The Shanghai laser electron gamma source(SLEGS)is a powerful tool for exploring photonuclear physics,such as giant dipole resonance(GDR)and pygmy dipole resonance,which are the main mechanisms of collective nuclear mo...The Shanghai laser electron gamma source(SLEGS)is a powerful tool for exploring photonuclear physics,such as giant dipole resonance(GDR)and pygmy dipole resonance,which are the main mechanisms of collective nuclear motion.The goal of the SLEGS neutron time-of-flight(TOF)spectrometer is to measure GDR and specific nuclear structures in the energy region above the neutron threshold.The SLEGS TOF spectrometer was designed to hold 20 sets of EJ301 and LaBr3 detectors.Geant4 was used to simulate the efficiency of each detector and the entire spectrometer,which provides a reference for the selection of detectors and layout of the SLEGS TOF spectrometer.Under the events of 208Pb,implementations of coincidence and time-of-flight technology for complex experiments are available;thus,and neutron decay events can be separated.The performance of SLEGS TOF spectrometer was systematically evaluated using offline experiments,in which the time resolution reached approximately 0.9 ns.展开更多
The Shanghai Laser Electron Gamma Source(SLEGS)is a powerful gamma source that provides MeV gamma-ray beams for nuclear science and technology.It was developed as one of the 16 beamline stations in the Phase Ⅱ Projec...The Shanghai Laser Electron Gamma Source(SLEGS)is a powerful gamma source that provides MeV gamma-ray beams for nuclear science and technology.It was developed as one of the 16 beamline stations in the Phase Ⅱ Project of the Shanghai Synchrotron Radiation Facility.The slant-scattering mode is for the first time systematically employed in laser Compton scattering at SLEGS to produce energy-tunable quasi-monoenergetic gamma-ray beams.The SLEGS officially completed its commissioning from July to December 2021.Gamma rays in the energy range of 0.25-21.7 MeV with a flux of 2.1×10^(4)-1.2×10^(7) photons/s and an energy spread of 2-15% were produced during the test.This paper reports the results from commissioning the SLEGS beamline.展开更多
Silver indium cadmium(Ag–In–Cd) control rod is widely used in pressurized water reactor nuclear power plants,and it is continuously consumed in a high neutron flux environment. The mass ratio of ^(107)Ag in the Ag...Silver indium cadmium(Ag–In–Cd) control rod is widely used in pressurized water reactor nuclear power plants,and it is continuously consumed in a high neutron flux environment. The mass ratio of ^(107)Ag in the Ag–In–Cd control rod is 41.44%. To accurately calculate the consumption value of the control rod, a reliable neutron reaction cross section of the ^(107)Ag is required. Meanwhile,^(107)Ag is also an important weak r nucleus. Thus, the cross sections for neutron induced interactions with ^(107)Ag are very important both in nuclear energy and nuclear astrophysics. The(n, γ) cross section of ^(107)Ag has been measured in the energy range of 1–60 eV using a back streaming white neutron beam line at China spallation neutron source. The resonance parameters are extracted by an R-matrix code. All the cross section of ^(107)Ag and resonance parameters are given in this paper as datasets. The datasets are openly available at http://www.doi.org/10.11922/sciencedb.j00113.00010.展开更多
The Closeby Habitable Exoplanet Survey(CHES) mission is proposed to discover habitable-zone Earth-like planets of nearby solar-type stars(~10 pc away from our solar system) via microarcsecond relative astrometry.The m...The Closeby Habitable Exoplanet Survey(CHES) mission is proposed to discover habitable-zone Earth-like planets of nearby solar-type stars(~10 pc away from our solar system) via microarcsecond relative astrometry.The major scientific objectives of CHES are:to search for Earth Twins or terrestrial planets in habitable zones orbiting100 FGK nearby stars;further to conduct a comprehensive survey and extensively characterize nearby planetary systems.The primary payload is a high-quality,low-distortion,high-stability telescope.The optical subsystem is a coaxial three-mirror anastigmat(TMA) with a 1.2 m-aperture,0°.44 × 0°.44 field of view and 500 nm-900 nm working wave band.The camera focal plane is composed of a mosaic of 81 scientific CMOS detectors each with4 k × 4 k pixels.The heterodyne laser interferometric calibration technology is employed to ensure microarcsecond level(1 μas) relative astrometry precision to meet the requirements for detection of Earth-like planets.The CHES satellite operates at the Sun-Earth L2 point and observes all the target stars for 5 yr.CHES will offer the first direct measurements of true masses and inclinations of Earth Twins and super-Earths orbiting our neighbor stars based on microarcsecond astrometry from space.This will definitely enhance our understanding of the formation of diverse nearby planetary systems and the emergence of other worlds for solar-type stars,and finally provide insights to the evolution of our own solar system.展开更多
The^(74)Se is one of 35 p-nuclei,and^(82)Se is a r-process only nucleus,and their(n,γ)cross sections are vital input parameters for nuclear astrophysics reaction network calculations.The neutron capture cross section...The^(74)Se is one of 35 p-nuclei,and^(82)Se is a r-process only nucleus,and their(n,γ)cross sections are vital input parameters for nuclear astrophysics reaction network calculations.The neutron capture cross section in the resonance range of isotopes and even natural selenium samples has not been measured.Promptγ-rays originating from neutron-induced capture events were detected by four C_(6)D_(6) liquid scintillator detectors at the Back-n facility of China Spallation Neutron Source(CSNS).The pulse height weighting technique(PHWT)was used to analyze the data in the 1 e V to 100 ke V region.The deduced neutron capture cross section was compared with ENDF/B-VIII.0,JEFF-3.2,and JENDL-4.0,and some differences were found.Resonance parameters were extracted by the R-matrix code SAMMY in the 1 e V-1 ke V region.All the cross sections ofnatSe and resonance parameters are given in the datasets.The datasets are openly available at http://www.doi.org/10.11922/sciencedb.j00113.00019.展开更多
Antigen 12, containing a phosphonyl peptide hapten with free C-terminal carboxylic group, was synthesized by 11 reaction steps. The design of the hapten was based on the transition state of peptide hydrolysis catalyze...Antigen 12, containing a phosphonyl peptide hapten with free C-terminal carboxylic group, was synthesized by 11 reaction steps. The design of the hapten was based on the transition state of peptide hydrolysis catalyzed by carboxypeptidase A.展开更多
The monoclonal antibody ID11D7 to carboxypeptidase A (CPA) was prepared. Theinhibitory effect of McAb ID11D7 on the peptidase activity of CPA was measured. The result reflectsthat the McAb ID11D7 can competitively inh...The monoclonal antibody ID11D7 to carboxypeptidase A (CPA) was prepared. Theinhibitory effect of McAb ID11D7 on the peptidase activity of CPA was measured. The result reflectsthat the McAb ID11D7 can competitively inhibit the peptidase activity of CPA with an apparentinhibitory constant of 6.3 × 10-9M. Based on this work. the McAb ID11D7 can be used as idiotypicantigen to prepare anti-idiotypic catalytic antibody with the peptidase activity similar to CPA.展开更多
1, 5-Benzothiazepines 1 react with phenylacetyl chloride to give the title compounds.The structures of these new compounds were confirmed by elemental analysis, ~1H NMR, ^(13)C NMRand MS spectroscopy, and their config...1, 5-Benzothiazepines 1 react with phenylacetyl chloride to give the title compounds.The structures of these new compounds were confirmed by elemental analysis, ~1H NMR, ^(13)C NMRand MS spectroscopy, and their configuration (the mutual positions of the substituents relative to theβ-lactam ring) and conformation of the compounds were determined by X-ray crystal analysis.展开更多
The Damocloids are a group of unusual asteroids that recently added a new member： 2010 EJ104. The dynamical evolution of the Damocloids may reveal a connection from the Main Belt to the Kuiper Belt and beyond the sca...The Damocloids are a group of unusual asteroids that recently added a new member： 2010 EJ104. The dynamical evolution of the Damocloids may reveal a connection from the Main Belt to the Kuiper Belt and beyond the scattered disk. According to our simulations, two regions may be considered as possible origins of the Damocloids： the scattered disk, or a part of the Oort cloud, which will be perturbed to a transient region located between 700 AU and 1000 AU. Based on their potential origin, the Damocloids can be classified into two types, depending on their semi-major axes, and about 65.5% of the Damocloids are classified into type I which mainly originate from the Oort cloud. Whether the Damocloids are inactive nuclei of the Halley Family of Comets may depend on their origin. K展开更多
The intramolecular reductive coupling reaction of 1,6-bis(subshtuted indolyl)hexane-1,6-dione using zero-valent titanium reagent as catalyst proderes the novel photochromic 1,2-diheterocyclic cyclohexenes 2, together ...The intramolecular reductive coupling reaction of 1,6-bis(subshtuted indolyl)hexane-1,6-dione using zero-valent titanium reagent as catalyst proderes the novel photochromic 1,2-diheterocyclic cyclohexenes 2, together with unexpected compounds 3展开更多
Twenty-seven oxadiazolino[5,4-d][1,5]benzodiheteropine derivatives have been synthesized by the 1,3-dipolar cycloaddition of benzodiheteropines with nitrile oxide 1,3-dipoles,their conformations and the characteristic...Twenty-seven oxadiazolino[5,4-d][1,5]benzodiheteropine derivatives have been synthesized by the 1,3-dipolar cycloaddition of benzodiheteropines with nitrile oxide 1,3-dipoles,their conformations and the characteristics of the newly formed oxadiazoline fused on them have been studied.It has also been found that the mass spectra show characteristic fragmentation patterns.展开更多
A dodecapeptide extracted from rape pollen was synthesized using solid—phase method,its conforma- tions in different states were studied by FT—IR,CD,and its physiological activities were determined.Seven segments an...A dodecapeptide extracted from rape pollen was synthesized using solid—phase method,its conforma- tions in different states were studied by FT—IR,CD,and its physiological activities were determined.Seven segments and five analogs were also synthesized to elucidate the structure—function relation.展开更多
基金supported by the National Natural Science Foundation of China (Nos.12275338,12005280,11905274 and 11875311)the Key Laboratory of Nuclear Data foundation (JCKY2022201C152)+1 种基金National key research and development program (No.2022YFA1602404)the Strategic Priority Research Program of the CAS (No.XDB34030000).
文摘The Shanghai laser electron gamma source(SLEGS)is a powerful tool for exploring photonuclear physics,such as giant dipole resonance(GDR)and pygmy dipole resonance,which are the main mechanisms of collective nuclear motion.The goal of the SLEGS neutron time-of-flight(TOF)spectrometer is to measure GDR and specific nuclear structures in the energy region above the neutron threshold.The SLEGS TOF spectrometer was designed to hold 20 sets of EJ301 and LaBr3 detectors.Geant4 was used to simulate the efficiency of each detector and the entire spectrometer,which provides a reference for the selection of detectors and layout of the SLEGS TOF spectrometer.Under the events of 208Pb,implementations of coincidence and time-of-flight technology for complex experiments are available;thus,and neutron decay events can be separated.The performance of SLEGS TOF spectrometer was systematically evaluated using offline experiments,in which the time resolution reached approximately 0.9 ns.
基金supported by the National Natural Science Foundation of China(Nos.11875311,11905274,12005280)the Chinese Academy of Sciences President’s International Fellowship Initiative(No.2021VMA0025).
文摘The Shanghai Laser Electron Gamma Source(SLEGS)is a powerful gamma source that provides MeV gamma-ray beams for nuclear science and technology.It was developed as one of the 16 beamline stations in the Phase Ⅱ Project of the Shanghai Synchrotron Radiation Facility.The slant-scattering mode is for the first time systematically employed in laser Compton scattering at SLEGS to produce energy-tunable quasi-monoenergetic gamma-ray beams.The SLEGS officially completed its commissioning from July to December 2021.Gamma rays in the energy range of 0.25-21.7 MeV with a flux of 2.1×10^(4)-1.2×10^(7) photons/s and an energy spread of 2-15% were produced during the test.This paper reports the results from commissioning the SLEGS beamline.
基金supported by the National Natural Science Foundation of China (Grant Nos. 11875311, 11905274, 1705156, U2032146, 11865010, 11765015, and 1160509)the Natural Science Foundation of Inner Mongolia, China (Grant Nos. 2019JQ01 and 2018MS01009)the Strategic Priority Research Program of the Chinese Academy of Sciences (Grant No. XDB34030000)。
文摘Silver indium cadmium(Ag–In–Cd) control rod is widely used in pressurized water reactor nuclear power plants,and it is continuously consumed in a high neutron flux environment. The mass ratio of ^(107)Ag in the Ag–In–Cd control rod is 41.44%. To accurately calculate the consumption value of the control rod, a reliable neutron reaction cross section of the ^(107)Ag is required. Meanwhile,^(107)Ag is also an important weak r nucleus. Thus, the cross sections for neutron induced interactions with ^(107)Ag are very important both in nuclear energy and nuclear astrophysics. The(n, γ) cross section of ^(107)Ag has been measured in the energy range of 1–60 eV using a back streaming white neutron beam line at China spallation neutron source. The resonance parameters are extracted by an R-matrix code. All the cross section of ^(107)Ag and resonance parameters are given in this paper as datasets. The datasets are openly available at http://www.doi.org/10.11922/sciencedb.j00113.00010.
基金financially supported by the Strategic Priority Research Program on Space Science of the Chinese Academy of Sciences (Grant No. XDA 15020800)the National Natural Science Foundation of China (Grant Nos. 12033010, 41604152 and U1938111)Foundation of Minor Planets of the Purple Mountain Observatory and Youth Innovation Promotion Association CAS (Grant No. 2018178)。
文摘The Closeby Habitable Exoplanet Survey(CHES) mission is proposed to discover habitable-zone Earth-like planets of nearby solar-type stars(~10 pc away from our solar system) via microarcsecond relative astrometry.The major scientific objectives of CHES are:to search for Earth Twins or terrestrial planets in habitable zones orbiting100 FGK nearby stars;further to conduct a comprehensive survey and extensively characterize nearby planetary systems.The primary payload is a high-quality,low-distortion,high-stability telescope.The optical subsystem is a coaxial three-mirror anastigmat(TMA) with a 1.2 m-aperture,0°.44 × 0°.44 field of view and 500 nm-900 nm working wave band.The camera focal plane is composed of a mosaic of 81 scientific CMOS detectors each with4 k × 4 k pixels.The heterodyne laser interferometric calibration technology is employed to ensure microarcsecond level(1 μas) relative astrometry precision to meet the requirements for detection of Earth-like planets.The CHES satellite operates at the Sun-Earth L2 point and observes all the target stars for 5 yr.CHES will offer the first direct measurements of true masses and inclinations of Earth Twins and super-Earths orbiting our neighbor stars based on microarcsecond astrometry from space.This will definitely enhance our understanding of the formation of diverse nearby planetary systems and the emergence of other worlds for solar-type stars,and finally provide insights to the evolution of our own solar system.
基金supported by the National Natural Science Foundation of China(Grant Nos.11875311,11905274,11705156,11605097,and U2032146)the Strategic Priority Research Program of Chinese Academy of Sciences(Grant No.XDB34030000)。
文摘The^(74)Se is one of 35 p-nuclei,and^(82)Se is a r-process only nucleus,and their(n,γ)cross sections are vital input parameters for nuclear astrophysics reaction network calculations.The neutron capture cross section in the resonance range of isotopes and even natural selenium samples has not been measured.Promptγ-rays originating from neutron-induced capture events were detected by four C_(6)D_(6) liquid scintillator detectors at the Back-n facility of China Spallation Neutron Source(CSNS).The pulse height weighting technique(PHWT)was used to analyze the data in the 1 e V to 100 ke V region.The deduced neutron capture cross section was compared with ENDF/B-VIII.0,JEFF-3.2,and JENDL-4.0,and some differences were found.Resonance parameters were extracted by the R-matrix code SAMMY in the 1 e V-1 ke V region.All the cross sections ofnatSe and resonance parameters are given in the datasets.The datasets are openly available at http://www.doi.org/10.11922/sciencedb.j00113.00019.
文摘Antigen 12, containing a phosphonyl peptide hapten with free C-terminal carboxylic group, was synthesized by 11 reaction steps. The design of the hapten was based on the transition state of peptide hydrolysis catalyzed by carboxypeptidase A.
文摘The monoclonal antibody ID11D7 to carboxypeptidase A (CPA) was prepared. Theinhibitory effect of McAb ID11D7 on the peptidase activity of CPA was measured. The result reflectsthat the McAb ID11D7 can competitively inhibit the peptidase activity of CPA with an apparentinhibitory constant of 6.3 × 10-9M. Based on this work. the McAb ID11D7 can be used as idiotypicantigen to prepare anti-idiotypic catalytic antibody with the peptidase activity similar to CPA.
文摘1, 5-Benzothiazepines 1 react with phenylacetyl chloride to give the title compounds.The structures of these new compounds were confirmed by elemental analysis, ~1H NMR, ^(13)C NMRand MS spectroscopy, and their configuration (the mutual positions of the substituents relative to theβ-lactam ring) and conformation of the compounds were determined by X-ray crystal analysis.
基金Wang S. is supported by the National Natural Science Foundation of China (Grant Nos. 10925313 and 10833001)the China Post doctoral Science Foundation (Grant No. 2011M500962)+4 种基金Z.H.B is supported by the National Natural Science Foundation of China (Grant Nos. 10503013 and 10933004)J.J.H is grateful for support by the National Natural Science Foundation of China (Grant Nos. 11273068, 10973044 and 10833001)the Natural Science Foundation of Jiangsu Province (Grant No. BK2009341)the Foundation of Minor Planets of Purple Mountain Observatorythe innovative and inter disciplinary program by CAS (Grant No. KJZD-EW-Z001)
文摘The Damocloids are a group of unusual asteroids that recently added a new member： 2010 EJ104. The dynamical evolution of the Damocloids may reveal a connection from the Main Belt to the Kuiper Belt and beyond the scattered disk. According to our simulations, two regions may be considered as possible origins of the Damocloids： the scattered disk, or a part of the Oort cloud, which will be perturbed to a transient region located between 700 AU and 1000 AU. Based on their potential origin, the Damocloids can be classified into two types, depending on their semi-major axes, and about 65.5% of the Damocloids are classified into type I which mainly originate from the Oort cloud. Whether the Damocloids are inactive nuclei of the Halley Family of Comets may depend on their origin. K
文摘The intramolecular reductive coupling reaction of 1,6-bis(subshtuted indolyl)hexane-1,6-dione using zero-valent titanium reagent as catalyst proderes the novel photochromic 1,2-diheterocyclic cyclohexenes 2, together with unexpected compounds 3
文摘目的探讨多发伤合并骨折患者外周血游离DNA、肿瘤坏死因子(TNF)-α水平变化对发生多器官功能障碍综合征(MODS)的预测价值。方法回顾性分析2016年5月至2019年5月南方医科大学深圳医院收治、受伤时间在24 h内的109例多发伤合并骨折患者的临床资料,按照MODS诊断标准将其分为MODS组(n=64)和非MODS组(n=45),另选择20例同期健康体检者为对照组,检测两组患者入院1、2、3 d及健康组外周血游离DNA和TNF-α水平。结果与健康组相比,MODS组和非MODS组患者外周血游离DNA和TNF-α含量均升高(P<0.05);入院后1、2、3 d MODS组上述指标均高于非MODS组,两组比较,差异有统计学意义(P<0.05);当游离DNA、TNF-α水平同时升高时,预测MODS的准确度最高,相对危险度为6.00,阳性预测值为99%。结论游离DNA、TNF-α可作为预测多发伤合并骨折患者并发MODS的指标,两者结合灵敏度和特异性更高。
文摘Twenty-seven oxadiazolino[5,4-d][1,5]benzodiheteropine derivatives have been synthesized by the 1,3-dipolar cycloaddition of benzodiheteropines with nitrile oxide 1,3-dipoles,their conformations and the characteristics of the newly formed oxadiazoline fused on them have been studied.It has also been found that the mass spectra show characteristic fragmentation patterns.
文摘A dodecapeptide extracted from rape pollen was synthesized using solid—phase method,its conforma- tions in different states were studied by FT—IR,CD,and its physiological activities were determined.Seven segments and five analogs were also synthesized to elucidate the structure—function relation.
