Ability of epitaxial perovskite oxide ferroelectric films to maintain a poled polarization state on a long-term scale is crucial for advanced devices employing such films.Here polarization relaxation with time,or agin...Ability of epitaxial perovskite oxide ferroelectric films to maintain a poled polarization state on a long-term scale is crucial for advanced devices employing such films.Here polarization relaxation with time,or aging,is experimentally studied in epitaxial capacitor heterostructures of PbTiO3 sandwiched between SrRuO_(3)and Pt electrodes.The relaxation obeys logarithmic time-decay for the time 10^(2)–10^(5)s after poling pulses.The decay is by factor10 slower than that reported for polycrystalline films.Our experimental results show that existing models are insufficient for epitaxial films.展开更多
基金the Finnish Funding Agency for Innovation(Grant No.400.31.2013).
文摘Ability of epitaxial perovskite oxide ferroelectric films to maintain a poled polarization state on a long-term scale is crucial for advanced devices employing such films.Here polarization relaxation with time,or aging,is experimentally studied in epitaxial capacitor heterostructures of PbTiO3 sandwiched between SrRuO_(3)and Pt electrodes.The relaxation obeys logarithmic time-decay for the time 10^(2)–10^(5)s after poling pulses.The decay is by factor10 slower than that reported for polycrystalline films.Our experimental results show that existing models are insufficient for epitaxial films.
