The Zeeman splitting effect is observed in a strong magnetic field generated by a laser-driven coil.The expanding plasma from the coil wire surface is concentrated at the coil center and interacts with the simultaneou...The Zeeman splitting effect is observed in a strong magnetic field generated by a laser-driven coil.The expanding plasma from the coil wire surface is concentrated at the coil center and interacts with the simultaneously generated magnetic field.The Cu I spectral lines at wavelengths of 510.5541,515.3235,and 521.8202 nm are detected and analyzed.The splittings of spectral lines are used to estimate the magnetic field strength at the coil center as∼31.4±15.7 T at a laser intensity of∼5.6310^(15) W/cm^(2),which agrees well with measurements using a B-dot probe.Some other plasma parameters of the central plasma disk are also studied.The temperature is evaluated from the Cu I spectral line intensity ratio,while the electron density is estimated from the Stark broadening effect.展开更多
We systematically investigate the influences of the input infrared spectrum, chirp, and polarization on the emitted intense terahertz spectrum and spatial dispersion in lithium niobate via optical rectification. The t...We systematically investigate the influences of the input infrared spectrum, chirp, and polarization on the emitted intense terahertz spectrum and spatial dispersion in lithium niobate via optical rectification. The terahertz yield and emission spectrum depend on both the chirp and spectrum of the input pump laser pulses. We also observe slight non-uniform spatial dispersion using a knife-edge measurement, which agrees well with the original predictions. The possible mechanism is the nonlinear distortion effect caused by high-energy laser pumping.Our study is very important and useful for developing intense terahertz systems with applications in extreme terahertz sciences and nonlinear phenomena.展开更多
We propose a spatial diffraction diagnostic method via inserting a millimeter-gap double slit into the collimated terahertz beam to monitor the minute variation of the terahertz beam in strong-field terahertz sources,...We propose a spatial diffraction diagnostic method via inserting a millimeter-gap double slit into the collimated terahertz beam to monitor the minute variation of the terahertz beam in strong-field terahertz sources,which is difficult to be resolved in conventional terahertz imaging systems.To verify the method,we intentionally fabricate tiny variations of the terahertz beam through tuning the iris for the infrared pumping beam before the tilted-pulse-front pumping setups.The phenomena can be well explained by the theory based on the tilted-pulse-front technique and terahertz diffraction.展开更多
To realize large-scale micro/nanofabrication process in superconducting devices,the nano laser direct writing(NLDW)as a potential tool was implemented.In this paper,thermal effect induced laser-matter(superconducting ...To realize large-scale micro/nanofabrication process in superconducting devices,the nano laser direct writing(NLDW)as a potential tool was implemented.In this paper,thermal effect induced laser-matter(superconducting film)interaction based on laser direct writing on Nb films and laser exposure on photoresist were investigated by simulation and experiment.To avoid nanoscale thermal effect on superconducting films,large-scale superconducting nanoarrays with the area up to 100μm×100μm based on laser exposure on photoresist were fabricated.Compared with laser direct writing on superconducting films,which lead to the degradation of superconducting performance such as critical current,transition temperature,the superconducting nanoarrays based on laser exposure on photoresist maintain excellent superconducting performance without degradation.Besides that,by further optimizing the process parameters and the thickness of photoresist,the nanowires with the width down to nanometers are plausible.Compared with the traditional electron beam and ion beam process,to some extent,the nanowires fabrication process based on NLDW provides a more efficient and cost-effective path for the fabrication of large-area superconducting devices/circuits.展开更多
A novel polyimide-inlaid amine-rich porous organic block copolymer(PI-b-ARPOP) was prepared via one-step polymerization by using different molar ratios of melamine(MA)/terephthalaldehyde(TA)/pyromellitic dianhydride(P...A novel polyimide-inlaid amine-rich porous organic block copolymer(PI-b-ARPOP) was prepared via one-step polymerization by using different molar ratios of melamine(MA)/terephthalaldehyde(TA)/pyromellitic dianhydride(PMDA), at molar ratios of 4/3/1, 4/2/2 and 4/1/3. The copolymer contained both aminal groups belonging to ARPOP and imide groups belonging to PI, and the bonding styles of the monomers and growth orientations of the polymeric chains were diversiform, forming an excellent porous structure. Notably, MA/TA/PMDA(4/2/2) had a surface area and pore volume of 487.27 m^2/g and 1.169 cm^3/g,respectively. The adsorption performance of the materials towards 2,4-dichlorophenol(2,4-DCP) in ultra-pure water was systematically studied. The pH value of 7 was optimal in aqueous solution. Na^+ and Cl^-ions did not negatively affect the adsorption process, while humic acid(HA) slightly decreased the capacity. The equilibrium time was 40 sec, and the maximum adsorption capacity reached 282.49 mg/g at 298 K. The removal process was endothermic and spontaneous, and the copolymer could maintain its porous structure and consistent performance after regeneration by treatment with alkali. Moreover, to further assess the practical applicability of the material, the adsorption performance towards 2,4-DCP in river water was also investigated. This paper demonstrated that the PI-b-ARPOP can be an efficient and practical adsorbent to remove chlorophenols from aqueous solution.展开更多
基金This work was supported in part by the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant Nos.XDA25010100,XDA25010300,and XDA25030100)the National Natural Science Foundation of China(Grant Nos.U1930107 and 11827807)the Japanese Ministry of Education,Science,Sports,and Culture through Grants-in-Aid,KAKENHI(Grant No.21H04454).
文摘The Zeeman splitting effect is observed in a strong magnetic field generated by a laser-driven coil.The expanding plasma from the coil wire surface is concentrated at the coil center and interacts with the simultaneously generated magnetic field.The Cu I spectral lines at wavelengths of 510.5541,515.3235,and 521.8202 nm are detected and analyzed.The splittings of spectral lines are used to estimate the magnetic field strength at the coil center as∼31.4±15.7 T at a laser intensity of∼5.6310^(15) W/cm^(2),which agrees well with measurements using a B-dot probe.Some other plasma parameters of the central plasma disk are also studied.The temperature is evaluated from the Cu I spectral line intensity ratio,while the electron density is estimated from the Stark broadening effect.
基金National Basic Research Program of China(2013CBA01501)National Natural Science Foundation of China(NSFC)(11334013,11520101003,11861121001,U1530150)+4 种基金Strategic Priority Research Program of the Chinese Academy of Sciences(CAS)(XDB07030300,XDB16010200,XDB17030500)National Science Foundation(NSF)(0968895,1102301,1263236)863 Program(2013AA014402)“Zhuoyue” Program(ZG216S1807)“Qingba” Program(KG12052501,ZG226S1832)
文摘We systematically investigate the influences of the input infrared spectrum, chirp, and polarization on the emitted intense terahertz spectrum and spatial dispersion in lithium niobate via optical rectification. The terahertz yield and emission spectrum depend on both the chirp and spectrum of the input pump laser pulses. We also observe slight non-uniform spatial dispersion using a knife-edge measurement, which agrees well with the original predictions. The possible mechanism is the nonlinear distortion effect caused by high-energy laser pumping.Our study is very important and useful for developing intense terahertz systems with applications in extreme terahertz sciences and nonlinear phenomena.
基金the Science Challenge Project(No.TZ2016005)the NationalNatural Science Foundation of China(Nos.11827807,61905007,11520101003,and 11861121001)the Strategic Priority Research Programof the Chinese Academy of Sciences(No.XDB16010200)。
文摘We propose a spatial diffraction diagnostic method via inserting a millimeter-gap double slit into the collimated terahertz beam to monitor the minute variation of the terahertz beam in strong-field terahertz sources,which is difficult to be resolved in conventional terahertz imaging systems.To verify the method,we intentionally fabricate tiny variations of the terahertz beam through tuning the iris for the infrared pumping beam before the tilted-pulse-front pumping setups.The phenomena can be well explained by the theory based on the tilted-pulse-front technique and terahertz diffraction.
基金supported by the National Natural Science Foundation of China(No.12104112)the Natural Science Foundation of Shandong Province(No.ZR2021QA036).
文摘To realize large-scale micro/nanofabrication process in superconducting devices,the nano laser direct writing(NLDW)as a potential tool was implemented.In this paper,thermal effect induced laser-matter(superconducting film)interaction based on laser direct writing on Nb films and laser exposure on photoresist were investigated by simulation and experiment.To avoid nanoscale thermal effect on superconducting films,large-scale superconducting nanoarrays with the area up to 100μm×100μm based on laser exposure on photoresist were fabricated.Compared with laser direct writing on superconducting films,which lead to the degradation of superconducting performance such as critical current,transition temperature,the superconducting nanoarrays based on laser exposure on photoresist maintain excellent superconducting performance without degradation.Besides that,by further optimizing the process parameters and the thickness of photoresist,the nanowires with the width down to nanometers are plausible.Compared with the traditional electron beam and ion beam process,to some extent,the nanowires fabrication process based on NLDW provides a more efficient and cost-effective path for the fabrication of large-area superconducting devices/circuits.
基金supported by the National Natural Scientific Foundation of China (Nos. 21477118, 51478445)the Open Projects Foundation of State Key Laboratory of Optical Fiber and Cable Manufacture Technology (YOFC) (No. 1604)
文摘A novel polyimide-inlaid amine-rich porous organic block copolymer(PI-b-ARPOP) was prepared via one-step polymerization by using different molar ratios of melamine(MA)/terephthalaldehyde(TA)/pyromellitic dianhydride(PMDA), at molar ratios of 4/3/1, 4/2/2 and 4/1/3. The copolymer contained both aminal groups belonging to ARPOP and imide groups belonging to PI, and the bonding styles of the monomers and growth orientations of the polymeric chains were diversiform, forming an excellent porous structure. Notably, MA/TA/PMDA(4/2/2) had a surface area and pore volume of 487.27 m^2/g and 1.169 cm^3/g,respectively. The adsorption performance of the materials towards 2,4-dichlorophenol(2,4-DCP) in ultra-pure water was systematically studied. The pH value of 7 was optimal in aqueous solution. Na^+ and Cl^-ions did not negatively affect the adsorption process, while humic acid(HA) slightly decreased the capacity. The equilibrium time was 40 sec, and the maximum adsorption capacity reached 282.49 mg/g at 298 K. The removal process was endothermic and spontaneous, and the copolymer could maintain its porous structure and consistent performance after regeneration by treatment with alkali. Moreover, to further assess the practical applicability of the material, the adsorption performance towards 2,4-DCP in river water was also investigated. This paper demonstrated that the PI-b-ARPOP can be an efficient and practical adsorbent to remove chlorophenols from aqueous solution.