Optical helicity provides us with an effective means to control the helicity-dependent photocurrent in the spinmomentum-locked surface states of topological insulators(TIs).Also,the TIs show potential in polarization ...Optical helicity provides us with an effective means to control the helicity-dependent photocurrent in the spinmomentum-locked surface states of topological insulators(TIs).Also,the TIs show potential in polarization detection as an intrinsic solid-state optical chirality detector for easier integration and fabrication.However,the complex photoresponses with the circular photogalvanic effect,the linear photogalvanic effect,and the photon drag effect in the TIs prevent them from direct chirality detection of the elliptically polarized light.Here,by fitting with the theoretical models to the measured photocurrents,the microscopic origin of different components of the helicity-dependent photocurrent has been demonstrated.We show a comprehensive study of the helicitydependent photocurrent in(Bi_(1-x)Sb_(x))_(2)Te_(3)thin films of different thicknesses as a function of the light incident angle and the gate-tuned chemical potential.The observation of the light incident angle dependence of the helicitydependent photocurrent provides us with a polarization detection strategy using a TI thin film without the use of any additional optical elements,and the detection accuracy can be enhanced by gate tuning.Additionally,the Stokes parameters can be extracted by arithmetic operation of photocurrents measured with different incident angles and gating voltages for complete characterization of the polarization states of a light beam.Using this means,we realize the polarization detection and the Stokes parameters analysis with a single device.Our work provides an alternative solution to develop miniaturized intrinsic polarization-sensitive photodetectors.展开更多
The growth and characterization of single-crystalline thin films of topological insulators(TIs)is an important step towards their possible applications.Using in situ scanning tunneling microscopy(STM)and angle-resolve...The growth and characterization of single-crystalline thin films of topological insulators(TIs)is an important step towards their possible applications.Using in situ scanning tunneling microscopy(STM)and angle-resolved photoemission spectroscopy(ARPES),we show that moderately thick Sb_(2)Te_(3)films grown layer-by-layer by molecular beam epitaxy(MBE)on Si(111)are atomically smooth,single-crystalline,and intrinsically insulating.Furthermore,these films were found to exhibit a robust TI electronic structure with their Fermi energy lying within the energy gap of the bulk that intersects only the Dirac cone of the surface states.Depositing Cs in situ moves the Fermi energy of the Sb_(2)Te_(3)films without changing the electronic band structure,as predicted by theory.We found that the TI behavior is preserved in Sb_(2)Te_(3)films down to five quintuple layers(QLs).展开更多
We have studied the magnetic and electrical transport properties of epitaxial NiAs-type CrTe thin films grown on SrTiO3(111) substrates. Unlike rectangle hysteresis loops obtained from magnetic measurements, we have...We have studied the magnetic and electrical transport properties of epitaxial NiAs-type CrTe thin films grown on SrTiO3(111) substrates. Unlike rectangle hysteresis loops obtained from magnetic measurements, we have identified intriguing extra bump/dip features from anomalous Hall experiments on the films with thicknesses less than 12 nm. This observed Hall anomaly is phenomenologically consistent with the occurrence of a topological Hall effect (THE) in chiral magnets with a skyrmion phase. Furthermore, the THE contribution can be tuned by the film thickness, showing the key contribution of asymmetric interfaces in stabilizing N6el-type skyrmions. Our work demonstrates that a CrTe thin film on SrTiO3(111) substrates is a good material candidate for studying real-space topological transport.展开更多
Pb nanobridges with a thickness of less than 10 nm and a width of several hundred nm have been fabricated from single-crystalline Pb fi lms using low-temperature molecular beam epitaxy and focus ion beam microfabricat...Pb nanobridges with a thickness of less than 10 nm and a width of several hundred nm have been fabricated from single-crystalline Pb fi lms using low-temperature molecular beam epitaxy and focus ion beam microfabrication techniques.We observed novel magnetoresistance oscillations below the superconducting transition temperature(TC)of the bridges.The oscillations which were not seen in the crystalline Pb fi lmsmay originate from the inhomogeneity of superconductivity induced by the applied magnetic fi elds on approaching the normal state,or the degradation of fi lm quality by thermal evolution.展开更多
The chirality associated with broken time-reversal symmetry in magnetically doped topological insulators has important implications for the quantum transport phenomena.Here we report anomalous Hall effect studies in M...The chirality associated with broken time-reversal symmetry in magnetically doped topological insulators has important implications for the quantum transport phenomena.Here we report anomalous Hall effect studies in Mn-and Cr-doped Bi_(2)Te_(3) topological insulators with varied thicknesses and doping contents.By tracing the magnitude of the anomalous Hall resistivity,we find that the Mn-type anomalous Hall effect characterized with clockwise chirality is strengthened by the reduction of film thickness,which is opposite to that of the Cr-type anomalous Hall effect with counterclockwise chirality.We provide a phenomenological physical picture to explain the evolution of the magnetic order and the anomalous Hall chirality in magnetically doped topological insulators.展开更多
基金National Natural Science Foundation of China(62074036,61674038,11574302)Foreign Cooperation Project of Fujian Province(2023I0005)+2 种基金Open Research Fund Program of the State Key Laboratory of Low-Dimensional Quantum Physics(KF202108)National Key Research and Development Program of China(2016YFB0402303)Foundation of Fujian Provincial Department of Industry and Information Technology(82318075)。
文摘Optical helicity provides us with an effective means to control the helicity-dependent photocurrent in the spinmomentum-locked surface states of topological insulators(TIs).Also,the TIs show potential in polarization detection as an intrinsic solid-state optical chirality detector for easier integration and fabrication.However,the complex photoresponses with the circular photogalvanic effect,the linear photogalvanic effect,and the photon drag effect in the TIs prevent them from direct chirality detection of the elliptically polarized light.Here,by fitting with the theoretical models to the measured photocurrents,the microscopic origin of different components of the helicity-dependent photocurrent has been demonstrated.We show a comprehensive study of the helicitydependent photocurrent in(Bi_(1-x)Sb_(x))_(2)Te_(3)thin films of different thicknesses as a function of the light incident angle and the gate-tuned chemical potential.The observation of the light incident angle dependence of the helicitydependent photocurrent provides us with a polarization detection strategy using a TI thin film without the use of any additional optical elements,and the detection accuracy can be enhanced by gate tuning.Additionally,the Stokes parameters can be extracted by arithmetic operation of photocurrents measured with different incident angles and gating voltages for complete characterization of the polarization states of a light beam.Using this means,we realize the polarization detection and the Stokes parameters analysis with a single device.Our work provides an alternative solution to develop miniaturized intrinsic polarization-sensitive photodetectors.
基金The work is supported by the National Natural Science Foundation of China(NSFC)the National Basic Research Program of the Ministry of Science and Technology of China(MOST)Work at Pennsylvania State University is supported by the National Science Foundation(NSF)under Grant No.DMR 0908700.
文摘The growth and characterization of single-crystalline thin films of topological insulators(TIs)is an important step towards their possible applications.Using in situ scanning tunneling microscopy(STM)and angle-resolved photoemission spectroscopy(ARPES),we show that moderately thick Sb_(2)Te_(3)films grown layer-by-layer by molecular beam epitaxy(MBE)on Si(111)are atomically smooth,single-crystalline,and intrinsically insulating.Furthermore,these films were found to exhibit a robust TI electronic structure with their Fermi energy lying within the energy gap of the bulk that intersects only the Dirac cone of the surface states.Depositing Cs in situ moves the Fermi energy of the Sb_(2)Te_(3)films without changing the electronic band structure,as predicted by theory.We found that the TI behavior is preserved in Sb_(2)Te_(3)films down to five quintuple layers(QLs).
文摘We have studied the magnetic and electrical transport properties of epitaxial NiAs-type CrTe thin films grown on SrTiO3(111) substrates. Unlike rectangle hysteresis loops obtained from magnetic measurements, we have identified intriguing extra bump/dip features from anomalous Hall experiments on the films with thicknesses less than 12 nm. This observed Hall anomaly is phenomenologically consistent with the occurrence of a topological Hall effect (THE) in chiral magnets with a skyrmion phase. Furthermore, the THE contribution can be tuned by the film thickness, showing the key contribution of asymmetric interfaces in stabilizing N6el-type skyrmions. Our work demonstrates that a CrTe thin film on SrTiO3(111) substrates is a good material candidate for studying real-space topological transport.
基金by the National Science Foundation and the Ministry of Science and Technology of China and the Penn.State MRSEC under NSF grant DMR-0820404.
文摘Pb nanobridges with a thickness of less than 10 nm and a width of several hundred nm have been fabricated from single-crystalline Pb fi lms using low-temperature molecular beam epitaxy and focus ion beam microfabrication techniques.We observed novel magnetoresistance oscillations below the superconducting transition temperature(TC)of the bridges.The oscillations which were not seen in the crystalline Pb fi lmsmay originate from the inhomogeneity of superconductivity induced by the applied magnetic fi elds on approaching the normal state,or the degradation of fi lm quality by thermal evolution.
基金This work was supported by the Basic Science Center Project of National Natural Science Foundation of China(Grant No.51788104)the National Key R&D Program of China(Grant Nos.2018YFA0307100,and 2018YFA0305603)This work was supported in part by the Beijing Advanced Innovation Center for Future Chip(ICFC).
文摘The chirality associated with broken time-reversal symmetry in magnetically doped topological insulators has important implications for the quantum transport phenomena.Here we report anomalous Hall effect studies in Mn-and Cr-doped Bi_(2)Te_(3) topological insulators with varied thicknesses and doping contents.By tracing the magnitude of the anomalous Hall resistivity,we find that the Mn-type anomalous Hall effect characterized with clockwise chirality is strengthened by the reduction of film thickness,which is opposite to that of the Cr-type anomalous Hall effect with counterclockwise chirality.We provide a phenomenological physical picture to explain the evolution of the magnetic order and the anomalous Hall chirality in magnetically doped topological insulators.