),enabling homogeneous lithium deposition for suppressing dendrite growth.Consequently,the Li–S battery with DPDTe exhibits remarkable cycling stability and superb rate capability,with a high capacity up to 1227.3 mAh g^(-1)and stable cycling over 300 cycles.Moreover,a Li–S pouch cell with DPDTe is evaluated as the proof of concept.This work demonstrates that organotelluride compounds can be used as functional electrolyte additives and offers new insights and opportunities for practical Li–S batteries. 展开更多
关键词 electrolyte additive Li anode Li2 S deposition Li–S battery sulfur kinetics
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克罗恩病术后吻合口复发风险因素的研究进展
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作者 姚宝佳 杨理超 +1 位作者 吴强 刘刚磊 《医学新知》 CAS 2023年第6期478-483,共6页
肠道切除、重建是克罗恩病手术治疗的关键步骤,重建术后吻合口复发是其常见的并发症之一。因吻合口复发涉及较为复杂的后续处理,越来越受到炎症性肠病专科医生的重视。本文通过对克罗恩病术后吻合口复发的风险因素进行总结,以期为临床... 肠道切除、重建是克罗恩病手术治疗的关键步骤,重建术后吻合口复发是其常见的并发症之一。因吻合口复发涉及较为复杂的后续处理,越来越受到炎症性肠病专科医生的重视。本文通过对克罗恩病术后吻合口复发的风险因素进行总结,以期为临床实践提供参考。 展开更多
关键词 克罗恩病 吻合口复发 炎症性肠病
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Contamination and human health risk assessment of heavy metal(loid)s in topsoil and groundwater around mining and dressing factories in Chifeng,North China
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作者 Di Zhao qiang wu +9 位作者 Yifan Zeng Juan Zhang Aoshuang Mei Xiaohui Zhang Shuai Gao Hanyuan Wang Honglei Liu Yong Zhang Shuai Qi Xu Jia 《International Journal of Coal Science & Technology》 EI CAS CSCD 2023年第1期33-47,共15页
Chifeng is a concentrated mining area for non-ferrous metal minerals,as well as a key prevention and control area for heavyduty enterprises.This situation necessitates an efective ecological and human health risk asse... Chifeng is a concentrated mining area for non-ferrous metal minerals,as well as a key prevention and control area for heavyduty enterprises.This situation necessitates an efective ecological and human health risk assessment of heavy metal(loid)s driven by the wide distribution of metal ore processing,mining,and smelting factories in Hexigten Banner and Bairin Left Banner.We conducted surveys to assess the levels of heavy metal(loid)s(Cr,As,Pb,Cd,and Hg)in the topsoil and groundwater of the areas.The results indicated that the concentrations of As,Cd,and Pb in partial soil samples exceeded the environmental quality standards of Grade II.Based on contamination assessments,such as geoaccumulation indices and pollution indices,we inferred that Cd,Pb,and As were primary pollutants in topsoil.Potential ecological risks when considered as part of the average risk indices(RI)are up to 1626.40 and 2818.76,respectively,in the two areas.Comparative analysis revealed that Cd posed a very high potential ecological risk,followed by As.Moreover,the evaluation showed that the three exposure pathways of carcinogenic and non-carcinogenic risk followed a descending order:inhalation>ingestion>dermal contact,except for Pb.Arsenic in topsoil posed a potential non-carcinogenic risk to human health,while there were no adverse efects of As in groundwater.In addition,the average total carcinogenic risk for As in the two areas,as well as the risk of Pb in the topsoil of Bairin Left Banner and all the fve heavy metal(loid)s in groundwater,exceeded human tolerance.Pb–Zn mines caused higher human health risks.In addition,the tandem contamination of heavy metal(loid)s in soil and groundwater was not obvious.This research study provides a basis for pollution remediation to control heavy industry-induced ecological and health risks of heavy metal(loid)s. 展开更多
关键词 Heavy metal(loid)s Contamination indices Ecological risks Human health risks Chifeng
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Satellite breakup behaviors and model under the hypervelocity impact and explosion:A review
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作者 Si-yuan Ren Zi-zheng Gong +5 位作者 qiang wu Guang-ming Song Qing-ming Zhang Pin-liang Zhang Chuan Chen Yan Cao 《Defence Technology(防务技术)》 SCIE EI CAS CSCD 2023年第9期284-307,共24页
The primary causes of satellite breakups are hypervelocity impact and explosion,the research on satellite breakup can be used not only to evaluate the influence of breakup event on the space environment,but also to tr... The primary causes of satellite breakups are hypervelocity impact and explosion,the research on satellite breakup can be used not only to evaluate the influence of breakup event on the space environment,but also to trace whether the satellite has been deliberately attacked.It is of great significance in both civil and military aspects.The study of satellite breakup behaviors and model is reviewed to summarize the research progress and insufficiency in recent decades,including the satellite breakup experiment,measurement and characterization of fragments,distribution characteristics of breakup fragments,satellite breakup model,etc.The classical studies are introduced in detail,and the limitations of the current research are pointed out.According to the current research results,the contemporary challenges and future directions for satellite breakup study are presented.The research on satellite breakup is developing in two directions:the miniaturization of satellite size and the complexity of satellite component.The study on satellite breakup needs to be explored and deepened on improving the experimental launch speed,expanding the model application range and breakup revealing the results under combined effect of impact and explosion. 展开更多
关键词 Satellite breakup Space environment Distribution characteristics Hypervelocity impact Explosion
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Grand canonical Monte Carlo simulation study of hydrogen storage by Li-decorated pha-graphene
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作者 张蒙蒙 张凤 +7 位作者 吴强 黄欣 闫巍 赵春梅 陈伟 杨志红 王允辉 武婷婷 《Chinese Physics B》 SCIE EI CAS CSCD 2023年第6期476-480,共5页
Grand canonical Monte Carlo simulation(GCMCs)is utilized for studying hydrogen storage gravimetric density by pha-graphene at different metal densities,temperatures and pressures.It is demonstrated that the optimum ad... Grand canonical Monte Carlo simulation(GCMCs)is utilized for studying hydrogen storage gravimetric density by pha-graphene at different metal densities,temperatures and pressures.It is demonstrated that the optimum adsorbent location for Li atoms is the center of the seven-membered ring of pha-graphene.The binding energy of Li-decorated phagraphene is larger than the cohesive energy of Li atoms,implying that Li can be distributed on the surface of pha-graphene without forming metal clusters.We fitted the force field parameters of Li and C atoms at different positions and performed GCMCs to study the absorption capacity of H_(2).The capacity of hydrogen storage was studied by the differing density of Li decoration.The maximum hydrogen storage capacity of 4Li-decorated pha-graphene was 15.88 wt%at 77 K and100 bar.The enthalpy values of adsorption at the three densities are in the ideal range of 15 kJ·mol^(-1)-25 kJ·mol^(-1).The GCMC results at different pressures and temperatures show that with the increase in Li decorative density,the hydrogen storage gravimetric ratio of pha-graphene decreases but can reach the 2025 US Department of Energy's standard(5.5 wt%).Therefore,pha-graphene is considered to be a potential hydrogen storage material. 展开更多
关键词 hydrogen storage pha-graphene grand canonical Monte Carlo simulation(GCMCs) force field
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Numerical simulation of a truncated cladding negative curvature fiber sensor based on the surface plasmon resonance effect
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作者 张志超 苑金辉 +6 位作者 邱石 周桂耀 周娴 颜玢玢 吴强 王葵如 桑新柱 《Chinese Physics B》 SCIE EI CAS CSCD 2023年第3期262-269,共8页
A refractive index(RI)sensor based on the surface plasmon resonance effect is proposed using a truncated cladding negative curvature fiber(TC-NCF).The influences of the TC-NCF structure parameters on the sensing perfo... A refractive index(RI)sensor based on the surface plasmon resonance effect is proposed using a truncated cladding negative curvature fiber(TC-NCF).The influences of the TC-NCF structure parameters on the sensing performances are investigated and compared with the traditional NCF.The simulation results show that the proposed TC-NCF RI sensor has an ultra-wide detection range from 1.16 to 1.43.The maximum wavelength sensitivity reaches 12400 nm/RIU,and the corresponding R^(2)of the polynomial fitting equation is 0.9999.The maximum and minimum resolutions are 2.56×10^(-5)and 8.06×10^(-6),respectively.In addition,the maximum amplitude sensitivity can reach-379.1 RIU^(-1)when the RI is chosen as 1.43.The proposed TC-NCF RI sensor could be useful in biochemical medicine,environmental monitoring,and food safety. 展开更多
关键词 truncated cladding negative curvature fiber refractive index sensor surface plasmon resonance
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