The process of photocatalysis,regarded as a promising approach for tackling the energy crisis and environmental pollution issues,is crucial for turning solar light into chemical resources.However,the solar-chemical co...The process of photocatalysis,regarded as a promising approach for tackling the energy crisis and environmental pollution issues,is crucial for turning solar light into chemical resources.However,the solar-chemical conversion efficiency of typical semiconductor catalysts is still too low,so it is vital to figure out how to boost photocatalytic performance of semiconductors.Under visible light illumination,the local surface plasmon resonance(LSPR)induced by coinage metal would enhance the local electric field and improve photocatalytic performance of semiconductors,especially in the visible range.Therefore,its attachment to semiconductors has been regarded as an efficient strategy to improve photocatalytic performance.This paper reviews the latest research progress of plasmonic photocatalysis from theory to application.Starting from the excitation and relaxation of plasmons,four main mechanisms of plasmon-enhanced semiconductor photocatalysis are introduced,including enhanced light absorption and scattering,local electromagnetic field enhancement,improved hot carriers(HCs)injection and enhanced thermal effect.Secondly,the current mainstream plasmonic photocatalysts,such as monometallic,bimetallic and non-noble metal-based plasmonic catalysts,are reviewed.Finally,the applications of plasmonic photocatalysts in H_(2) production,CO_(2) reduction,and antibacterial are further summarized.展开更多
A brief review of recent progress in researches, productions and applications of full distributed fiber Raman photon sensors at China Jiliang University (CJLU) is presented. In order to improve the measurement dista...A brief review of recent progress in researches, productions and applications of full distributed fiber Raman photon sensors at China Jiliang University (CJLU) is presented. In order to improve the measurement distance, the accuracy, the space resolution, the ability of multi-parameter measurements, and the intelligence of full distributed fiber sensor systems, a new generation fiber sensor technology based on the optical fiber nonlinear scattering fusion principle is proposed. A series of new generation full distributed fiber sensors are investigated and designed, which consist of new generation ultra-long distance full distributed fiber Raman and Rayleigh scattering photon sensors integrated with a fiber Raman amplifier, auto-correction full distributed fiber Raman photon temperature sensors based on Raman correlation dual sources, full distributed fiber Raman photon temperature sensors based on a pulse coding source, full distributed fiber Raman photon temperature sensors using a fiber Raman wavelength shifter, a new type of Brillouin optical time domain analyzers (BOTDAs) integrated with a fiber Raman amplifier for replacing a fiber Brillouin amplifier, full distributed fiber Raman and Brillouin photon sensors integrated with a fiber Raman amplifier, and full distributed fiber Brillouin photon sensors integrated with a fiber Brillouin frequency shifter. The Internet of things is believed as one of candidates of the next technological revolution, which has driven hundreds of millions of class markets. Sensor networks are important components of the Internet of things. The full distributed optical fiber sensor network (Rayleigh, Raman, and Brillouin scattering) is a 3S (smart materials, smart structure, and smart skill) system, which is easy to construct smart fiber sensor networks. The distributed optical fiber sensor can be embedded in the power grids, railways, bridges, tunnels, roads, constructions, water supply systems, dams, oil and gas pipelines and other facilities, and can be integrated with wireless networks.展开更多
基金supported by the National Key Research and Development Program of China(2019YFA0705400)the National Natural Science Foundation of China(22104124,22005130,22272069,and 22104135)+1 种基金the State Key Laboratory of Fine Chemicals,Dalian University of Technology(KF2002)the Fundamental Research Funds for the Central Universities(20720220117).
文摘The process of photocatalysis,regarded as a promising approach for tackling the energy crisis and environmental pollution issues,is crucial for turning solar light into chemical resources.However,the solar-chemical conversion efficiency of typical semiconductor catalysts is still too low,so it is vital to figure out how to boost photocatalytic performance of semiconductors.Under visible light illumination,the local surface plasmon resonance(LSPR)induced by coinage metal would enhance the local electric field and improve photocatalytic performance of semiconductors,especially in the visible range.Therefore,its attachment to semiconductors has been regarded as an efficient strategy to improve photocatalytic performance.This paper reviews the latest research progress of plasmonic photocatalysis from theory to application.Starting from the excitation and relaxation of plasmons,four main mechanisms of plasmon-enhanced semiconductor photocatalysis are introduced,including enhanced light absorption and scattering,local electromagnetic field enhancement,improved hot carriers(HCs)injection and enhanced thermal effect.Secondly,the current mainstream plasmonic photocatalysts,such as monometallic,bimetallic and non-noble metal-based plasmonic catalysts,are reviewed.Finally,the applications of plasmonic photocatalysts in H_(2) production,CO_(2) reduction,and antibacterial are further summarized.
文摘A brief review of recent progress in researches, productions and applications of full distributed fiber Raman photon sensors at China Jiliang University (CJLU) is presented. In order to improve the measurement distance, the accuracy, the space resolution, the ability of multi-parameter measurements, and the intelligence of full distributed fiber sensor systems, a new generation fiber sensor technology based on the optical fiber nonlinear scattering fusion principle is proposed. A series of new generation full distributed fiber sensors are investigated and designed, which consist of new generation ultra-long distance full distributed fiber Raman and Rayleigh scattering photon sensors integrated with a fiber Raman amplifier, auto-correction full distributed fiber Raman photon temperature sensors based on Raman correlation dual sources, full distributed fiber Raman photon temperature sensors based on a pulse coding source, full distributed fiber Raman photon temperature sensors using a fiber Raman wavelength shifter, a new type of Brillouin optical time domain analyzers (BOTDAs) integrated with a fiber Raman amplifier for replacing a fiber Brillouin amplifier, full distributed fiber Raman and Brillouin photon sensors integrated with a fiber Raman amplifier, and full distributed fiber Brillouin photon sensors integrated with a fiber Brillouin frequency shifter. The Internet of things is believed as one of candidates of the next technological revolution, which has driven hundreds of millions of class markets. Sensor networks are important components of the Internet of things. The full distributed optical fiber sensor network (Rayleigh, Raman, and Brillouin scattering) is a 3S (smart materials, smart structure, and smart skill) system, which is easy to construct smart fiber sensor networks. The distributed optical fiber sensor can be embedded in the power grids, railways, bridges, tunnels, roads, constructions, water supply systems, dams, oil and gas pipelines and other facilities, and can be integrated with wireless networks.