A large amount of real complex wastewaters are generated every year,which leads to a great environmental burden.Various treatment technologies were deployed to remove the contaminants in the wastewaters.However,these ...A large amount of real complex wastewaters are generated every year,which leads to a great environmental burden.Various treatment technologies were deployed to remove the contaminants in the wastewaters.However,these actual wastewaters have not been sufficiently treated due to their complex properties,high-concentration organics,incomplete utilization of hard-biodegradable substrates,the high energy input required,etc.Recently,microbial electrolysis cells(MECs),a great potential technology,has emerged for various wastewater treatment,because not only do they demonstrate satisfactory performance during wastewater treatment,but they also generate renewable H2 as a clean energy carrier.Unlike previous reviews,this review introduced the characteristics of every complicated wastewater,and focused on analyzing and summarizing MEC development for wastewater treatment.The performances of MECs were systematically reviewed in terms of organics removal,H2 production,Columbic efficiency,and energy efficiency.MEC performances for treating actual complex wastewaters and producing H2 can be optimized through operation parameters,electrode materials,catalyst materials,etc.In addition,the challenges and opportunities including complexity of wastewaters,instability of H2 production,robust microorganisms,effect of membrane on two-chamber MEC,and integration of MEC with other treatment processes were deeply discussed.Except for the technical feasibility,both environmental feasibility and economic feasibility also need to meet social requirements.This review can indeed provide a basis for high-efficiency treatment and practical commercial applications of recalcitrant wastewaters via MECs in the future.展开更多
Algal blooms have become a worldwide environmental concern due to water eutrophication.Dianchi Lake in Yunnan Province,China is suffering from severe eutrophication and is listed in the Three Important Lakes Restorati...Algal blooms have become a worldwide environmental concern due to water eutrophication.Dianchi Lake in Yunnan Province,China is suffering from severe eutrophication and is listed in the Three Important Lakes Restoration Act of China.Hydrothermal liquefaction allows a promising and direct conversion of algal biomass into biocrude oil.In this study,algal samples were collected from Dianchi Lake after a separation procedure including dissolved air flotation with polyaluminum chloride and centrifugation during four months,April,June,August and October.The algal biochemical components varied over the period;lipids from 0.7%to 2.1%ash-free dry weight(afdw),protein from 20.9%to 33.4%afdw and ash from 36.6%to 45.2%dry weight.The algae in June had the highest lipid and protein concentrations,leading to a maximum biocrude oil yield of 24.3%afdw.Biodiversity analysis using pyrosequencing revealed different distributions of microbial communities,specifically Microcystis in April(89.0%),June(63.7%)and August(84.0%),and Synechococcus in April(2.2%),June(12.0%)and August(1.0%).This study demonstrated remarkable temporal changes in the biochemical composition and biodiversity of algae harvested from Dianchi Lake and changes in biocrude oil production potential.展开更多
基金supported by China Postdoctoral Science Foundation(2018M641295)China Agriculture Research System(CARS-02)National Natural Science Foundation of China(51561145013).
文摘A large amount of real complex wastewaters are generated every year,which leads to a great environmental burden.Various treatment technologies were deployed to remove the contaminants in the wastewaters.However,these actual wastewaters have not been sufficiently treated due to their complex properties,high-concentration organics,incomplete utilization of hard-biodegradable substrates,the high energy input required,etc.Recently,microbial electrolysis cells(MECs),a great potential technology,has emerged for various wastewater treatment,because not only do they demonstrate satisfactory performance during wastewater treatment,but they also generate renewable H2 as a clean energy carrier.Unlike previous reviews,this review introduced the characteristics of every complicated wastewater,and focused on analyzing and summarizing MEC development for wastewater treatment.The performances of MECs were systematically reviewed in terms of organics removal,H2 production,Columbic efficiency,and energy efficiency.MEC performances for treating actual complex wastewaters and producing H2 can be optimized through operation parameters,electrode materials,catalyst materials,etc.In addition,the challenges and opportunities including complexity of wastewaters,instability of H2 production,robust microorganisms,effect of membrane on two-chamber MEC,and integration of MEC with other treatment processes were deeply discussed.Except for the technical feasibility,both environmental feasibility and economic feasibility also need to meet social requirements.This review can indeed provide a basis for high-efficiency treatment and practical commercial applications of recalcitrant wastewaters via MECs in the future.
基金the Chinese Universities Scientific Fund(2015SYL004).
文摘Algal blooms have become a worldwide environmental concern due to water eutrophication.Dianchi Lake in Yunnan Province,China is suffering from severe eutrophication and is listed in the Three Important Lakes Restoration Act of China.Hydrothermal liquefaction allows a promising and direct conversion of algal biomass into biocrude oil.In this study,algal samples were collected from Dianchi Lake after a separation procedure including dissolved air flotation with polyaluminum chloride and centrifugation during four months,April,June,August and October.The algal biochemical components varied over the period;lipids from 0.7%to 2.1%ash-free dry weight(afdw),protein from 20.9%to 33.4%afdw and ash from 36.6%to 45.2%dry weight.The algae in June had the highest lipid and protein concentrations,leading to a maximum biocrude oil yield of 24.3%afdw.Biodiversity analysis using pyrosequencing revealed different distributions of microbial communities,specifically Microcystis in April(89.0%),June(63.7%)and August(84.0%),and Synechococcus in April(2.2%),June(12.0%)and August(1.0%).This study demonstrated remarkable temporal changes in the biochemical composition and biodiversity of algae harvested from Dianchi Lake and changes in biocrude oil production potential.
